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Journal of Experimental and Theoretical Physics Letters

Repopulation of equidistant levels by two coherent resonant phase-shifted electromagnetic fields

Д.Ф. Зарецкий, S. B. Sazonov

Published Aug 1, 2000• 1 citation
Publisher

Abstract

A new method of atomic and nuclear orientation and polarization is suggested. The method is based on the use of two coherent resonant phase-shifted monochromatic electromagnetic waves. It is demonstrated that a profound phase-shift-dependent level repopulation can be accomplished in a pulsed mode at room temperature. The possible application of this effect to quantum computers is briefly discussed.

DOI
10.1134/1.1320105

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A new method of atomic and nuclear orientation and polarization is suggested. The method is based on the use of two coherent resonant phase-shifted monochromatic electromagnetic waves. It is demonstrated that a profound phase-shift-dependent level repopulation can be accomplished in a pulsed mode at room temperature. The possible application of this effect to quantum computers is briefly discussed.
A method is proposed for fast and deep polarization of the system of hyperfine sublevels of the ground state of an atom having an optical excited state by means of two-component microwave pulses. The pulse of the bichromatic optical field that induces the transitions between the ground state and excited state of the atom is supposed to provide coherence among the hyperfine sublevels of the atomic ground state via the effect of coherent population trapping. The subsequent resonance microwave pulses create the polarization of equally populated ground state sublevels of the atom. The proposed polarization technique may be used for designing the new schemes of quantum computers, for the pulse transformation in optical experiments when light passes through a resonant medium containing rear-earth ions, as well as for producing polarized nuclear targets.
The coherent repopulation of a quantum system consisting of three nonequidistant levels in the field of a resonant bichromatic rf wave is studied. The atoms are assumed to have an impulsive interaction with the rf wave in which the pulse duration is less than any of the relaxation times. The hyperfine structure of gas atoms and a system of atomic oscillator levels in a magnetic trap are considered as examples of such a quantum system. It is shown that in the second case, the coherent repopulation effect can be used to cool neutral atoms in magnetic traps.
A method has been proposed for rapidly and deeply changing the population in the system of unequally populated hyperfine atomic levels, including the ground-state sublevels, due to the impact of mutually coherent pulsed resonance electromagnetic fields. The method can be implemented, e.g., to create new schemes of the amplification or effective absorption of the radiation passing through a medium, to develop the new field of quantum electronics, spintronics, involving the current of polarized electrons, and to create new schemes of quantum computers.
Resonant scattering (redistribution) of weak monochromatic light by atoms in the presence of collisions has been considered by Omont et al., who allowed for the broadening of both upper and lower levels of the transition. Mollow (who also has considered this problem for intense radiation) has shown that their results are applicable only if collisional repopulation of the levels (in contrast to collisional depopulation) is ignored. We here consider in detail the effect of repopulation. It leads, in the weak-field limit, to a true-coherent component ($\ensuremath{\delta}$-function spectrum) at the driving frequency, as well as a component at this frequency whose width is essentially the inelastic collisional rate of the lower state. An additional redistributed component due to repopulation of the upper level is also obtained.
We propose and develop a method for theoretical description of circularly (elliptically) polarized optical pulse resonant coherent interactions with two-level atoms. The method is based on the time-evolution equations of a two-level quantum system in the presence of a time-dependent dipole perturbation for electric dipole transitions between states with total angular-momentum projection difference $(\ensuremath{\Delta}{J}_{z}=\ifmmode\pm\else\textpm\fi{}1)$ excited by a circularly polarized electromagnetic field [Feynman et al., J. Appl. Phys. 28, 49 (1957)]. The adopted real-vector representation approach allows for coupling with the vectorial Maxwell's equations for the optical wave propagation and thus the resulting Maxwell pseudospin equations can be numerically solved in the time domain without any approximations. The model permits a more exact study of the ultrafast coherent pulse propagation effects taking into account the vector nature of the electromagnetic field and hence the polarization state of the optical excitation. We demonstrate self-induced transparency effects and formation of polarized solitons. The model represents a qualitative extension of the well-known optical Maxwell-Bloch equations valid for linearly polarized light and a tool for studying coherent quantum control mechanisms.