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Journal of the Optical Society of America

Electric-Field and Multiple-Foil Excitation Experiments on Beam-Foil-Excited Hydrogen Atoms*

William S. Bickel

Published Feb 1, 1968• 32 citations
Publisher

Abstract

Four experiments involving individual and combined effects of electric fields and multiple exciter foils on beam-foil-excited hydrogen atoms are described.The use of multiple exciter foils shows that excitation equilibrium does not occur in the thin carbon foils used here. The change of the rate of decay of Ly-α flux emitted by beam-foil excited hydrogen atoms in an electric field has been used to determine the relative populations of the 2s and 2p levels at the foil. The 2s level is overpopulated with respect to the 2p level when one foil is used and two exciter foils enhance the overpopulations. Photoelectric measurements of Ly-α flux and photographic measurements of the decay of Balmer-δ flux emitted by atoms in an electric field show that quasiperiodic intensity variations exist on the decay curve. The variations are attributed to the effect of the electric field but discrepancies arise between the experimental frequencies and those calculated from Stark-effect theory.

DOI
10.1364/josa.58.000213

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Physical Review Letters•Feb 11, 1974•69 citations
Four experiments involving individual and combined effects of electric fields and multiple exciter foils on beam-foil-excited hydrogen atoms are described.The use of multiple exciter foils shows that excitation equilibrium does not occur in the thin carbon foils used here. The change of the rate of decay of Ly-α flux emitted by beam-foil excited hydrogen atoms in an electric field has been used to determine the relative populations of the 2s and 2p levels at the foil. The 2s level is overpopulated with respect to the 2p level when one foil is used and two exciter foils enhance the overpopulations. Photoelectric measurements of Ly-α flux and photographic measurements of the decay of Balmer-δ flux emitted by atoms in an electric field show that quasiperiodic intensity variations exist on the decay curve. The variations are attributed to the effect of the electric field but discrepancies arise between the experimental frequencies and those calculated from Stark-effect theory.
Protons with velocities ranging from 3.2 \ifmmode\times\else\texttimes\fi{} 108{10}^{8}108 to 6.3 \ifmmode\times\else\texttimes\fi{} 108{10}^{8}108 cm/sec were passed through a carbon foil producing excited hydrogen atoms which decayed in flight after emergence. With the foil in magnetic fields from 2 to 25 G, the lines ${\mathrm{H}}_{\ensuremath{\alpha}}$ through ${\mathrm{H}}_{\ensuremath{\epsilon}}$ showed periodic intensity fluctuations due to Stark mixings of fine-structure levels caused by motional electric fields (6-158 V/cm). An extension of the Bethe-Lamb theory of Stark quenching provides good agreement between a small number of theoretically dominant frequencies and the measured fluctuation frequencies. Apparent discrepancies between theory and experiment noted by other experimenters are shown to be removed by our calculations except in one measurement on ${\mathrm{Ly}}_{\ensuremath{\alpha}}$. The necessity of using double foils postulated in the previous work is discussed. Our analysis suggests the preferential alignment of the final-state angular momenta perpendicular to the beam direction. Reasons for this alignment are given.
Passage of a beam of foil-excited He+{\mathrm{He}}^{+}He+ ions through a small electric field induced quasiperiodic fluctuations in the intensity of the light emitted from levels n=7,8,9,and10n=7, 8, 9, \mathrm{and} 10n=7,8,9,and10. Both He3{\mathrm{He}}^{3}He3 and He4{\mathrm{He}}^{4}He4 beams were used. Only one foil was needed, in contrast to the double-foil arrangement reported necessary for hydrogen. The observations are discussed in terms of Stark-induced interference of the fine-structure levels of He ii, but discrepancies between the data and the calculations are large.
Hydrogen atoms are excited into high Rydberg states following fast proton impact on a thin carbon foil. The effects of various electromagnetic fields on these atoms are observed by measuring the integral ionization yield in an additional constant electric field. These experiments reveal oscillations in that yield, regularly spaced as a function of electric field. A model is outlined that quantitatively describes the observed field dependence. This new phenomenon indicates selective excitation of the Stark substates.
Intensity beats in the emission of $\mathrm{L}{\mathrm{y}}_{\ensuremath{\alpha}}$ from beam-foil excited hydrogen in various static electromagnetic field configurations have been studied. The observed beat frequencies agree with the calculated values, which are independent of the field directions. The beat amplitudes, however, show significant dependence on the field directions relative to the beam. The theory for emission of light from the decay of coherently excited states is applied in the sudden perturbation limit. Agreement with experiment can only be obtained under the assumption that the foil excitation generates initial coherent wave functions ${\ensuremath{\Psi}}_{\mathrm{I},\mathrm{I}\mathrm{I}}=\ensuremath{\alpha}|p,\frac{1}{2},\ifmmode\pm\else\textpm\fi{}\frac{1}{2}〉+\ensuremath{\beta}|s,\frac{1}{2},\ensuremath{\mp}\frac{1}{2}〉$, where ∣l,j,mj〉|l,j,{m}_{j}〉∣l,j,mj​〉 notation and the beam as quantization axis are used. The ratio $\frac{\ensuremath{\alpha}}{\ensuremath{\beta}}$ is then determined, which gives the ratio of the excitation cross section of the ppp to that of the sss states as $\frac{{\ensuremath{\sigma}}_{p}}{{\ensuremath{\sigma}}_{s}}>~4\ifmmode\pm\else\textpm\fi{}1$ at a beam energy of 200 (keV) per atom.
A beam–foil experiment is proposed for observation of a phase shift π in a beat intensity of light emitted by hydrogen and antihydrogen atoms in an external electric field. This effect is based on the existence of the terms linear in the electric field in the expression for the radiation probability of an atom. The linear terms have an opposite sign for hydrogen and antihydrogen atoms and lead to such a difference in a beat signal. Experimental conditions for observation of this effect are discussed.
The intensity of beam-foil-excited $\mathrm{Ly}\ensuremath{-}\ensuremath{\alpha}$ radiation has been measured in electric fields alternately parallel and antiparallel to the beam. Measurements were made at three energies---110, 165, and 210 keV---and three field strengths. From these data the $S\ensuremath{-}P$ co-herence term ${\ensuremath{\sigma}}_{\mathrm{SP}}$ has been determined. The magnitude of ${\ensuremath{\sigma}}_{\mathrm{SP}}$ is found to be 0.07 at 110 keV, 0.19 at 160 keV, and 0.22 at 210 keV. These results establish that beam-foil-excited hydrogen atoms have a nonzero electric dipole moment.