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Physical Review A

Limits of superradiance as a process for achieving short pulses of high energy

J. C. MacGillivray, Michael S. Feld

Published Mar 1, 1981• 64 citations
Publisher

Abstract

This paper augments previous theoretical descriptions of superradiance in an extended optically thick medium by giving expressions which limit the length and density of a high-gain system which can superradiate as a whole, or equivalently, the shortness of its output radiation pulses. Limits arising from experimental conditions such as finite inversion time, finite decay and dephasing times, finite transit time (cooperation length), feedback, diffraction, and Fresnel number not approximately one, are discussed. Modifications to the simple analytical expressions for the output radiation of the superradiant system due to each of these effects are described in detail. Detailed computer results are also given.

DOI
10.1103/physreva.23.1334

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Physical Review A•Sep 1, 1988•81 citations
This paper augments previous theoretical descriptions of superradiance in an extended optically thick medium by giving expressions which limit the length and density of a high-gain system which can superradiate as a whole, or equivalently, the shortness of its output radiation pulses. Limits arising from experimental conditions such as finite inversion time, finite decay and dephasing times, finite transit time (cooperation length), feedback, diffraction, and Fresnel number not approximately one, are discussed. Modifications to the simple analytical expressions for the output radiation of the superradiant system due to each of these effects are described in detail. Detailed computer results are also given.
This paper presents a semiclassical treatment of the evolution of an initially inverted system into a superradiant state in an extended, optically thick medium. In this process spontaneous emission and background thermal radiation initiate the collective radiative decay and produce a superradiant output pulse of intensity proportional to the square of the number of radiators. The treatment is based on the coupled Maxwell-Schr\"odinger equations, modified to include a fluctuating polarization source properly constructed to account for the effects of spontaneous emission. Computer results show that for a high-gain system only two parameters significantly influence the evolution process: TR{T}_{R}TR​, the characteristic radiation damping time of the collective system; and ${\ensuremath{\theta}}_{0}$, a function of the conditions which initiate the superradiant process. In this limit one obtains a normalized emission curve and simple analytical expressions for the time delay, pulse width, and peak intensity of the output radiation. These results are in good agreement with experiments. A comparison of our model with previous treatments of superradiance is given.
It is argued that superradiant processes are those in which the radiative response of an atom to an excitation is appreciably influenced by interactions with its neighbors, rather than processes in which the output intensity is proportional to the square of the number NNN of atoms. On the basis of this criterion, optical free induction is a limiting response of an inhomogeneously broadened system in which cooperative effects become very small, but in which there is a strict N2{N}^{2}N2 dependence. In such a system, superradiance is manifest by a departure of the output from an N2{N}^{2}N2 dependence. Expressions are derived for the free induction response of an atomic system to an arbitrary excitation pulse, and are reduced to simple analytic forms in certain special cases. The free induction and superradiant responses are compared under conditions in which the inhomogeneous lifetime is shorter than the superradiance time $\frac{1}{N\ensuremath{\beta}}$, and an error in a previously published curve is corrected.
A theoretical model for the propagation of coherent light pulses in resonant media where a large number of atoms cooperate in spontaneous emission (superradiance) is discussed. The medium is supposedly free of inhomogeneous broadening, and no lossy relaxation mechanisms are taken into account. The conditions for the emission of all spontaneous radiation in the direction of pulse propagation are described. A semi-classical model is used and, at each point in the medium, the propagation field and the spontaneous damping field are considered separately. The equation governing the evolution of a superradiant system in the presence of an applied pulse is derived. A mechanism of energy transfer from the traveling pulse to the medium is described which includes superradiant spontaneous emission effects. As a result of the neglect of all lossy relaxation processes, all energy stored in the medium is eventually returned to the pulse by coherent spontaneous emission. Therefore, in this theory, all pulses travel through the medium without energy loss. Numerical results for square input pulses are discussed which show two possible types of propagation behavior: (a) Low input intensities produce a negative tail to the input (positive) pulse and sharpening of the tail with the advance in the medium; (b) higher input intensities produce, after sufficient penetration, a steady-state pulse envelope somewhat similar to the $2\ensuremath{\pi}$ pulses of self-induced transparency. The steady-state solutions of the equations of motion are found numerically and the pulse shapes are computed for different degrees of superradiance. In the limit of strong superradiance, very asymmetric pulse envelopes of large area are found. For negligible superradiance, approximately $2\ensuremath{\pi}$ hyperbolic-secant pulses are obtained. The effects of inhomogeneous broadening are briefly considered, and the consequences of important superradiant damping in photon-echo experiments are qualitatively discussed.
In order to study the cooperative emission of radiation from an extended system of NNN two-level atoms, we use the master-equation approach within the Born and Markov approximations. All the properties of the emission of radiation can be deduced from the diagonalization of the coupling matrix $\ensuremath{\Gamma}$, where an element ${\ensuremath{\Gamma}}_{\mathrm{jk}}$ gives the coupling between the atoms labeled jjj and kkk via the electromagnetic field. We choose a pencil-shaped volume and study analytically the coupling matrix in the limit for small and large Fresnel numbers. For Fresnel numbers of order unity numerical methods are used. Thus we prove that, for the pencil-shaped geometry, any elaborated model must take into account the interaction of the atoms with the infinity of electromagnetic field modes lying inside two small solid angles about the axis of the largest linear dimension, which we label the zzz axis. In other words, the intensity of radiation emitted by any atom of the system depends on its position with respect to the others and this "propagation effect" cannot be neglected when interpreting superradiance experiments. For small Fresnel numbers the zzz dependence predominates, in the opposite case the (x,yx, yx,y) dependence does, while for Fresnel numbers of order unity the dependence of all three components must be taken into account. Preliminary calculations are given for which only the zzz dependence is considered; for Fresnel numbers of magnitude of order unity or smaller, the effect of propagation along the zzz axis displays large delays for the appearance of superradiance with respect to the time at which the superradiant pulse is maximum when the "propagation effects" are neglected (one-mode model).
The steady-state behavior of amplifiers in which the excitation is swept at the speed of light is discussed in the semiclassical approximation. In the present work we examine the case where the decay time of the population is comparable to that of the polarization. Pulse propagation is shown to obey a generalized sine-Gordon equation which contains the effects of atomic relaxations. The analytical expression of the steady-state pulses (SSP) gives two threshold conditions. In the region of limited gain the SSP is a broad pulse with small area which can be obtained by small signal theory. In the second region of high gain the SSP is the superradiant $\ensuremath{\pi}$ pulse. Its pulse power is not limited as in usual superradiant theory because, as we show, for a swept excitation the cooperation-length limit does not exist.
The reflection of short optical pulses from the boundary of a resonant medium is investigated theoretically by the coupled system of the Maxwell and optical Bloch equations. In order to describe the reflected wave, the slowly-varying-envelope approximation in space is not exploited. The coherent reflection is shown to be in connection with Dicke superradiance. It takes place if the relaxation time of the polarization is longer than the superradiation time of the atoms in an optically thin boundary layer of the medium. That is why much of the relevant information can be obtained already in the thin-medium limit, which is considered separately. The conditions of strong reflection from an extended medium are similar to the ones found for a thin sample. The transition into the incoherent and stationary regime is discussed.