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Physical review. B, Condensed matter

Dimer stability region in a frustrated quantum Heisenberg antiferromagnet

Andrey V. Chubukov, Th. Jolicœur

Published Dec 1, 1991• 70 citations
Publisher

Abstract

We study the stability region for the columnar dimer state proposed as a candidate ground state for the square-lattice quantum antiferromagnet with first- and second-neighbor antiferromagnetic couplings (${\mathit{J}}_{1}$-${\mathit{J}}_{2}$ model). We use a boson representation of the spin operators suited to the perturbative expansion around a dimer ground state. At lowest order, the columnar dimer is found to be stable only at the classical critical value ${\mathit{J}}_{2}$/${\mathit{J}}_{2}$=1/2. However, we show that the leading anharmonic corrections stabilize the dimerized phase in a region of a finite width around ${\mathit{J}}_{2}$/${\mathit{J}}_{1}$=1/2. A comparison of the ground-state energies shows that among the possible dimerized states the columnar dimer is the most favorable candidate to separate the two ordered states in the S=1/2 antiferromagnetic with first- and second-neighbor exchange.

DOI
10.1103/physrevb.44.12050

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Spin-1/2 frustrated antiferromagnet on a spatially anisotopic square lattice: contribution of exact diagonalizations

Philippe Sindzingre

The phase diagram of a spin-1/2 $J-J'-J_2$ model is investigated by means of exact diagonalizations on finite samples. This model is a generalization of the $J_1-J_2$ model on the square lattice with two different nearest-neighbor couplings $J,J'$ and may be also viewed as an array of coupled Heisenberg chains. The results suggest that the resonnating valence bond state predicted by Nersesyan and Tsvelik [Phys. Rev. B {\bf 67}, 024422 (2003)] for $J_2=0.5J' \ll J$ is realized and extends beyond the limit of small interchain coupling along a curve nearly coincident with the line where the energy per spin is maximum. This line is likely bordered on both side by a columnar dimer long range order. This columnar order could extends for $J'\to J$ which correspond to the $J_1-J_2$ model.

