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The Search For FFLO in a Quasi-One-Dimensional Ultracold Fermi Gas

Jacob A. Fry

Published Apr 20, 2022• 0 citations
OpenAlex

Abstract

The Fulde-Ferrell Larkin-Ovchinnikov (FFLO) type superconductor is an exotic form of matter known as a supersolid because it simultaneously supports superfluid and magnetic order. In both condensed matter and ultracold atomic gases, this phase has yet to be conclusively observed despite long interest in both theory and experiment. In one-dimension (1D), unlike expectations for higher dimensions, the FFLO phase is found in a large region of the phase diagram [1]. The effect of quantum and thermal fluctuations, however, are expected to be reduced in higher dimensions. These considerations motivated the proposal to search for FFLO near the 1D-3D dimensional crossover [2], which we have identified and characterized [3]. We confine a spin-imbalanced Fermi gas of lithium 6 to an array of 1D tubes using a 2D optical lattice. We bring the system into the dimensional crossover by increasing the inter-tube tunneling rate and using a Feshbach resonance to tune interactions. The periodicity of these domain walls, which depends on the magnitude of the polarization, is a definitive signature of the FFLO phase. In this work, we develop new experimental and analytical methods to extract periodic signals that, if they indeed are domain walls, lay the foundation for full confirmation of the FFLO phase. [1] Y. A. Liao, A. S. C. Rittner, T. Paprotta, W. Li, G. B. Partridge, R. G. Hulet, S. K. Baur, and E. J. Mueller, “Spin-imbalance in a one-dimensional Fermi gas,” Nature 467, 567 (2010). [2] M. M. Parish, S. K. Baur, E. J. Mueller, and D. A. Huse, “Quasi-One- Dimensional Polarized Fermi Superfluids,” Phys. Rev. Lett. 99, 250403 (2007). [3] M. C. Revelle, J. A. Fry, B. A. Olsen, and R. G. Hulet, “1D to 3D Crossover of a Spin-Imbalanced Fermi Gas,” Physical Review Letters 117 (2016).

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Ultracold atoms have become an essential tool in studying condensed matter phenomena. The advantage of atomic physics experiments is that they provide an easily tunable system. This experiment uses the lowest two ground state hyperfine levels of fermionic lithium. Having two different states creates a pseudo-spin-1/2 system and allows us to emulate electronic systems, such as superconductors and crystal lattices. In our experiment, we can control the ratio between these two states resulting in either a spin-balanced or a spin-imbalanced gas. Imposing an imbalance is analogous to applying a magnetic field to a superconductor which causes the electrons in the material to align to the field (thus breaking the electron pairs which cause superconductivity). This motivates us to understand the phases created when a spin-imbalance is created and the effect of changing the atomic interactions. In a 3D system, we find where superfluidity is suppressed throughout the BEC to BCS crossover. Using phase separation as a guide, we probe the dimensional crossover between 1D and 3D. The phase separation in 1D is inverted from that in 3D, which provides a unique characteristic to distinguish between the dimensions. By varying the tunneling between tubes and the atomic interactions in a 2D optical lattice, we control whether the system is 1D, 3D, or in between. Using the properties of a 3D gas as a guide, we directly observe when the gas has crossed over from being dominated by 1D-like behavior to 3D. In this way, we have found a universal value for the dimensional crossover. The 1D-3D crossover paves the way to search for the exotic FFLO (Fulde-Ferrell-Larkin-Ovchinnikov) superconductor. While most superconductors do not coexist with magnetism, the FFLO phase requires large magnetic fields to support its pairing mechanism. Additionally, this phase is more likely to be found in lower dimensional systems. However, at low dimensions, the effect of temperature fluctuations on the phase is destabilizing, but these temperature effects are reduced with higher dimensionality. Thus, the quasi-1D regime is the optimal region of parameter space to find this phase. The search for direct evidence of FFLO continues in this regime.

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The question whether an imbalanced Fermi gas can accommodate polarized superfluidity has been the subject of intense study. One prominent candidate for a polarized superfluid state is the Fulde–Ferrell–Larkin–Ovchinnikov (FFLO) state. In a one-dimensional (1D) Fermi gas, indirect evidence for this state has recently been found, but in the three-dimensional (3D) case, this exotic state has hitherto remained elusive. In this brief review, we study the influence of a 1D periodic potential on the FFLO state in an imbalanced 3D Fermi gas. We present a path-integral derivation of the free energy of the system, where the possibility of the FFLO state is included through the saddle-point approximation. Using the free energy, the phase diagram of the system, both at fixed chemical potentials and at fixed densities, is constructed, showing that the stability region of the FFLO state is significantly enlarged by the 1D potential. Subsequently, the influence of the potential on the FFLO pairing mechanism is investigated, leading to a qualitative understanding of the shape of the FFLO region in the different phase diagrams. We conclude by investigating the possibility of an FFLO state with a wave vector that lies skewed with respect to the direction along which the periodic potential varies. Our results provide an additional way to facilitate the experimental observation of the FFLO state in a 3D Fermi gas.

