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Physical review. B, Condensed matter

Cooper pairs versus Bose condensed molecules: The ground-state current in superfluid ^{3}He-A

N. David Mermin, Paul Muzikar

Published Feb 1, 1980• 84 citations
Publisher

Abstract

We present a new calculation of the current $\stackrel{\ensuremath{\rightarrow}}{\mathrm{g}}$ flowing in a ground state of the Bardeen-Cooper-Schrieffer (BCS) form for a weakly inhomogeneous superfluid with the symmetry of $^{3}\mathrm{He}$-$A$. When the structure of the order parameter not determined by symmetry is appropriate to $^{3}\mathrm{He}$-$A$ and when the mass density $\ensuremath{\rho}$ of the helium is essentially uniform, our current reduces to that calculated by Cross. If the mass density is allowed to vary, we find a generalization of the Cross current which shows that when ${\stackrel{\ensuremath{\rightarrow}}{\mathrm{v}}}_{s}=0$ and the anisotropy axis $\stackrel{\ensuremath{\rightarrow}}{\mathrm{l}}$ is uniform, then the current is simply $(\frac{\ensuremath{\hbar}}{4M}){\stackrel{\ensuremath{\rightarrow}}{\ensuremath{\nabla}}}_{\ensuremath{\rho}}\ifmmode\times\else\texttimes\fi{}\stackrel{\ensuremath{\rightarrow}}{\mathrm{l}}$. We show that this property of the BCS ground state, which taken with the Cross definition leads to an "intrinsic angular momentum density" of $\frac{\ensuremath{\rho}\ensuremath{\hbar}}{2M}$ at zero temperature, also follows directly from the Gor'kov equations. If the range of the order parameter is taken to be small compared with the interatomic separation, then the ground state does not describe $^{3}\mathrm{He}$-$A$, but a Bose-Einstein condensate of tightly bound diatomic molecules. In this limit our current reduces to the form calculated by Ishikawa et al. We indicate why their analysis is only valid in this limit, and offer some rather more general remarks on the differences between Cooper pairing and the Bose-Einstein condensation of diatomic molecules.

