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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

Spin-3 dynamics study in a chromium Bose-Einstein Condensate

O. Gorceix, Benjamin Pasquiou, G. Bismut, É. Maréchal, P. Pedri, L. Vernac, B. Laburthe-Tolra

Published May 1, 2011• 0 citations
Publisher

Abstract

Dipole-dipole interactions are long-ranged and anisotropic. They induce a coupling between spin and angular momentum degrees of freedom yielding new interesting physics in the field of dilute quantum gases. We have thoroughly studied dipolar relaxation DR processes in a chromium BEC transferred into an excited magnetic m = +3 sublevel and loaded in 1D and 2D optical lattices. We demonstrate and quantify how the confinement of a quantum gas in optical lattices deeply modifies the DR processes. In particular, we show that DR is strongly inhibited at low magnetic fields when the released energy becomes smaller than the vibrational quantum of energy at the bottom of the lattice wells. We show that interband transitions are induced above the corresponding threshold and that metastability of the "excited state BEC" is reached below the 2D threshold.

DOI
10.1109/cleoe.2011.5943291

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Dipole-dipole interactions are long-ranged and anisotropic. They induce a coupling between spin and angular momentum degrees of freedom yielding new interesting physics in the field of dilute quantum gases. We have thoroughly studied dipolar relaxation DR processes in a chromium BEC transferred into an excited magnetic m = +3 sublevel and loaded in 1D and 2D optical lattices. We demonstrate and quantify how the confinement of a quantum gas in optical lattices deeply modifies the DR processes. In particular, we show that DR is strongly inhibited at low magnetic fields when the released energy becomes smaller than the vibrational quantum of energy at the bottom of the lattice wells. We show that interband transitions are induced above the corresponding threshold and that metastability of the "excited state BEC" is reached below the 2D threshold.
Magnetic dipole-dipole interactions (MDDIs) are long-ranged and anisotropic. They induce a coupling between spin and angular momentum degrees of freedom paving the way for new interesting physics in the fields of quantum gases and magnetism. This paper thoroughly studies dipolar relaxation (DR) processes in a chromium BEC. Atoms are transferred from the absolute ground state with m = -3 to the excited m = +3 Zeeman state and are loaded in a 3D optical lattice; the magnetic state distribution of this system under various conditions is monitored. In a previous publication, it was demonstrated how the confinement of a quantum gas in 1D and 2D optical lattices deeply modifies the DR processes. In particular, it was shown that DR is inhibited at low magnetic fields when the released energy becomes smaller than the vibrational quantum of energy at the bottom of the lattice wells. In the present work, instability (or decay) of the “excited state BEC” appears as a resonant process as the released energy matches band excitation. Analyzing these resonances as a function of the magnetic field orientation reveals a new manifestation of the anisotropy of MDDIs. The spectroscopy of these resonances as a function of the field intensity is found to be sensitive to the lattice site number occupancy as demonstrated by performing it after various system preparation schemes including number-squeezed Mott states. Decays from sites housing three atoms produce entangled spin and orbital states.
We observe interband transitions mediated by the dipole-dipole interaction for an array of 1D quantum gases of chromium atoms, trapped in a 2D optical lattice. Interband transitions occur when dipolar relaxation releases an energy which matches or overcomes the lattice band gap. We analyze the role of tunneling in higher lattice bands on this process. We compare the experimental dipolar relaxation rate with a calculation based on a multiple Fermi Golden Rule approach, when the lattice sites are symmetric, and the magnetic field is parallel to the lattice axis. We also show that an almost complete suppression of dipolar relaxation is obtained below a magnetic field threshold set by the depth of the lattice: 1D quantum gases in an excited Zeeman state then become metastable.
We observe interband transitions mediated by dipole-dipole interactions for an array of 1D quantum gases of chromium atoms, trapped in a 2D optical lattice. Interband transitions occur when dipolar relaxation releases an energy larger than the lattice band gap. For symmetric lattice sites, and a magnetic field parallel to the lattice axis, we compare the measured dipolar relaxation rate with a Fermi golden rule calculation. Below a magnetic field threshold, we obtain an almost complete suppression of dipolar relaxation, leading to metastable 1D gases in the highest Zeeman state.
We analyze the physics of spin-3 Bose-Einstein condensates, and, in particular, the new physics expected in ongoing experiments with condensates of chromium atoms. We first discuss the ground-state properties, which, depending on still unknown chromium parameters, and for low magnetic fields, can present various types of phases. We also discuss the spinor dynamics in chromium spinor condensates, which present significant qualitative differences when compared to other spinor condensates. In particular, dipole-induced spin relaxation may lead for low magnetic fields to transfer of spin into angular momentum similar to the well-known Einstein-de Haas effect. Additionally, a rapid large transference of population between distant magnetic states also becomes possible.
We report on experiments exploring the physics of dipolar quantum gases using a Chromium Bose-Einstein condensate (BEC). By means of a Feshbach resonance, it is possible to reduce the effects of short range interactions and reach a regime where the physics is governed by the long-range, anisotropic dipole-dipole interaction between the large (6μB6 μ_{\rm B}6μB​) magnetic moments of Chromium atoms. Several dramatic effects of the dipolar interaction are observed: the usual inversion of ellipticity of the condensate during time-of flight is inhibited, the stability of the dipolar gas depends strongly on the trap geometry, and the explosion following the collapse of an unstable dipolar condensate displays d-wave like features.
We study dipolar relaxation of a chromium BEC loaded into a 3D optical lattice. We observe dipolar relaxation resonances when the magnetic energy released during the inelastic collision matches an excitation towards higher energy bands. A spectroscopy of these resonances for two orientations of the magnetic field provides a 3D band spectroscopy of the lattice. The narrowest resonance is registered for the lowest excitation energy. Its line-shape is sensitive to the on-site interaction energy. We use such sensitivity to probe number squeezing in a Mott insulator, and we reveal the production of three-body states with entangled spin and orbital degrees of freedom.