•Jan 1, 2004•0 citations
We study the stability region for the columnar dimer state proposed as a candidate ground state for the square-lattice quantum antiferromagnet with first- and second-neighbor antiferromagnetic couplings (J1{\mathit{J}}_{1}J1​-J2{\mathit{J}}_{2}J2​ model). We use a boson representation of the spin operators suited to the perturbative expansion around a dimer ground state. At lowest order, the columnar dimer is found to be stable only at the classical critical value J2{\mathit{J}}_{2}J2​/J2{\mathit{J}}_{2}J2​=1/2. However, we show that the leading anharmonic corrections stabilize the dimerized phase in a region of a finite width around J2{\mathit{J}}_{2}J2​/J1{\mathit{J}}_{1}J1​=1/2. A comparison of the ground-state energies shows that among the possible dimerized states the columnar dimer is the most favorable candidate to separate the two ordered states in the S=1/2 antiferromagnetic with first- and second-neighbor exchange.
An antiferromagnetic spin S=1/2 model, the J1{\mathit{J}}_{1}J1​-J2{\mathit{J}}_{2}J2​-J3{\mathit{J}}_{3}J3​-J4{\mathit{J}}_{4}J4​-J5{\mathit{J}}_{5}J5​ model, is considered in two dimensions. J1{\mathit{J}}_{1}J1​,J2{\mathit{J}}_{2}J2​,J3{\mathit{J}}_{3}J3​,J4{\mathit{J}}_{4}J4​,J5{\mathit{J}}_{5}J5​ are the strengths of the nearest-neighbor, diagonal, next-nearest-neighbor, knight's-move-distance-away, and further-neighbor-diagonal interactions, respectively. It is known that when J1{\mathit{J}}_{1}J1​:J2{\mathit{J}}_{2}J2​:J3{\mathit{J}}_{3}J3​:J4{\mathit{J}}_{4}J4​:J5{\mathit{J}}_{5}J5​=1:1:1/2:1/2:1/4 the four columnar dimer states are the exact eigenstates. In a bosonic mean-field theory, we find that the columnar dimer state is the ground state. We compare the results obtained with those obtained in the same mean-field theory for the one-dimensional Majumdar-Ghosh (MG) model. For special values of the couplings, the dimer state is known to be the exact ground state of the MG model. The comparison of the mean-field results for both the models leads to the conjecture that the columnar dimer states are the exact ground states of the J1{\mathit{J}}_{1}J1​-J2{\mathit{J}}_{2}J2​-J3{\mathit{J}}_{3}J3​-J4{\mathit{J}}_{4}J4​-J5{\mathit{J}}_{5}J5​ model.
Aiming to describe frustrated quantum magnets with nonmagnetic singlet ground states, we have extended the Rokhsar-Kivelson (RK) loop expansion to derive a generalized quantum dimer model containing only connected terms up to arbitrary order. For the square-lattice frustrated Heisenberg antiferromagnet (${J}_{1}\text{\ensuremath{-}}{J}_{2}\text{\ensuremath{-}}{J}_{3}$ model), an expansion up to eighth order shows that the leading correction to the original RK model comes from dimer moves on length-6 loops. This model free of the original sign problem is treated by advanced numerical techniques. The results suggest that a rotationally anisotropic plaquette phase [A. Ralko, D. Poilblanc, and R. Moessner, Phys. Rev. Lett. 100, 037201 (2008)] is the ground state of the Heisenberg model in the parameter region of maximum frustration.
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We study the S=1S=1S=1 square lattice Heisenberg antiferromagnet with spatially anisotropic nearest-neighbor couplings J1x{J}_{1x}J1x​ and J1y{J}_{1y}J1y​ frustrated by a next-nearest-neighbor coupling J2{J}_{2}J2​ numerically using the density-matrix renormalization-group (DMRG) method and analytically employing the Schwinger-Boson mean-field theory (SBMFT). Up to relatively strong values of the anisotropy, within both methods we find quantum fluctuations to stabilize the N\'eel-ordered state above the classically stable region. Whereas SBMFT suggests a fluctuation-induced first-order transition between the N\'eel state and a stripe antiferromagnet for $1/3\ensuremath{\le}{J}_{1x}/{J}_{1y}\ensuremath{\le}1$ and an intermediate paramagnetic region opening only for very strong anisotropy, the DMRG results clearly demonstrate that the two magnetically ordered phases are separated by a quantum-disordered region for all values of the anisotropy with the remarkable implication that the quantum paramagnetic phase of the spatially isotropic ${J}_{1}\text{\ensuremath{-}}{J}_{2}$ model is continuously connected to the limit of decoupled Haldane spin chains. Our findings indicate that for S=1S=1S=1 quantum fluctuations in strongly frustrated antiferromagnets are crucial and not correctly treated on the semiclassical level.
We construct and study the two frustrated quantum spin-1∕21∕21∕2 models on square lattice, which are like the antiferromagnetic ${J}_{1}\text{\ensuremath{-}}{J}_{2}$ model with some additional four-spin exchange interactions. These models admit an exactly solvable case in which the ground state consists of four degenerate columnar-dimer singlet (CDS) configurations. Away from the exact case, we employ bond-operator mean-field theory to investigate the evolution of the ground state by varying the interaction parameters. The mean-field calculation reveals a quantum phase diagram in which the CDS phase undergoes a continuous phase transition to either N\'eel or collinear ordered antiferromagnetic phases.
The phase diagram of a spin-1/2 J−J′−J2J-J'-J_2J−J′−J2​ model is investigated by means of exact diagonalizations on finite samples. This model is a generalization of the J1−J2J_1-J_2J1​−J2​ model on the square lattice with two different nearest-neighbor couplings J,J′J,J'J,J′ and may be also viewed as an array of coupled Heisenberg chains. The results suggest that the resonnating valence bond state predicted by Nersesyan and Tsvelik [Phys. Rev. B {\bf 67}, 024422 (2003)] for J2=0.5J′≪JJ_2=0.5J' \ll JJ2​=0.5J′≪J is realized and extends beyond the limit of small interchain coupling along a curve nearly coincident with the line where the energy per spin is maximum. This line is likely bordered on both side by a columnar dimer long range order. This columnar order could extends for J′→JJ'\to JJ′→J which correspond to the J1−J2J_1-J_2J1​−J2​ model.