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Science

FFLO on the Horizon

J. Stajic

Published Oct 21, 2010• 1 citation
Publisher

Abstract

Physics Such counterintuitive phenomena as the flow of electrical current through a solid without any dissipation, or the zero viscosity of 3He at low temperatures, may be explained by the unlikely pairing of the electrons or He atoms (respectively) that constitute the flow. In the simplest case, pairing occurs between fermions of opposite spins and momenta, so that the total momentum of a pair is zero. Usually, the numbers of fermions of opposite spins is balanced, so that each up-spin has a down-spin partner; an exotic situation when this is not the case may lead to the formation of the so-called Fulde-Ferrell-Larkin-Ovchinnikov (FFLO), state, in which the pair momentum is finite and the pair density is oscillating in space. It is expected that this state will be the most stable in a one-dimensional (1D) wire-like system. Liao et al. recreate this situation in an ultracold gas of 6Li confined to an array of 1D tubes. In line with theoretical predictions, the measured spin density profiles indicate that a core with unequal densities of up- and down-spins (a potential FFLO state) is flanked by either a fully paired or a fully spin-polarized state, depending on the overall degree of spin imbalance. Although not a direct demonstration of an FFLO state, the experiment may set the groundwork for such observations in the future. Nature 467 , 567 (2010).

DOI
10.1126/science.330.6003.429-b

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Spin-Imbalance in One and Three-Dimensional Fermi Gases

Randall G. Hulet

The FFLO modulated superconductor state was independently proposed by Fulde and Ferrell, and Larkin and Ovchinnikov, as a way of accommodating the excess spin in a spin-polarized superconductor. The pairs in the FFLO state have non-zero center-of-mass momentum, which can produce a periodic structure with a spatially-modulated order parameter. Although there is some evidence for FFLO pairing in certain heavy fermion compounds that are able to accommodate both magnetic and superconducting order, conclusive experimental proof remains elusive. Motivated by the search for exotic paired states, we have performed experiments with spin-imbalanced ultracold atomic Fermi gases in both 3D and 1D. We use two hyperfine levels of 6Li to emulate the spin-up and down states. The s-wave pairing interactions are controlled via a magnetically-tuned collisional (Feshbach) resonance. In 3D, we find that the gas phase separates into an evenly paired BCS-like core, surrounded by the excess spin-up atoms [1]. For the 1D experiment, a two-dimensional optical lattice was used to create an array of 1D tubes that are each filled with ∼200 atoms. The weak axial confinement again produces a phase separation, but in contrast to 3D we find a partially-polarized central core surrounded by either fully-paired or fully-polarized wings, depending on the degree of overall spin-polarization [2]. Theory predicts that the partially-polarized phase is an FFLO superfluid. We are currently trying to obtain direct evidence for FFLO pairing, which may be revealed in the pair momentum distribution found by releasing the atoms axially and allowing them to expand in time-of-flight. We are also exploring the 1D-3D dimensional crossover that occurs when the coupling between tubes is reduced.

Bulletin of the American Physical Society•Feb 28, 2012•0 citations

The Search For FFLO in a Quasi-One-Dimensional Ultracold Fermi Gas

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The Fulde-Ferrell Larkin-Ovchinnikov (FFLO) type superconductor is an exotic form of matter known as a supersolid because it simultaneously supports superfluid and magnetic order. In both condensed matter and ultracold atomic gases, this phase has yet to be conclusively observed despite long interest in both theory and experiment. In one-dimension (1D), unlike expectations for higher dimensions, the FFLO phase is found in a large region of the phase diagram [1]. The effect of quantum and thermal fluctuations, however, are expected to be reduced in higher dimensions. These considerations motivated the proposal to search for FFLO near the 1D-3D dimensional crossover [2], which we have identified and characterized [3]. We confine a spin-imbalanced Fermi gas of lithium 6 to an array of 1D tubes using a 2D optical lattice. We bring the system into the dimensional crossover by increasing the inter-tube tunneling rate and using a Feshbach resonance to tune interactions. The periodicity of these domain walls, which depends on the magnitude of the polarization, is a definitive signature of the FFLO phase. In this work, we develop new experimental and analytical methods to extract periodic signals that, if they indeed are domain walls, lay the foundation for full confirmation of the FFLO phase. [1] Y. A. Liao, A. S. C. Rittner, T. Paprotta, W. Li, G. B. Partridge, R. G. Hulet, S. K. Baur, and E. J. Mueller, “Spin-imbalance in a one-dimensional Fermi gas,” Nature 467, 567 (2010). [2] M. M. Parish, S. K. Baur, E. J. Mueller, and D. A. Huse, “Quasi-One- Dimensional Polarized Fermi Superfluids,” Phys. Rev. Lett. 99, 250403 (2007). [3] M. C. Revelle, J. A. Fry, B. A. Olsen, and R. G. Hulet, “1D to 3D Crossover of a Spin-Imbalanced Fermi Gas,” Physical Review Letters 117 (2016).

