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Journal of Chemical Sciences

Superlocalization of fracton wavefunctions excited on percolating networks

Kousuke Yakubo, Tsuneyoshi Nakayama

Published Oct 1, 1990• 2 citations
Publisher
DOI
10.1007/bf03040784

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Characteristics of Fractons: from Specific Realizations to Ensemble Averages

Tsuneyoshi Nakayama, Kousuke Yakubo, R. Orbach

Specific realizations due to computer experiments show that fracton excitations possess a core in which the vibrational amplitudes fall off sharply at their edges. When constructing the ensemble average of the fracton wave functions, we find \(\langle\phi_{\text{fr}}\rangle{\sim}\exp[-(r/\varLambda(\omega))^{d_{\phi}}]\), where \(\varLambda(\omega){\sim}\omega^{-0.71}\). The exponent, -0.71, is in close agreement with the prediction of the fracton dispersion law for a two-dimensional percolating network, -0.705, and the geometrical exponent d φ is much larger than current theoretical limits for impurity electronic states. This suggests that the two problems are different.

Journal of the Physical Society of Japan•Jun 15, 1989•24 citations
We discuss the localization of electronic eigenfunctions and vibrational excitations (``fractons'') on self-similar percolation clusters at criticality on the Cayley tree, in d=2d=2d=2, and in d=3d=3d=3, both in topological (l)(\mathcal{l})(l) and in Euclidian (r)(r)(r) space. We find that the localization behavior of electrons and fractons is very similar, but does depend on the type of average performed and on the number of configurations NNN taken into account. It can be characterized by three different localization regimes. In the first regime, at small distances l\mathcal{l}l and rrr from the localization center, electrons and fractons are superlocalized in l\mathcal{l}l space, while the localization is not exponential in rrr space. In the intermediate regime, which is the most important one, we find stretched exponential localization (``sublocalization''), $\mathrm{ln}〈\ensuremath{\psi}〉\ensuremath{\sim}\ensuremath{-}{\mathcal{l}}^{{d}_{\ensuremath{\Psi},\mathcal{l}}}$ or $\ensuremath{\sim}\ensuremath{-}{r}^{{d}_{\ensuremath{\Psi},r}}$ with effective localization exponents ${d}_{\ensuremath{\Psi},\mathcal{l}}\ensuremath{\approx}{d}_{\ensuremath{\Psi},r}\ensuremath{\approx}0.6$. In the third regime, for large l\mathcal{l}l and rrr, the averages strongly depend on the number of configurations, even in l\mathcal{l}l space, and superlocalization ${(d}_{\ensuremath{\Psi},\mathcal{l}}{,d}_{\ensuremath{\Psi},r}>1)$ is observed, converging to simple exponential behavior asymptotically. To understand this complicated localization behavior, we present an analytical calculation of $\mathrm{ln}〈\ensuremath{\psi}〉$ for the third regime, which is based on the fact that the local amplitudes at large distances from the localization center obey a log-normal distribution.
Scaling curves for the density of states and localization length of fractons near a percolation threshold are obtained for dilute and superconducting lattices in both two and three dimensions. These are used to verify the predictions of single-parameter scaling and to show that the energy dependence of the inverse localization length is consistent with known values of the spectral dimensionalities of these structures. The results demonstrate that eigenstates of an infinite, percolating, dilute structure exhibit superlocalization of the form \ensuremath{\psi}(r)\ensuremath{\sim}${\mathit{e}}^{\mathrm{\ensuremath{-}}\mathrm{\ensuremath{\beta}}\mathit{r}\mathrm{\ensuremath{\delta}}}$ with values of \ensuremath{\delta}=1.13\ifmmode\pm\else\textpm\fi{}0.06 and 1.39\ifmmode\pm\else\textpm\fi{}0.07 in two and three dimensions, respectively.
Specific realizations due to computer experiments show that fracton excitations possess a core in which the vibrational amplitudes fall off sharply at their edges. When constructing the ensemble average of the fracton wave functions, we find ⟨ϕfr⟩∼exp⁡[−(r/Λ(ω))dϕ]\langle\phi_{\text{fr}}\rangle{\sim}\exp[-(r/\varLambda(\omega))^{d_{\phi}}]⟨ϕfr​⟩∼exp[−(r/Λ(ω))dϕ​], where Λ(ω)∼ω−0.71\varLambda(\omega){\sim}\omega^{-0.71}Λ(ω)∼ω−0.71. The exponent, -0.71, is in close agreement with the prediction of the fracton dispersion law for a two-dimensional percolating network, -0.705, and the geometrical exponent d φ is much larger than current theoretical limits for impurity electronic states. This suggests that the two problems are different.