Modern Physics Letters B•Jul 27, 2012•7 citations
The Fulde-Ferrell Larkin-Ovchinnikov (FFLO) type superconductor is an exotic form of matter known as a supersolid because it simultaneously supports superfluid and magnetic order. In both condensed matter and ultracold atomic gases, this phase has yet to be conclusively observed despite long interest in both theory and experiment. In one-dimension (1D), unlike expectations for higher dimensions, the FFLO phase is found in a large region of the phase diagram [1]. The effect of quantum and thermal fluctuations, however, are expected to be reduced in higher dimensions. These considerations motivated the proposal to search for FFLO near the 1D-3D dimensional crossover [2], which we have identified and characterized [3]. We confine a spin-imbalanced Fermi gas of lithium 6 to an array of 1D tubes using a 2D optical lattice. We bring the system into the dimensional crossover by increasing the inter-tube tunneling rate and using a Feshbach resonance to tune interactions. The periodicity of these domain walls, which depends on the magnitude of the polarization, is a definitive signature of the FFLO phase. In this work, we develop new experimental and analytical methods to extract periodic signals that, if they indeed are domain walls, lay the foundation for full confirmation of the FFLO phase. [1] Y. A. Liao, A. S. C. Rittner, T. Paprotta, W. Li, G. B. Partridge, R. G. Hulet, S. K. Baur, and E. J. Mueller, “Spin-imbalance in a one-dimensional Fermi gas,” Nature 467, 567 (2010). [2] M. M. Parish, S. K. Baur, E. J. Mueller, and D. A. Huse, “Quasi-One- Dimensional Polarized Fermi Superfluids,” Phys. Rev. Lett. 99, 250403 (2007). [3] M. C. Revelle, J. A. Fry, B. A. Olsen, and R. G. Hulet, “1D to 3D Crossover of a Spin-Imbalanced Fermi Gas,” Physical Review Letters 117 (2016).
Ultracold atoms have become an essential tool in studying condensed matter phenomena. The advantage of atomic physics experiments is that they provide an easily tunable system. This experiment uses the lowest two ground state hyperfine levels of fermionic lithium. Having two different states creates a pseudo-spin-1/2 system and allows us to emulate electronic systems, such as superconductors and crystal lattices. In our experiment, we can control the ratio between these two states resulting in either a spin-balanced or a spin-imbalanced gas. Imposing an imbalance is analogous to applying a magnetic field to a superconductor which causes the electrons in the material to align to the field (thus breaking the electron pairs which cause superconductivity). This motivates us to understand the phases created when a spin-imbalance is created and the effect of changing the atomic interactions. In a 3D system, we find where superfluidity is suppressed throughout the BEC to BCS crossover. Using phase separation as a guide, we probe the dimensional crossover between 1D and 3D. The phase separation in 1D is inverted from that in 3D, which provides a unique characteristic to distinguish between the dimensions. By varying the tunneling between tubes and the atomic interactions in a 2D optical lattice, we control whether the system is 1D, 3D, or in between. Using the properties of a 3D gas as a guide, we directly observe when the gas has crossed over from being dominated by 1D-like behavior to 3D. In this way, we have found a universal value for the dimensional crossover. The 1D-3D crossover paves the way to search for the exotic FFLO (Fulde-Ferrell-Larkin-Ovchinnikov) superconductor. While most superconductors do not coexist with magnetism, the FFLO phase requires large magnetic fields to support its pairing mechanism. Additionally, this phase is more likely to be found in lower dimensional systems. However, at low dimensions, the effect of temperature fluctuations on the phase is destabilizing, but these temperature effects are reduced with higher dimensionality. Thus, the quasi-1D regime is the optimal region of parameter space to find this phase. The search for direct evidence of FFLO continues in this regime.
The FFLO modulated superconductor state was independently proposed by Fulde and Ferrell, and Larkin and Ovchinnikov, as a way of accommodating the excess spin in a spin-polarized superconductor. The pairs in the FFLO state have non-zero center-of-mass momentum, which can produce a periodic structure with a spatially-modulated order parameter. Although there is some evidence for FFLO pairing in certain heavy fermion compounds that are able to accommodate both magnetic and superconducting order, conclusive experimental proof remains elusive. Motivated by the search for exotic paired states, we have performed experiments with spin-imbalanced ultracold atomic Fermi gases in both 3D and 1D. We use two hyperfine levels of 6Li to emulate the spin-up and down states. The s-wave pairing interactions are controlled via a magnetically-tuned collisional (Feshbach) resonance. In 3D, we find that the gas phase separates into an evenly paired BCS-like core, surrounded by the excess spin-up atoms [1]. For the 1D experiment, a two-dimensional optical lattice was used to create an array of 1D tubes that are each filled with ∼200 atoms. The weak axial confinement again produces a phase separation, but in contrast to 3D we find a partially-polarized central core surrounded by either fully-paired or fully-polarized wings, depending on the degree of overall spin-polarization [2]. Theory predicts that the partially-polarized phase is an FFLO superfluid. We are currently trying to obtain direct evidence for FFLO pairing, which may be revealed in the pair momentum distribution found by releasing the atoms axially and allowing them to expand in time-of-flight. We are also exploring the 1D-3D dimensional crossover that occurs when the coupling between tubes is reduced.
