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Physical Review Letters

Quantized Atom-Field Dynamics in Unstable Cavities

Claus Lamprecht, Helmut Ritsch

Published May 10, 1999• 32 citations
Publisher

Abstract

We develop a quantum description for the dynamics of a single atom inside an unstable optical resonator. For spherical mirrors with a finite Gaussian aperture we find a discrete complete set of normalizable eigenmodes, their biorthogonal adjoint modes, eigenfrequencies, decay rates, and overlap integrals. With these modes we formulate a quantum description for the coupled dynamics of the field and a single atom inside the resonator. We find a strongly geometry and position dependent nonexponential decay probability. Under certain special conditions one gets a modified single-mode description incorporating the Petermann excess noise factor $K$ even on a single-atom level.

DOI
10.1103/physrevlett.82.3787

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Unexpected role of excess noise in spontaneous emission

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A single inverted two-level atom is used as a theoretical model for a quantum noise detector to investigate fundamental properties of excess noise in an unstable optical resonator. For a symmetric unstable spherical mirror cavity, we develop an analytic quantum description of the field in terms of a complete set of normalizable biorthogonal quasimodes and adjoint modes. Including the interaction with a single two-level atom leads to a description analogous to the Jaynes-Cummings model with modified coupling constants. One finds a strong position and geometry-dependent atomic decay probability proportional to the square root $\sqrt{K}$ of the excess noise factor K at the cavity center. Introducing an additional homogeneous gain one recovers the K-fold emission enhancement that has been predicted before for the linewidth of an unstable cavity laser. We find that excess noise may be viewed as a spatial redistribution of the field quantum noise inside the resonator. Taking a position average of the atomic decay rate over the cavity volume leads to a cancellation of the excess noise enhancement.

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The spontaneous emission of an excited atom in a lossy cavity with nonorthogonal eigenmodes is analyzed. The quantum Langevin formalism is used to describe the dynamics of the spontaneous decay. The analysis shows that the spontaneous decay is modified by the Q value and the effective mode volume factor of each cavity eigenmode. The effective mode volume is generalized for cavities with nonorthogonal modes, which can be a very significant modification in the microcavity regime. It is shown that the spontaneous decay is not enhanced by the excess noise factor as claimed by other analyses.