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The recent development of experimental techniques in ultracold atomic Fermi gases is extremely helpful in the progress of the realization of the unconventional Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) superfluid phase in quasi-one dimensional systems (Liao et al 2010 Nature 467 567). Due to a Fermi surface nesting, which is enhanced in 1D, the low-dimensional systems are particularly good candidates to find the FFLO phase stable. We investigate the influence of a dimensional crossover (from one dimension (1D) to two dimensions (2D) or three dimensions (3D)) on the stability of the FFLO state in the spin-imbalanced attractive Hubbard model.

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Realization and Detection of Fulde-Ferrell-Larkin-Ovchinnikov Superfluid Phases in Trapped Atomic Fermion Systems

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In a very interesting recent Letter\cite{machida}, the authors suggested the possibility of realizing the spatially modulated, or Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) superfluid state in trapped atomic fermion systems. The authors this Letter used a 1D mean field solution as guidance to estimate the parameter range for the existence of the FFLO phase, and also discussed the possibility of its detection by imaging the atomic density of the system. In this comment I wish to make two points. (i) In 1D there exists an exact solution based on bosonization, which fully takes into account the important quantum fluctuation effects\cite{yang01}; the exact solution suggests a wider parameter range for the FFLO state than that obtained from the mean-field solution of the present Letter. (ii) One can detect the FFLO pairing (in which Cooper pairs carry finite momenta) more directly by extending the methods used to detect BCS pairing\cite{regal,altman,greiner}.

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The exotic Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) states have been actively searched for experimentally since the mean-field based FFLO theories were put forward half a century ago. Here, we investigate the stability of FFLO states in the presence of pairing fluctuations. We conclude that FFLO superfluids cannot exist in continuum in three and two dimensions, due to their intrinsic instability, associated with infinite quantum degeneracy of the pairs. These results address the absence of convincing experimental observations of FFLO phases in both condensed matter and in ultracold atomic Fermi gases with a population imbalance. We predict that the true ground state has a pair momentum distribution highly peaked on an entire constant energy surface.

