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Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics

Electrons and fractons on percolation structures at criticality: Sublocalization and superlocalization

Jan W. Kantelhardt, Armin Bunde A

Published Dec 1, 1997• 23 citations
Publisher

Abstract

We discuss the localization of electronic eigenfunctions and vibrational excitations (``fractons'') on self-similar percolation clusters at criticality on the Cayley tree, in $d=2$, and in $d=3$, both in topological $(\mathcal{l})$ and in Euclidian $(r)$ space. We find that the localization behavior of electrons and fractons is very similar, but does depend on the type of average performed and on the number of configurations $N$ taken into account. It can be characterized by three different localization regimes. In the first regime, at small distances $\mathcal{l}$ and $r$ from the localization center, electrons and fractons are superlocalized in $\mathcal{l}$ space, while the localization is not exponential in $r$ space. In the intermediate regime, which is the most important one, we find stretched exponential localization (``sublocalization''), $\mathrm{ln}〈\ensuremath{\psi}〉\ensuremath{\sim}\ensuremath{-}{\mathcal{l}}^{{d}_{\ensuremath{\Psi},\mathcal{l}}}$ or $\ensuremath{\sim}\ensuremath{-}{r}^{{d}_{\ensuremath{\Psi},r}}$ with effective localization exponents ${d}_{\ensuremath{\Psi},\mathcal{l}}\ensuremath{\approx}{d}_{\ensuremath{\Psi},r}\ensuremath{\approx}0.6$. In the third regime, for large $\mathcal{l}$ and $r$, the averages strongly depend on the number of configurations, even in $\mathcal{l}$ space, and superlocalization ${(d}_{\ensuremath{\Psi},\mathcal{l}}{,d}_{\ensuremath{\Psi},r}>1)$ is observed, converging to simple exponential behavior asymptotically. To understand this complicated localization behavior, we present an analytical calculation of $\mathrm{ln}〈\ensuremath{\psi}〉$ for the third regime, which is based on the fact that the local amplitudes at large distances from the localization center obey a log-normal distribution.