Physical Review Letters•Aug 30, 2006•11 citations
We develop a quantum description for the dynamics of a single atom inside an unstable optical resonator. For spherical mirrors with a finite Gaussian aperture we find a discrete complete set of normalizable eigenmodes, their biorthogonal adjoint modes, eigenfrequencies, decay rates, and overlap integrals. With these modes we formulate a quantum description for the coupled dynamics of the field and a single atom inside the resonator. We find a strongly geometry and position dependent nonexponential decay probability. Under certain special conditions one gets a modified single-mode description incorporating the Petermann excess noise factor KKK even on a single-atom level.
A single inverted two-level atom is used as a theoretical model for a quantum noise detector to investigate fundamental properties of excess noise in an unstable optical resonator. For a symmetric unstable spherical mirror cavity, we develop an analytic quantum description of the field in terms of a complete set of normalizable biorthogonal quasimodes and adjoint modes. Including the interaction with a single two-level atom leads to a description analogous to the Jaynes-Cummings model with modified coupling constants. One finds a strong position and geometry-dependent atomic decay probability proportional to the square root K\sqrt{K}K​ of the excess noise factor K at the cavity center. Introducing an additional homogeneous gain one recovers the K-fold emission enhancement that has been predicted before for the linewidth of an unstable cavity laser. We find that excess noise may be viewed as a spatial redistribution of the field quantum noise inside the resonator. Taking a position average of the atomic decay rate over the cavity volume leads to a cancellation of the excess noise enhancement.
Field quantization in unstable optical systems is treated by expanding the vector potential in terms of non-Hermitean (Fox-Li) modes. We define non-Hermitean modes and their adjoints in both the cavity and external regions and make use of the important bi-orthogonality relationships that exist within each mode set. We employ a standard canonical quantization procedure involving the introduction of generalized coordinates and momenta for the electromagnetic (EM) field. Three-dimensional systems are treated, making use of the paraxial and monochromaticity approximations for the cavity non-Hermitean modes. We show that the quantum EM field is equivalent to a set of quantum harmonic oscillators (QHOs), associated with either the cavity or the external region non-Hermitean modes, and thus confirming the validity of the photon model in unstable optical systems. Unlike in the conventional (Hermitean mode) case, the annihilation and creation operators we define for each QHO are not Hermitean adjoints. It is shown that the quantum Hamiltonian for the EM field is the sum of non-commuting cavity and external region contributions, each of which can be expressed as a sum of independent QHO Hamiltonians for each non-Hermitean mode, except that the external field Hamiltonian also includes a coupling term responsible for external non-Hermitean mode photon exchange processes. The non-commutativity of certain cavity and external region annihilation and creation operators is associated with cavity energy gain and loss processes, and may be described in terms of surface integrals involving cavity and external region non-Hermitean mode functions on the cavity-external region boundary. Using the essential states approach and the rotating wave approximation, our results are applied to the spontaneous decay of a two-level atom inside an unstable cavity. We find that atomic transitions leading to cavity non-Hermitean mode photon absorption are associated with a different coupling constant to that for transitions leading to photon emission, a feature consequent on the use of non-Hermitean mode functions. We show that under certain conditions the spontaneous decay rate is enhanced by the Petermann factor.
In the multimode regime of cavity quantum electrodynamics (cQED), light-matter coupling can be strong enough such as to allows a quantum emitter to couple with multiple resonant field modes. This regime leaves distinctive signatures in the behavior of both the field and the emitter, which are already accessible by modern experimental techniques. To model such effects in lossy cavities, effective discrete-mode approaches have been widely employed, despite their accuracy beyond two modes remaining rarely benchmarked. In this work, we demonstrate the necessity of employing multiple modes to describe the multimode signatures by analyzing the dynamics of an atom in a one-dimensional lossy resonator. The atom's dynamics is simulated using the formalism developed in Weitzel et al. (2026) (arXiv:2512.18478), where a resonance quantization prescription is provided. We investigate its dependency with respect to two different parameters: the light-matter coupling strength and the atom's position. In the former case, we find that the minimal number of modes necessary to capture the essential features of the atom's dynamics increases with the coupling strength. In the latter, we further observe that the multimode regime leads to a strong position-dependency of the atom's dynamics. In all cases, we discuss the physical interpretation of our results and further discuss about how the employed formalism can be used to recover physically relevant quantities.
We study the quantum properties of the electromagnetic field in optical cavities coupled to an arbitrary number of escape channels. We consider both inhomogeneous dielectric resonators with a scalar dielectric constant $\ensuremath{\epsilon}(\mathbf{r})$ and cavities defined by mirrors of arbitrary shape. Using the Feshbach projector technique we quantize the field in terms of a set of resonator and bath modes. We rigorously show that the field Hamiltonian reduces to the system-and-bath Hamiltonian of quantum optics. The field dynamics is investigated using the input-output theory of Gardiner and Collet. In the case of strong coupling to the external radiation field we find spectrally overlapping resonator modes. The mode dynamics is coupled due to the damping and noise inflicted by the external field. For wave chaotic resonators the mode dynamics is determined by a non-Hermitean random matrix. Upon including an amplifying medium, our dynamics of open-resonator modes may serve as a starting point for a quantum theory of random lasing.
The quantum theory of a one-dimensional optical cavity is developed with emphasis on the presence of output coupling. First the resonant mode is defined and calculated classically. Then the field is decomposed into a sequence of modes by introducing an imaginary boundary at a large distance. The mode functions are proved to be orthogonal with respect to an integration with the dielectric constant as a weighting factor. The Hamiltonian of the field is shown to be equivalent to that of a collection of independent harmonic oscillators, the mass of which is a function of the frequency of oscillation. This equivalent of mass appears on normalizing the mode functions and proves to carry information on the structure of the cavity. Quantization of the field is carried out, and the commutation relation for the electric fields inside and outside the cavity is derived. The commutator is composed of an infinite set of derivatives of $\ensuremath{\delta}$ functions, which discloses the effect of the presence of output coupling and that of the small size of the cavity on the radiation field. Also, the commutator is shown to have some properties common with the classical resonant mode, i.e., the property of exponential decay and its rate.
The spontaneous emission of an excited atom in a lossy cavity with nonorthogonal eigenmodes is analyzed. The quantum Langevin formalism is used to describe the dynamics of the spontaneous decay. The analysis shows that the spontaneous decay is modified by the Q value and the effective mode volume factor of each cavity eigenmode. The effective mode volume is generalized for cavities with nonorthogonal modes, which can be a very significant modification in the microcavity regime. It is shown that the spontaneous decay is not enhanced by the excess noise factor as claimed by other analyses.