We study the competition between antiferromagnetic order and valence-bond-crystal formation in a two-dimensional frustrated spin-
1∕2 model. The ${J}_{1}\text{\ensuremath{-}}{J}_{2}$ model on the square lattice is further frustrated by introducing products of three-spin projectors which stabilize four dimer-product states as degenerate ground state. These four states are reminiscent of the dimerized singlet ground state of the Shastry-Sutherland model. Using exact diagonalization, we study the evolution of the ground state by varying the ratio of interactions. For a large range of parameters $({J}_{2}\ensuremath{\gtrsim}0.25{J}_{1})$, our model shows a direct transition between the valence-bond-crystal phase and the collinear antiferromagnetic phase. For small values of
J2, several intermediate phases appear which are also analyzed.
We study a spin-half frustrated coupled ladder system, in which ladders with leg, rung, and diagonal interactions are linked via nearest-neighbor coupling. By introducing a leg-symmetric inter-ladder interaction that connects the left-to-left and right-to-right legs of adjacent ladders, the model is found to possess an exact dimer ground state, characterized by a product of two-spin singlets forming a columnar dimer phase. We analyze this model using bond-operator mean-field theory (BOMFT) and the density matrix renormalization group (DMRG) to probe the phase transitions that occur as one traverses the coupling space. The BOMFT reveals three distinct phases: a double-stripe ordered phase, a Néel ordered phase, and a quantum disordered dimerized phase. The critical points for the transitions are at $ J_1 = -0.81 $ (double-stripe to dimerized) and at $ J_1 = 2.81 $ (dimerized to Néel phase). Further, the DMRG results corroborate the exact ground state and refine the critical points to $ J_1 = -0.79 $ and $ J_1 = 2.29 $ for the respective transitions. Additionally, another transition is identified as the Néel order vanishes for $ J_1 \ge 4.5 $. The model can alternatively be represented as a network of orthogonal zigzag and fully frustrated spin ladders, offering a structural framework conducive to quantum materials engineering.
An antiferromagnetic spin S=1/2 model, the
J1-
J2-
J3-
J4-
J5 model, is considered in two dimensions.
J1,
J2,
J3,
J4,
J5 are the strengths of the nearest-neighbor, diagonal, next-nearest-neighbor, knight's-move-distance-away, and further-neighbor-diagonal interactions, respectively. It is known that when
J1:
J2:
J3:
J4:
J5=1:1:1/2:1/2:1/4 the four columnar dimer states are the exact eigenstates. In a bosonic mean-field theory, we find that the columnar dimer state is the ground state. We compare the results obtained with those obtained in the same mean-field theory for the one-dimensional Majumdar-Ghosh (MG) model. For special values of the couplings, the dimer state is known to be the exact ground state of the MG model. The comparison of the mean-field results for both the models leads to the conjecture that the columnar dimer states are the exact ground states of the
J1-
J2-
J3-
J4-
J5 model.
In a recent work [Phys. Rev. B {\bf 77}, 014419 (2008)], a quantum spin-1/2 model having an exact fourfold degenerate Shastry-Sutherland ground state was constructed, and studied using finite-size numerical exact diagonalization. There, a schematic quantum phase diagram suggesting many competing phases was also proposed. In the present work, an extended version of this model is investigated using dimer and plaquette triplon mean-field theories. The quantum phase diagram of the extended model (in the thermodynamic limit) is found to have many interesting phases: commensurate and incommensurate magnetically ordered phases, and columnar dimer, sublattice columnar dimer, Shastry-Sutherland and plaquette spin-gapped phases. Among themselves, these phases undergo a continuous or a level-crossing transition.
The mean-field triplon analysis is developed for spin-
S quantum antiferromagnets with dimerized ground states. For the spin-1/2 case, it reduces to the well-known bond-operator mean-field theory. It is applied to a columnar dimer model on square lattice and to a model on honeycomb lattice with spontaneous dimerization in the ground state. Different phases in the ground state are investigated as a function of spin. It is found that under suitable conditions (such as strong frustration), a quantum ground state (dimerized singlet phase in the present study) can survive even in the limit $S\ensuremath{\rightarrow}\ensuremath{\infty}$. Two quick extensions of this representation are also presented. In one case, it is extended to include the quintet states. In another, a similar representation is worked out on a square plaquette. A convenient procedure for evaluating the total-spin eigenstates for a pair of quantum spins is presented in the appendix.
Using the coupled-cluster method for high orders of approximation and Lanczos exact diagonalization we study the ground-state phase diagram of a quantum spin-
21 J1-
J2 model on the square lattice with plaquette structure. We consider antiferromagnetic (
J1>0) as well as ferromagnetic (
J1<0) nearest-neighbor interactions together with frustrating antiferromagnetic next-nearest-neighbor interaction
J2>0. The strength of interplaquette interaction $\ensuremath{\lambda}$ varies between $\ensuremath{\lambda}=1$ (which corresponds to the uniform
J1-
J2 model) and $\ensuremath{\lambda}=0$ (which corresponds to isolated frustrated 4-spin plaquettes). While on the classical level ($s\ensuremath{\rightarrow}\ensuremath{\infty}$) both versions of models (i.e., with ferro- and antiferromagnetic
J1) exhibit the same ground-state behavior, the ground-state phase diagram differs basically for the quantum case
s=1/2. For the antiferromagnetic case (
J1>0) N\'eel antiferromagnetic long-range order at small
J2/J1 and $\ensuremath{\lambda}\ensuremath{\gtrsim}0.47$ as well as collinear striped antiferromagnetic long-range order at large
J2/J1 and $\ensuremath{\lambda}\ensuremath{\gtrsim}0.30$ appear which correspond to their classical counterparts. Both semiclassical magnetic phases are separated by a nonmagnetic quantum paramagnetic phase. The parameter region, where this nonmagnetic phase exists, increases with decreasing $\ensuremath{\lambda}$. For the ferromagnetic case (
J1<0) we have the trivial ferromagnetic ground state at small
J2/∣J1∣. By increasing
J2 this classical phase gives way for a semiclassical plaquette phase, where the plaquette block spins of length
s=2 are antiferromagnetically long-range ordered. Further increasing of
J2 then yields collinear striped antiferromagnetic long-range order for $\ensuremath{\lambda}\ensuremath{\gtrsim}0.38$, but a nonmagnetic quantum paramagnetic phase $\ensuremath{\lambda}\ensuremath{\lesssim}0.38$.