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Physical Review A

Intrinsic optical bistability in collections of spatially distributed two-level atoms

Y. Ben-Aryeh, C. M. Bowden, John C. Englund

Published Nov 1, 1986• 156 citations
Publisher

Abstract

We use a quantum-electrodynamical, many-body treatment to show mirrorless optical bistability in terms of the spatial properties of coherent dipole-dipole interactions among interacting two-level atoms. The general theory is applied to two special cases: (1) a thin sample of two-level atoms, with a width smaller than a resonance wavelength and (2) a long sample of two-level atoms, with dimensions very large relative to a resonance wavelength. While for the thin sample we are able to use a mean-field approximation with validity, for the long sample we are compelled to take into account retardation and propagation. In both cases bistability is found to be related to a renormalization of the frequency (or relaxation rate) that is inversion dependent. For the long sample the frequency renormalization is significant for high atomic densities and for large oscillator strengths.

DOI
10.1103/physreva.34.3917

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We use a quantum-electrodynamical, many-body treatment to show mirrorless optical bistability in terms of the spatial properties of coherent dipole-dipole interactions among interacting two-level atoms. The general theory is applied to two special cases: (1) a thin sample of two-level atoms, with a width smaller than a resonance wavelength and (2) a long sample of two-level atoms, with dimensions very large relative to a resonance wavelength. While for the thin sample we are able to use a mean-field approximation with validity, for the long sample we are compelled to take into account retardation and propagation. In both cases bistability is found to be related to a renormalization of the frequency (or relaxation rate) that is inversion dependent. For the long sample the frequency renormalization is significant for high atomic densities and for large oscillator strengths.
We use a fully quantum, many-body treatment to show mirrorless optical bistability in terms of the spacial properties of interacting two-level systems. The bistability effects are related to the coherent dipole-dipole interactions which introduce an inversion-dependent renormalization of the frequency (or relaxation). Conditions of stability and instability are discussed for a thin sample of two-level atoms with a width smaller than a wavelength. For a long sample of two-level atoms, we find that the two phases of high transmissivity and low transmissivity may coexist spacially in the material.
A system of coherently driven spatially distributed two-level atoms, coupled with each other via dipole–dipole interaction, exhibits intrinsic optical bistability (IOB) at solid-state densities,1 i.e., optical bistability without optical feedback. The origin of the IOB was shown to be due to inversion-dependent renormalization of the single-atom resonance frequency caused by dipole–dipole interaction among the atoms located mainly within an atomic resonance wavelength.2 For normally incident plane waves of intensity beyond threshold, a spatially dependent discontinuity in the nonlinear refractive index was shown to exist inside the medium,1 corresponding to spatial separation of the high and low absorption phases of the IOB. We present numerical results for the time-dependent solutions of the equations of motion and dynamics of the field propagation.
We investigate the problem of resonant re flection and transmission of an ultrashort light pulse passing through a medium consisting of two-level atoms. We show that for a thin layer it is important to take into account the difference between the external macroscopic field and the field acting on the individual atoms within the medium. The local field correction leads to an inversion dependent resonant frequency. In thin layers this generates a new mechanism of nonlinear transparency induced by the dynamical frequency shift. When the excitation frequency is larger than the original resonant frequency, then the transmission of the layer exhibits bistable behavior.
Intrinsic (mirrorless) optical bistability (MOB) has been predicted independently by a number of authors1. Recent experiments have demonstrated at least one major aspect of this phenomenon, i.e., MOB due to increasing absorption2. Other categories of MOB which have been predicted from theoretical models are caused by: interatomic correlation in a many-body quantum model, the anharmonic contribution in a classical Duffing oscillator, the local field correction in the macroscopic Maxwell-Bloch formulation, and coherent dipole-dipole interaction in a microscopic semiclassical model of a finite number of damped, two-level atoms driven by an external field3. All of these models share a single common characteristic which causes MOB in some region of the parameter space of each model. The characteristic is simply: an interaction-dependent nonlinearity which causes a renormalization of the resonance frequency. In each case, the sign and magnitude of the incident field detuning from the unrenormalized resonance is a crucial parameter.
Intrinsic optical bi-stability in dense two-level systems is developed for the bad cavity limit where electromagnetic modes are adiabatically eliminated. Each atom interacts via dipole–dipole forces with its nearby spatial distribution of atoms. The theory is developed into two parts, corresponding to the short sample, with dimensions shorter than the wavelength, and the long sample. In both cases, the local field corrections modify the Maxwell–Bloch equations, so that cubic or quartic equations are obtained for the inversion of population as a function of the external light intensity, thus leading to intrinsic bi-stability. The effects of noise sources on intrinsic bi-stability were treated, and I found that while the observability of bi-stability was not obtained experimentally for a simple two-level system, there were many observations of bi-stability obtained through the ‘up-conversion’ of rare earth excited crystals. I show the differences between these two systems.