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Journal of Modern Optics

Magnetism in ultracold quantum gases

H. Schmaljohann, M. Erhard, J. Kronjägert, M. Kottke, S. van Staa, J. Arlt, Kai Bongs, K. Sengstock

Published Jun 18, 2004• 2 citations
Publisher

Abstract

We study the static and dynamic magnetic properties of ultracold quantum gases, in particular the spinor physics of F = 1 and F = 2 Bose-Einstein condensates of 87Rb atoms. Our data lead to the conclusion, that the F = 2 ground state of 87Rb is polar, while we find the F = 1 ground state to be ferromagnetic. The dynamics of spinor systems is linked to an interplay between coherent mean-field interactions, losses and interactions with atoms in the thermal cloud. Within this rich parameter space we observe indications for coherent spinor dynamics and novel thermalization regimes.

DOI
10.1080/09500340408232494

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We study the static and dynamic magnetic properties of ultracold quantum gases, in particular the spinor physics of F = 1 and F = 2 Bose-Einstein condensates of 87Rb atoms. Our data lead to the conclusion, that the F = 2 ground state of 87Rb is polar, while we find the F = 1 ground state to be ferromagnetic. The dynamics of spinor systems is linked to an interplay between coherent mean-field interactions, losses and interactions with atoms in the thermal cloud. Within this rich parameter space we observe indications for coherent spinor dynamics and novel thermalization regimes.
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We experimentally investigate and analyze the rich dynamics in F=2F=2F=2 spinor Bose-Einstein condensates of 87Rb^{87}\mathrm{R}\mathrm{b}87Rb. An interplay between mean-field driven spin dynamics and hyperfine-changing losses in addition to interactions with the thermal component is observed. In particular, we measure conversion rates in the range of ${10}^{\ensuremath{-}12}\text{ }\text{ }{\mathrm{c}\mathrm{m}}^{3}\text{ }{\mathrm{s}}^{\ensuremath{-}1}$ for spin-changing collisions within the F=2F=2F=2 manifold and spin-dependent loss rates in the range of ${10}^{\ensuremath{-}13}\text{ }\text{ }{\mathrm{c}\mathrm{m}}^{3}\text{ }{\mathrm{s}}^{\ensuremath{-}1}$ for hyperfine-changing collisions. We observe polar behavior in the F=2F=2F=2 ground state of 87Rb^{87}\mathrm{R}\mathrm{b}87Rb, while we find the F=1F=1F=1 ground state to be ferromagnetic. We further see a magnetization for condensates prepared with nonzero total spin.
Spinor Bose gases form a family of quantum fluids manifesting both magnetic order and superfluidity. This article reviews experimental and theoretical progress in understanding the static and dynamic properties of these fluids. The connection between system properties and the rotational symmetry properties of the atomic states and their interactions are investigated. Following a review of the experimental techniques used for characterizing spinor gases, their mean-field and many-body ground states, both in isolation and under the application of symmetry-breaking external fields, are discussed. These states serve as the starting point for understanding low-energy dynamics, spin textures, and topological defects, effects of magnetic-dipole interactions, and various nonequilibrium collective spin-mixing phenomena. The paper aims to form connections and establish coherence among the vast range of works on spinor Bose gases, so as to point to open questions and future research opportunities.
We study the nonequilibrium coherent spin-mixing dynamics in ferromagnetic spin-1 and antiferromagnetic spin-2 thermal gases of ultracold 87Rb^{87}\mathrm{Rb}87Rb atoms. Long-lasting spin population oscillations with magnetic-field-dependent resonances are observed in both cases. Our observations are well reproduced by Boltzmann equations of the Wigner distribution function. Compared to the equation of motion of spinor Bose-Einstein condensates, the only difference here is a factor-of-2 increase in the spin-dependent interaction, which is confirmed directly in the spin-2 case by measuring the relation between the oscillation amplitude and the sample's density.
Spinor Bose gases form a family of quantum fluids manifesting both magnetic order and superfluidity. This article reviews experimental and theoretical progress in understanding the static and dynamic properties of these fluids. The connection between system properties and the rotational symmetry properties of the atomic states and their interactions are investigated. Following a review of the experimental techniques used for characterizing spinor gases, their mean-field and many-body ground states, both in isolation and under the application of symmetry-breaking external fields, are discussed. These states serve as the starting point for understanding low-energy dynamics, spin textures and topological defects, effects of magnetic dipole interactions, and various non-equilibrium collective spin-mixing phenomena. The paper aims to form connections and establish coherence among the vast range of works on spinor Bose gases, so as to point to open questions and future research opportunities.
Bose-Einstein condensation (BEC) is a phenomenon in which identical bosons occupy the same quantum state below a certain critical temperature. A hallmark of BEC is the coherence between particles every particle shares the same quantum wavefunction and phase. This coherence has been demonstrated for the external (motional) degrees of freedom of the atomic condensates by interfering two condensates. In this thesis, the coherence is shown to extend to the internal spin degrees of freedom of a spin-1 Bose gas evidenced by the observed coherent and reversible spin-changing collisions. The observed coherent dynamics are analogous to Josephson oscillations in weakly connected superconductors and represent a type of matter-wave four-wave mixing. Control of the coherent evolution of the system using magnetic fields is also demonstrated. The studies on spinor condensates begin by creating spinor condensates directly using all-optical approaches that were first developed in our laboratory. All-optical formation of Bose-Einstein condensates (BEC) in 1D optical lattice and single focus trap geometries are developed and presented. These techniques offer considerable flexibility and speed compared to magnetic trap approaches, and the trapping potential can be essentially spin-independent and are ideally suited for studying spinor condensates. Using condensates with well-defined initial non-equilibrium spin configuration, spin mixing of F = 1 and F = 2 spinor condensates of rubidium-87 atoms confined in an optical trap is observed. The equilibrium spin configuration in the F = 1 manifold confirms that 87Rb is ferromagnetic. The coherent spinor dynamics are demonstrated by initiating spin mixing deterministically with a non-stationary spin population configuration. Finally, the interplay between the coherent spin mixing and spatial dynamics in spin-1 condensates with ferromagnetic interactions is investigated.