The recent development of experimental techniques in ultracold atomic Fermi gases is extremely helpful in the progress of the realization of the unconventional Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) superfluid phase in quasi-one dimensional systems (Liao et al 2010 Nature 467 567). Due to a Fermi surface nesting, which is enhanced in 1D, the low-dimensional systems are particularly good candidates to find the FFLO phase stable. We investigate the influence of a dimensional crossover (from one dimension (1D) to two dimensions (2D) or three dimensions (3D)) on the stability of the FFLO state in the spin-imbalanced attractive Hubbard model.
We calculate the zero-temperature (T=0) phase diagram of a polarized two-component Fermi gas in an array of weakly coupled parallel one-dimensional (1D) "tubes" produced by a two-dimensional optical lattice. Increasing the lattice strength drives a crossover from three-dimensional (3D) to 1D behavior, stabilizing the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) modulated superfluid phase. We argue that the most promising regime for observing the FFLO phase is in the quasi-1D regime, where the atomic motion is largely 1D but there is weak tunneling in the other directions that stabilizes long-range order. In the FFLO phase, we describe a phase transition where the quasiparticle spectrum changes from gapless near the 3D regime to gapped in quasi-1D.
Ultracold atomic gases have emerged as an ideal laboratory system to emulate many-body physics in an unprecedentedly controllable manner. Numerous many-body quantum states and phases have been experimentally explored and characterized using the ultracold atomic gases, offering new insights into many exciting physics ranging from condensed matters to cosmology. In this thesis, we will present a systematic numerical study of a novel experimental system, population imbalanced two-component ultracold Fermi gases. We explore the phase diagram of this system in both 3D and 1D especially focusing on the exotic Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase, which is characterized by a spatially oscillating order parameter. In 3D, we solve for the stationary states of trapped imbalanced Fermi gases in a wide range of parameter space with a home-made parallel eigen-solver for Bogoliubov-de Gennes (BdG) equations. Our results show that there exists a metastable state with a FFLO type oscillating order parameter. In 1D, we simulate the dynamical expansion of the population imbalanced Fermi gases from the trap. A numerically quasi-exact scheme, time-evolving block decimation (TEBD), is introduced for the comparative studies with the solution of the time-dependent BdG equation. Our results predict that the existence of FFLO states will leave conspicuous signatures in the density profiles during the expansion. For further understanding of the interplay between the population imbalance and two-body pairing interaction between two spin components, we also study the spin transport properties through trapped ultracold Fermi gases. The preliminary results will be discussed.
The question whether an imbalanced Fermi gas can accommodate polarized superfluidity has been the subject of intense study. One prominent candidate for a polarized superfluid state is the Fulde–Ferrell–Larkin–Ovchinnikov (FFLO) state. In a one-dimensional (1D) Fermi gas, indirect evidence for this state has recently been found, but in the three-dimensional (3D) case, this exotic state has hitherto remained elusive. In this brief review, we study the influence of a 1D periodic potential on the FFLO state in an imbalanced 3D Fermi gas. We present a path-integral derivation of the free energy of the system, where the possibility of the FFLO state is included through the saddle-point approximation. Using the free energy, the phase diagram of the system, both at fixed chemical potentials and at fixed densities, is constructed, showing that the stability region of the FFLO state is significantly enlarged by the 1D potential. Subsequently, the influence of the potential on the FFLO pairing mechanism is investigated, leading to a qualitative understanding of the shape of the FFLO region in the different phase diagrams. We conclude by investigating the possibility of an FFLO state with a wave vector that lies skewed with respect to the direction along which the periodic potential varies. Our results provide an additional way to facilitate the experimental observation of the FFLO state in a 3D Fermi gas.