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Soviet Journal of Quantum Electronics

Investigation of the amplification of ultrashort light pulses in three-level resonant systems

Leonid A Bol'shov, Nickolai N. Elkin, T. K. Kirichenko, Vladimir V. Likhanskii, Anatolii P. Napartovich

Published Jul 31, 1982• 5 citations
Publisher

Abstract

An analysis is made of simultaneous propagation of pulses of different frequencies in many-level resonantly amplifying and absorbing media. Analytic expressions are obtained for the envelopes of fields in the case of propagation of two-frequency radiation in a three-level medium with a common lower level. Self-similar equations are obtained for the radiation propagating in an amplifying medium; in certain special cases, these equations are identical with those considered earlier.

DOI
10.1070/qe1982v012n07abeh005705

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An analysis is made of simultaneous propagation of pulses of different frequencies in many-level resonantly amplifying and absorbing media. Analytic expressions are obtained for the envelopes of fields in the case of propagation of two-frequency radiation in a three-level medium with a common lower level. Self-similar equations are obtained for the radiation propagating in an amplifying medium; in certain special cases, these equations are identical with those considered earlier.
The results are given of a theoretical investigation of the interaction between two ultrashort pulses J1 and J2 of frequencies ω31 and ω21 with a three-level amplifying medium. It is assumed that the signal J1 of frequency ω31 is a steady-state π pulse and the signal J2 is weak so that its influence on the level populations can be ignored. The case when the signal J2 has a steady-state amplitude profile and an exponential gain is considered. The analysis is made ignoring the group delay effects and also allowing for the mismatch of the group velocities of the signals. The results obtained can be used in studies of the amplification of ultrashort pulses in molecular media such as organic dyes or CO2 molecules.
Propagation and amplification of an ultrashort laser pulse in a two-level medium is numerically investigated with the use of the finite-difference time-domain (FDTD) procedure simultaneously solving Maxwell and Schrodinger equations with no assumptions characteristic of slowly varying envelope approximation. Comparison of the results of FDTD numerical simulations with the predictions of the pulse area theorem has demonstrated that the developed numerical procedure provides an adequate description of pulse evolution in a two-level medium. Amplification of ultrashort light pulses in a two-level medium is analyzed. Two methods of improving the gain of ultrashort pulses in a two-level medium by modulating the spatial distribution of dipole moments of resonant transitions and using initially chirped frequency-detuned pulses are explored.
The Maxwell–Schrödinger equations describing the ultrashort laser pulse propagation in multilevel molecular media are shown to be analytically solvable and to reduce to nonlinear multisine-Gordon equations for certain models of the field–molecule system. Special cases of level schemes are shown to lead to soliton propagation. A numerical study is presented in order to examine the effect of nonresonant (virtual) transitions on pulse propagation and amplification in a three-level molecular system as a function of intensity and detuning.
A review is given of recent theoretical investigations on coherent propagation and nonlinear interaction of multifrequency ultrashort radiation pulses in resonantly absorbing media. An analysis is made of frequency conversion by parametric interaction and stimulated Raman scattering of laser pulses in resonant three-level media. New ways of controlling the parameters of coherent pulses and the use of multifrequency pulses in the spectroscopy of multilevel media are discussed. The experimental capabilities of the investigated effects are considered.
A study is made of the resonant interaction of monochromatic radiation with many-level weakly nonequidistant systems and also of the interaction of ultrashort radiation pulses with systems of the same kind when the carrier frequency of the pulses is near a resonance frequency. In both cases, equations are obtained that describe the interaction of the radiation with the many-level systems. Analytic solutions of the problem are obtained for a three-level equidistant system under certain additional assumptions. A way of reducing the problem to a set of homogeneous algebraic equations is indicated for the case of monochromatic radiation.