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Physical Review Letters

Pinning and Roughening of Domain Walls in Ising Systems Due to Random Impurities

David A. Huse, Christopher L. Henley

Published Jun 24, 1985• 766 citations
Publisher

Abstract

Randomly placed impurities that alter the local exchange couplings, but do not generate random fields or destroy the long-range order, roughen domain walls in Ising systems for dimensionality $\frac{5}{3}<d<5$. They also pin (localize) the walls in energetically favorable positions. This drastically slows down the kinetics of ordering. The pinned domain wall is a new critical phenomenon governed by a zero-temperature fixed point. For $d=2$, the critical exponents for domain-wall pinning energies and roughness as a function of length scale are estimated from numerically generated ground states.

DOI
10.1103/physrevlett.54.2708

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Randomly placed impurities that alter the local exchange couplings, but do not generate random fields or destroy the long-range order, roughen domain walls in Ising systems for dimensionality 53<d<5\frac{5}{3}<d<535​<d<5. They also pin (localize) the walls in energetically favorable positions. This drastically slows down the kinetics of ordering. The pinned domain wall is a new critical phenomenon governed by a zero-temperature fixed point. For d=2d=2d=2, the critical exponents for domain-wall pinning energies and roughness as a function of length scale are estimated from numerically generated ground states.
The nature of the zero-temperature ordering transition in the three-dimensional Gaussian random-field Ising magnet is studied numerically, aided by scaling analyses. Various numerical calculations are used to consistently infer the location of the transition to a high precision. A variety of boundary conditions are imposed on large samples to study the order of the transition and the number of states in the large volume limit. In the ferromagnetic phase, where the domain walls have fractal dimension ds=2,{d}_{s}=2,ds​=2, the scaling of the roughness of the domain walls, $w\ensuremath{\sim}{L}^{\ensuremath{\zeta}},$ is consistent with the theoretical prediction $\ensuremath{\zeta}=2/3.$ As the randomness is increased through the transition, the probability distribution of the interfacial tension of domain walls scales in a manner that is clearly consistent with a single second-order transition. At the critical point, the fractal dimensions of domain walls and the fractal dimension of the outer surface of spin clusters are investigated: there are at least two distinct physically important fractal dimensions that describe domain walls. These dimensions are argued to be related by scaling to combinations of the energy scaling exponent $\ensuremath{\theta},$ which determines the violation of hyperscaling, the correlation length exponent $\ensuremath{\nu},$ and the magnetization exponent $\ensuremath{\beta}.$ The value $\ensuremath{\beta}=0.017\ifmmode\pm\else\textpm\fi{}0.005$ computed from finite-size scaling of the magnetization is very nearly zero: this estimate is supported by the study of the spin cluster size distribution at criticality. The variation of configurations in the interior of a sample with boundary conditions is consistent with the hypothesis that there is a single transition separating the disordered phase with one ground state from the ordered phase with two ground states. The array of results, including values for several exponents, are shown to be consistent with a scaling picture and a geometric description of the influence of boundary conditions on the spins. The details of the algorithm used and its implementation are also described.
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A review is given on some recent developments in the theory of the Ising model in a random field. This model is a good representation of a large number of impure materials. After a short repetition of earlier arguments, which prove the absence of ferromagnetic order in d≤2d\le 2d≤2 space dimensions for uncorrelated random fields, we consider different random field correlations and in particular the generation of uncorrelated from anti-correlated random fields by thermal fluctuations. In discussing the phase transition, we consider the transition to be characterized by a divergent correlation length and compare the critical exponents obtained from various methods (real space RNG, Monte Carlo calculations, weighted mean field theory etc.). The ferromagnetic transition is believed to be preceded by a spin glass transition which manifests itself by replica symmetry breaking. In the discussion of dynamical properties, we concentrate mainly on the zero temperature depinning transition of a domain wall, which represents a critical point far from equilibrium with new scaling relations and critical exponents.
We investigate roughening transitions in the context of transverse-field Ising models. As a modification of the transverse Ising model with short range interactions, which has been shown to exhibit domain wall roughening, we have looked into the possibility of a roughening transition for the case of long-range interactions, since such a system is physically realized in the insulator LiHoF4\mathrm{Li}\mathrm{Ho}{\mathrm{F}}_{4}LiHoF4​. The combination of strong Ising anisotropy and long-range forces lead naturally to the formation of domain walls but we find that the long-range forces destroy the roughening transition.
A simple scaling description of the ordering transition in random-field Ising systems is developed and supported by renormalization-group arguments in terms of a zero-temperature critical fixed point. The main prediction is that the characteristic relaxation time \ensuremath{\tau} will diverge extremely rapidly as the critical point is approached: \ensuremath{\tau}\ensuremath{\sim}exp(${\ensuremath{\xi}}^{\mathrm{theta}}$) with \ensuremath{\xi} the correlation length and theta the ``violation of hyperscaling'' exponent (d-theta)\ensuremath{\nu}=2-\ensuremath{\alpha}. Recent experiments which exhibit onset of hysteresis in a very narrow temperature range are discussed.
An efficient Monte Carlo method is extended to evaluate directly domain-wall free energy for randomly frustrated spin systems. Using the method, critical phenomena of spin-glass phase transition are investigated in the 4d+/-J Ising model under the replica boundary condition. Our values of the critical temperature and exponent, obtained by finite-size scaling, are in good agreement with those of the standard Monte Carlo and the series expansion studies. In addition, two exponents, the stiffness exponent and the fractal dimension of the domain wall, which characterize the ordered phase, are obtained. The latter value is larger than d-1, indicating that the domain wall is really rough in the 4d Ising spin-glass phase.