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Physics
Such counterintuitive phenomena as the flow of electrical current through a solid without any dissipation, or the zero viscosity of 3He at low temperatures, may be explained by the unlikely pairing of the electrons or He atoms (respectively) that constitute the flow. In the simplest case, pairing occurs between fermions of opposite spins and momenta, so that the total momentum of a pair is zero. Usually, the numbers of fermions of opposite spins is balanced, so that each up-spin has a down-spin partner; an exotic situation when this is not the case may lead to the formation of the so-called Fulde-Ferrell-Larkin-Ovchinnikov (FFLO), state, in which the pair momentum is finite and the pair density is oscillating in space. It is expected that this state will be the most stable in a one-dimensional (1D) wire-like system. Liao et al. recreate this situation in an ultracold gas of 6Li confined to an array of 1D tubes. In line with theoretical predictions, the measured spin density profiles indicate that a core with unequal densities of up- and down-spins (a potential FFLO state) is flanked by either a fully paired or a fully spin-polarized state, depending on the overall degree of spin imbalance. Although not a direct demonstration of an FFLO state, the experiment may set the groundwork for such observations in the future.
Nature 467 , 567 (2010).
The FFLO modulated superconductor state was independently proposed by Fulde and Ferrell, and Larkin and Ovchinnikov, as a way of accommodating the excess spin in a spin-polarized superconductor. The pairs in the FFLO state have non-zero center-of-mass momentum, which can produce a periodic structure with a spatially-modulated order parameter. Although there is some evidence for FFLO pairing in certain heavy fermion compounds that are able to accommodate both magnetic and superconducting order, conclusive experimental proof remains elusive. Motivated by the search for exotic paired states, we have performed experiments with spin-imbalanced ultracold atomic Fermi gases in both 3D and 1D. We use two hyperfine levels of 6Li to emulate the spin-up and down states. The s-wave pairing interactions are controlled via a magnetically-tuned collisional (Feshbach) resonance. In 3D, we find that the gas phase separates into an evenly paired BCS-like core, surrounded by the excess spin-up atoms [1]. For the 1D experiment, a two-dimensional optical lattice was used to create an array of 1D tubes that are each filled with ∼200 atoms. The weak axial confinement again produces a phase separation, but in contrast to 3D we find a partially-polarized central core surrounded by either fully-paired or fully-polarized wings, depending on the degree of overall spin-polarization [2]. Theory predicts that the partially-polarized phase is an FFLO superfluid. We are currently trying to obtain direct evidence for FFLO pairing, which may be revealed in the pair momentum distribution found by releasing the atoms axially and allowing them to expand in time-of-flight. We are also exploring the 1D-3D dimensional crossover that occurs when the coupling between tubes is reduced.
The Fulde-Ferrell Larkin-Ovchinnikov (FFLO) type superconductor is an exotic form of matter known as a supersolid because it simultaneously supports superfluid and magnetic order. In both condensed matter and ultracold atomic gases, this phase has yet to be conclusively observed despite long interest in both theory and experiment. In one-dimension (1D), unlike expectations for higher dimensions, the FFLO phase is found in a large region of the phase diagram [1]. The effect of quantum and thermal fluctuations, however, are expected to be reduced in higher dimensions. These considerations motivated the proposal to search for FFLO near the 1D-3D dimensional crossover [2], which we have identified and characterized [3]. We confine a spin-imbalanced Fermi gas of lithium 6 to an array of 1D tubes using a 2D optical lattice. We bring the system into the dimensional crossover by increasing the inter-tube tunneling rate and using a Feshbach resonance to tune interactions. The periodicity of these domain walls, which depends on the magnitude of the polarization, is a definitive signature of the FFLO phase. In this work, we develop new experimental and analytical methods to extract periodic signals that, if they indeed are domain walls, lay the foundation for full confirmation of the FFLO phase. [1] Y. A. Liao, A. S. C. Rittner, T. Paprotta, W. Li, G. B. Partridge, R. G. Hulet, S. K. Baur, and E. J. Mueller, “Spin-imbalance in a one-dimensional Fermi gas,” Nature 467, 567 (2010). [2] M. M. Parish, S. K. Baur, E. J. Mueller, and D. A. Huse, “Quasi-One- Dimensional Polarized Fermi Superfluids,” Phys. Rev. Lett. 99, 250403 (2007). [3] M. C. Revelle, J. A. Fry, B. A. Olsen, and R. G. Hulet, “1D to 3D Crossover of a Spin-Imbalanced Fermi Gas,” Physical Review Letters 117 (2016).
The recent development of experimental techniques in ultracold atomic Fermi gases is extremely helpful in the progress of the realization of the unconventional Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) superfluid phase in quasi-one dimensional systems (Liao et al 2010 Nature 467 567). Due to a Fermi surface nesting, which is enhanced in 1D, the low-dimensional systems are particularly good candidates to find the FFLO phase stable. We investigate the influence of a dimensional crossover (from one dimension (1D) to two dimensions (2D) or three dimensions (3D)) on the stability of the FFLO state in the spin-imbalanced attractive Hubbard model.
We review the concepts and the present state of theoretical studies of spin-imbalanced superfluidity, in particular the elusive Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state, in the context of ultracold quantum gases. The comprehensive presentation of the theoretical basis for the FFLO state that we provide is useful also for research on the interplay between magnetism and superconductivity in other physical systems. We focus on settings that have been predicted to be favourable for the FFLO state, such as optical lattices in various dimensions and spin-orbit coupled systems. These are also the most likely systems for near-future experimental observation of the FFLO state. Theoretical bounds, such as Bloch's and Luttinger's theorems, and experimentally important limitations, such as finite-size effects and trapping potentials, are considered. In addition, we provide a comprehensive review of the various ideas presented for the observation of the FFLO state. We conclude our review with an analysis of the open questions related to the FFLO state, such as its stability, superfluid density, collective modes and extending the FFLO superfluid concept to new types of lattice systems.
In a very interesting recent Letter\cite{machida}, the authors suggested the possibility of realizing the spatially modulated, or Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) superfluid state in trapped atomic fermion systems. The authors this Letter used a 1D mean field solution as guidance to estimate the parameter range for the existence of the FFLO phase, and also discussed the possibility of its detection by imaging the atomic density of the system. In this comment I wish to make two points. (i) In 1D there exists an exact solution based on bosonization, which fully takes into account the important quantum fluctuation effects\cite{yang01}; the exact solution suggests a wider parameter range for the FFLO state than that obtained from the mean-field solution of the present Letter. (ii) One can detect the FFLO pairing (in which Cooper pairs carry finite momenta) more directly by extending the methods used to detect BCS pairing\cite{regal,altman,greiner}.
The exotic Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) states have been actively searched for experimentally since the mean-field based FFLO theories were put forward half a century ago. Here, we investigate the stability of FFLO states in the presence of pairing fluctuations. We conclude that FFLO superfluids cannot exist in continuum in three and two dimensions, due to their intrinsic instability, associated with infinite quantum degeneracy of the pairs. These results address the absence of convincing experimental observations of FFLO phases in both condensed matter and in ultracold atomic Fermi gases with a population imbalance. We predict that the true ground state has a pair momentum distribution highly peaked on an entire constant energy surface.