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Journal of the Optical Society of America B

Instantaneous resonance fluorescence spectrum of a two-level system for an exponential decay of the driving field

Weisi Tan, Weihan Tan, Dongsheng Zhao, Renghong Liu

Published Sep 1, 1993• 4 citations
Publisher

Abstract

We evaluate the commutation relations and quantum-mechanical Langevin equations satisfied by two-level operators in the case of exponential decay of the driving field. We rewrite the dynamical equation in the form of a difference equation by Laplace transformation. From the solution of the difference equation, the instantaneous resonance fluorescence spectrum is calculated.

DOI
10.1364/josab.10.001610

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We evaluate the commutation relations and quantum-mechanical Langevin equations satisfied by two-level operators in the case of exponential decay of the driving field. We rewrite the dynamical equation in the form of a difference equation by Laplace transformation. From the solution of the difference equation, the instantaneous resonance fluorescence spectrum is calculated.
We examine the radiative properties of a two-level atom driven by a strong bichromatic field with frequencies ${\mathrm{\ensuremath{\omega}}}_{1}$=${\mathrm{\ensuremath{\omega}}}_{0}$-${\mathrm{\ensuremath{\delta}}}_{1}$ and ${\mathrm{\ensuremath{\omega}}}_{2}$=${\mathrm{\ensuremath{\omega}}}_{0}$+${\mathrm{\ensuremath{\delta}}}_{2}$, which can be asymmetrically placed about the atomic transition frequency ${\mathrm{\ensuremath{\omega}}}_{0}$ and can have different Rabi frequencies ${\mathrm{\ensuremath{\Omega}}}_{1}$ and ${\mathrm{\ensuremath{\Omega}}}_{2}$. Applying the optical Bloch equations for the bichromatic excitation, we derive an infinite set of equations of motion for the time evolution of the atomic variables. The equations are solved numerically by matrix inversion and Laplace transforms. Using the quantum regression theorem, we then solve for the steady-state total fluorescence intensity, and the resonance-fluorescence and absorption spectra. The spectra are found to depend on the frequency difference 2\ensuremath{\delta}=${\mathrm{\ensuremath{\delta}}}_{1}$+${\mathrm{\ensuremath{\delta}}}_{2}$, the average detuning \ensuremath{\Delta}=${\mathrm{\ensuremath{\omega}}}_{0}$-1/2(${\mathrm{\ensuremath{\omega}}}_{1}$+${\mathrm{\ensuremath{\omega}}}_{2}$), and the Rabi frequencies of the driving fields. For ${\mathrm{\ensuremath{\Omega}}}_{1}$=${\mathrm{\ensuremath{\Omega}}}_{2}$=\ensuremath{\Omega}, the total fluorescent intensity displays a series of maxima for \ensuremath{\Delta}=\ifmmode\pm\else\textpm\fi{}n\ensuremath{\delta}\ensuremath{\mp}${\mathrm{\ensuremath{\Omega}}}^{2}$/4\ensuremath{\delta}, where the n are the odd integers. The intensity-dependent shift from the resonances n\ensuremath{\delta} is explained as an analog of the generalized Bloch-Siegert shift. The resonance-fluorescence spectrum for \ensuremath{\Delta}\ensuremath{\ne}0 appears to contain more peaks than that for \ensuremath{\Delta}=0.This is due to the splitting of the central peak and the even sidebands into doublets. The absorption spectrum of a weak-probe beam for \ensuremath{\Delta}=0 and equal Rabi frequencies consists of a symmetric series of dispersionlike sidebands separated from ${\mathrm{\ensuremath{\omega}}}_{0}$ by integer multiples of \ensuremath{\delta}, together with a central absorption peak at ${\mathrm{\ensuremath{\omega}}}_{0}$, whose amplitude oscillates with \ensuremath{\Omega}. For \ensuremath{\Delta}\ensuremath{\ne}0 and/or ${\mathrm{\ensuremath{\Omega}}}_{1}$\ensuremath{\ne}${\mathrm{\ensuremath{\Omega}}}_{2}$, the odd sidebands remain dispersionlike, while the central peak and the even sidebands split into absorption-emission doublets. A simple physical interpretation of the spectral features is given in terms of the dressed-atom model.
An S-conserving theory of collective resonance fluorescence by NNN two-level atoms driven by a uniform strong field is presented. The detuning between field and atoms can be varied. A canonical transformation to dress the atoms by the driving field and Langevin equations for dressed operators are used to investigate the behavior of the system. For sufficiently large detuning the dressed atoms are shown to reach a steady state after a transient super-radiant-like decay in times short, compared with the long decay time which is attained on resonance and which is the same as the single-atom spontaneous-decay time. In the transient regime the parameters of the quasi-super-radiant decay are shown to vary with detuning and with the driving-field amplitude. Both the amplitude spectrum and the integrated intensity of the fluorescence field, emitted off resonance by the dressed atoms during the transient, are shown to bear pulselike traces of the quasi-super-radiant decay. The elastic components of the off-resonance amplitude spectrum at the end of the super-radiant-like transient are broadened with respect to resonance, and the integrated intensity exhibits a sudden transient decrease in an appropriate range of detuning, which has been given the name "superdarkening" and which disappears on resonance. After the steady-state regime is attained, the resonance intensity spectrum is shown to coincide with that obtained by other authors, while off resonance the inelastic lines are broadened in a super-radiant-like fashion.
We present analytical and numerical results for the steady-state resonance fluorescence spectrum produced by a coherently driven two-level atom in the presence of a broadband squeezed vacuum. Here the central frequency of the squeezed vacuum is off-resonant with the driving field frequency, while maintaining resonance between the driving frequency and the atomic resonance. Numerical solutions of the Bloch equations of the system are obtained under the strong driving field approximation which agree well with the analytic results.
A canonical transformation, which diagonalizes the single-mode radiation Hamiltonian in the rotating wave approximation, is exploited to dress a two-level atom by the strong monochromatic driving field in the resonance fluorescence phenomenon. Langevin equations of motion are obtained for dressed atomic operators, and their solutions yield the amplitude of waves scattered into the fluorescence field. The power spectrum of the scattered field is obtained from the first-order correlation functions between dressed atomic operators. The results of the present treatment are compared with others, and advantages and disadvantages of the present method are discussed.