DOI
10.1103/physreve.56.6693

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We discuss the localization of electronic eigenfunctions and vibrational excitations (fractons'') on self-similar percolation clusters at criticality on the Cayley tree, in $d=2$, and in $d=3$, both in topological $(\mathcal{l})$ and in Euclidian $(r)$ space. We find that the localization behavior of electrons and fractons is very similar, but does depend on the type of average performed and on the number of configurations $N$ taken into account. It can be characterized by three different localization regimes. In the first regime, at small distances $\mathcal{l}$ and $r$ from the localization center, electrons and fractons are superlocalized in $\mathcal{l}$ space, while the localization is not exponential in $r$ space. In the intermediate regime, which is the most important one, we find stretched exponential localization (sublocalization''), ln〈\ensuremathψ〉\ensuremath∼\ensuremath−ld\ensuremathΨ,l\mathrm{ln}〈\ensuremath{\psi}〉\ensuremath{\sim}\ensuremath{-}{\mathcal{l}}^{{d}_{\ensuremath{\Psi},\mathcal{l}}}ln〈\ensuremathψ〉\ensuremath∼\ensuremath−ld\ensuremathΨ,l​ or \ensuremath∼\ensuremath−rd\ensuremathΨ,r\ensuremath{\sim}\ensuremath{-}{r}^{{d}_{\ensuremath{\Psi},r}}\ensuremath∼\ensuremath−rd\ensuremathΨ,r​ with effective localization exponents d\ensuremathΨ,l\ensuremath≈d\ensuremathΨ,r\ensuremath≈0.6{d}_{\ensuremath{\Psi},\mathcal{l}}\ensuremath{\approx}{d}_{\ensuremath{\Psi},r}\ensuremath{\approx}0.6d\ensuremathΨ,l​\ensuremath≈d\ensuremathΨ,r​\ensuremath≈0.6. In the third regime, for large l\mathcal{l}l and rrr, the averages strongly depend on the number of configurations, even in l\mathcal{l}l space, and superlocalization (d\ensuremathΨ,l,d\ensuremathΨ,r>1){(d}_{\ensuremath{\Psi},\mathcal{l}}{,d}_{\ensuremath{\Psi},r}>1)(d\ensuremathΨ,l​,d\ensuremathΨ,r​>1) is observed, converging to simple exponential behavior asymptotically. To understand this complicated localization behavior, we present an analytical calculation of ln〈\ensuremathψ〉\mathrm{ln}〈\ensuremath{\psi}〉ln〈\ensuremathψ〉 for the third regime, which is based on the fact that the local amplitudes at large distances from the localization center obey a log-normal distribution.
Scaling curves for the density of states and localization length of fractons near a percolation threshold are obtained for dilute and superconducting lattices in both two and three dimensions. These are used to verify the predictions of single-parameter scaling and to show that the energy dependence of the inverse localization length is consistent with known values of the spectral dimensionalities of these structures. The results demonstrate that eigenstates of an infinite, percolating, dilute structure exhibit superlocalization of the form \ensuremath{\psi}(r)\ensuremath{\sim}${\mathit{e}}^{\mathrm{\ensuremath{-}}\mathrm{\ensuremath{\beta}}\mathit{r}\mathrm{\ensuremath{\delta}}}$ with values of \ensuremath{\delta}=1.13\ifmmode\pm\else\textpm\fi{}0.06 and 1.39\ifmmode\pm\else\textpm\fi{}0.07 in two and three dimensions, respectively.
Specific realizations due to computer experiments show that fracton excitations possess a core in which the vibrational amplitudes fall off sharply at their edges. When constructing the ensemble average of the fracton wave functions, we find ⟨ϕfr⟩∼exp⁡[−(r/Λ(ω))dϕ]\langle\phi_{\text{fr}}\rangle{\sim}\exp[-(r/\varLambda(\omega))^{d_{\phi}}]⟨ϕfr​⟩∼exp[−(r/Λ(ω))dϕ​], where Λ(ω)∼ω−0.71\varLambda(\omega){\sim}\omega^{-0.71}Λ(ω)∼ω−0.71. The exponent, -0.71, is in close agreement with the prediction of the fracton dispersion law for a two-dimensional percolating network, -0.705, and the geometrical exponent d φ is much larger than current theoretical limits for impurity electronic states. This suggests that the two problems are different.
We show that the amplitude fluctuations of fractons on a percolating cluster have well-defined multifractal properties. The multifractal spectrum turns out to be explicitly dependent on the frequency of the modes and rather stable for modes with similar frequency. The physical implications of this result are that self-similar fluctuations are an intrinsic characteristic of fractons. Therefore, smoothing or averaging procedures can be questionable in this respect. This property could also help clarify the ambiguities that are present in the definition of the correlation length. It is interesting to note that the localization of fractons is of a different nature with respect to Anderson localized wave functions because these are multifractal only at the mobility edge.
We examine the average cluster distribution as a function of lattice probability for a very small (L=6)(L=6)(L=6) lattice and determine the scaling function of three-dimensional percolation. The behavior of the second moment, calculated from the average cluster distribution of L=6L=6L=6 and L=63L=63L=63 lattices, is compared to power-law behavior predicted by the scaling function. We also examine the finite-size scaling of the critical point and the size of the largest cluster at the critical point. This analysis leads to estimates of the critical exponent $\ensuremath{\nu}$ and the ratio of critical exponents $\ensuremath{\beta}/\ensuremath{\nu}$.
The fracton dynamics of percolating Heisenberg antiferromagnets are studied in terms of a dynamic scaling argument and large-scale numerical analysis. It is shown that the spectral (or fracton) dimension for antiferromagnetic fractons, d~AF\tilde{d}_{\rm AF}d~AF​, is bounded by the relation d~AF≤1\tilde{d}_{\rm AF}\le 1d~AF​≤1. The densities of states (DOS) are calculated for very large percolating antiferromagnets at the critical concentration p c formed on d =2, 3, and 4 simple cubic lattices. It is concluded, from the calculated DOS's, that the spectral dimensions d~AF\tilde{d}_{\rm AF}d~AF​ are very close to unity for any Euclidean dimension d (≥2). We have also calculated the DOS for percolating antiferromagnets above p c in order to clarify the crossover behavior from extended magnons to fractons. In addition, the dynamical structure factor S ( q ,ω) is investigated both analytically and numerically. It is found, postulating a single-length scaling, that the asymptotic behaviors can be characterized by two exponents, the dynamical exponent z AF and a new exponent y . The numerical results for S ( q ,ω) support the validity of the single-length-scale postulate.