DOI
10.1103/physrevb.21.980

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We present a new calculation of the current g\ensuremath→\stackrel{\ensuremath{\rightarrow}}{\mathrm{g}}g\ensuremath→​ flowing in a ground state of the Bardeen-Cooper-Schrieffer (BCS) form for a weakly inhomogeneous superfluid with the symmetry of 3He^{3}\mathrm{He}3He-AAA. When the structure of the order parameter not determined by symmetry is appropriate to 3He^{3}\mathrm{He}3He-AAA and when the mass density \ensuremathρ\ensuremath{\rho}\ensuremathρ of the helium is essentially uniform, our current reduces to that calculated by Cross. If the mass density is allowed to vary, we find a generalization of the Cross current which shows that when v\ensuremath→s=0{\stackrel{\ensuremath{\rightarrow}}{\mathrm{v}}}_{s}=0v\ensuremath→s​=0 and the anisotropy axis l\ensuremath→\stackrel{\ensuremath{\rightarrow}}{\mathrm{l}}l\ensuremath→​ is uniform, then the current is simply (\ensuremathℏ4M)\ensuremath∇\ensuremath→\ensuremathρ\ifmmode×\else\texttimes\fil\ensuremath→(\frac{\ensuremath{\hbar}}{4M}){\stackrel{\ensuremath{\rightarrow}}{\ensuremath{\nabla}}}_{\ensuremath{\rho}}\ifmmode\times\else\texttimes\fi{}\stackrel{\ensuremath{\rightarrow}}{\mathrm{l}}(4M\ensuremathℏ​)\ensuremath∇\ensuremath→​\ensuremathρ​\ifmmode×\else\texttimes\fil\ensuremath→​. We show that this property of the BCS ground state, which taken with the Cross definition leads to an "intrinsic angular momentum density" of \ensuremathρ\ensuremathℏ2M\frac{\ensuremath{\rho}\ensuremath{\hbar}}{2M}2M\ensuremathρ\ensuremathℏ​ at zero temperature, also follows directly from the Gor'kov equations. If the range of the order parameter is taken to be small compared with the interatomic separation, then the ground state does not describe 3He^{3}\mathrm{He}3He-AAA, but a Bose-Einstein condensate of tightly bound diatomic molecules. In this limit our current reduces to the form calculated by Ishikawa et al. We indicate why their analysis is only valid in this limit, and offer some rather more general remarks on the differences between Cooper pairing and the Bose-Einstein condensation of diatomic molecules.
Abstract The superfluid density ns(T)n_{s}(T)ns​(T) n s ( T ) of a superconductor is calculated based on the generalized Bose–Einstein condensation (GBEC) theory that addresses a fully-interacting ternary boson-fermion gas mixture of free electrons as fermions, plus two-electron Cooper pairs (2eCPs) and also, explicitly, two-hole Cooper pairs (2hCPs), both as bosons. Here we consider two special cases (i) 100%–0% (i.e., with no condensed 2hCPs) and (ii) 0%–100% (i.e., with no condensed 2eCPs). Subsumed in GBEC are the Bardeen–Cooper–Schrieffer (BCS) and Bose–Einstein condensation (BEC) theories along with the BCS-BEC crossover theory extended with 2hCPs. We find that in the weak-coupling regime ns(0)n_{s}(0)ns​(0) n s ( 0 ) agrees with data from the Uemura et al. (2004) graph for several elemental SCs by taking in 3D with a quadratic energy-dispersion relation while in 2D with a linear relation are much too far below the data. In the strong-coupling regime the linear behavior of critical temperature TcT_{c}Tc​ T c vs ns(0)n_{s}(0)ns​(0) n s ( 0 ) obtained here is just as Božović et al. (2016) found. However, in 2D with a linear relation accounting for 0%–100%, ns(T)/ns(0)n_{s}(T)/n_{s}(0)ns​(T)/ns​(0) n s ( T ) / n s ( 0 ) compares well with some high- TcT_{c}Tc​ T c -cuprate SC data between the two coupling regimes.
We report results of quantum Monte Carlo calculations of the ground state of dilute Fermi gases with attractive short-range two-body interactions. The strength of the interaction is varied to study different pairing regimes which are characterized by the product of the sss-wave scattering length and the Fermi wave vector, akFa{k}_{F}akF​. We report results for the ground-state energy, the pairing gap $\ensuremath{\Delta}$, and the quasiparticle spectrum. In the weak-coupling regime, $1∕a{k}_{F}<\ensuremath{-}1$, we obtain Bardeen-Cooper-Schrieffer (BCS) superfluid and the energy gap $\ensuremath{\Delta}$ is much smaller than the Fermi gas energy EFG{E}_{\mathrm{FG}}EFG​. When a>0a>0a>0, the interaction is strong enough to form bound molecules with energy Emol{E}_{\mathrm{mol}}Emol​. For $1∕a{k}_{F}\ensuremath{\gtrsim}0.5$, we find that weakly interacting composite bosons are formed in the superfluid gas with $\ensuremath{\Delta}$ and gas energy per particle approaching $\ensuremath{\mid}{E}_{\mathrm{mol}}\ensuremath{\mid}∕2$. In this region, we seem to have Bose-Einstein condensation (BEC) of molecules. The behavior of the energy and the gap in the BCS-to-BEC transition region, $\ensuremath{-}0.5<1∕a{k}_{F}<0.5$, is discussed.
We consider the current correlation function for a three-dimensional system of fermions embedded in a homogeneous background and mutually interacting via an attractive short-range potential, below the (superconducting) critical temperature. Diagrammatic contributions in the broken-symmetry phase are identified, which yield for the (wave-vector and frequency-dependent) current correlation function the fermionic BCS approximation in the weak-coupling limit and the bosonic Bogoliubov approximation in the strong-coupling limit (whereby composite bosons form as bound-fermion pairs). The temperature dependence of the superfluid density (from the BCS exponential behavior at weak coupling to a power-law behavior at strong coupling) and the form of the Pippard-like kernel at zero temperature are explicitly obtained from weak to strong coupling. Quite generally, it is shown that the Pippard-like kernel is the sum of a local (London-like) term and of a nonlocal component, the local term being dominant in the strong-coupling limit and the nonlocal component in the BCS (weak-coupling) limit. It is also shown that the range of the nonlocal component is determined by the coherence length measuring the spatial correlations of the amplitude of the order parameter, namely, the correlations among different Cooper pairs (or composite bosons), rather than between the fermionic partners of a given pair. In addition, a prescription is provided for mapping the fermionic onto the bosonic diagrammatic theories in the broken-symmetry phase, thus complementing what has been already done in the normal phase.
Particle interactions in a Fermi gas may be such as to attract pairs near the Fermi surface more strongly in l=1,2,3l=1, 2, 3l=1,2,3 or higher states than in the simple spherically symmetrical sss state. In that case the Bardeen-Cooper-Schrieffer condensed state must be generalized, and the resulting state is an anisotropic superfluid. We have studied the properties of this type of state in considerable detail, especially for l=1and2l=1 \mathrm{and} 2l=1and2. We have derived expressions for the energy, the moment of inertia, the magnetic susceptibility and the specific heat. We also derive the density correlation function and the density-current density correlation; in some cases the latter implies that the liquid has net surface currents and a net orbital angular momentum. The ground state for l=2l=2l=2 is different from those previously considered, and has cubic symmetry and no net angular momentum. A general method for replacing the possibly rather complicated potential by a simple scattering matrix is given. A brief discussion of possible collective effects is included. We apply our results to liquid He3{\mathrm{He}}^{3}He3; after correction for scattering by a method due to Suhl, it is found that the predicted transition should take place below 0.02\ifmmode^\circ\else\textdegree\fi{}K. Other possible applications are suggested.
We analyze the evolution of superfluidity for nonzero orbital angular momentum channels from the Bardeen-Cooper-Schrieffer (BCS) to the Bose-Einstein condensation (BEC) limit in three dimensions. First, we analyze the low-energy scattering properties of finite range interactions for all possible angular momentum channels. Second, we discuss ground-state (T=0)(T=0)(T=0) superfluid properties including the order parameter, chemical potential, quasiparticle excitation spectrum, momentum distribution, atomic compressibility, ground-state energy, and low-energy collective excitations. We show that a quantum phase transition occurs for nonzero angular momentum pairing, unlike the sss-wave case where the BCS to BEC evolution is just a crossover. Third, we present a Gaussian fluctuation theory near the critical temperature (T=Tc)(T={T}_{\mathrm{c}})(T=Tc​), and we analyze the number of bound, scattering, and unbound fermions as well as the chemical potential. Finally, we derive the time-dependent Ginzburg-Landau functional near Tc{T}_{\mathrm{c}}Tc​, and compare the Ginzburg-Landau coherence length with the zero-temperature average Cooper pair size.
We derive the Josephson relation for a dilute Bose gas in the framework of an auxiliary-field (AF) resummation of the theory in terms of the normal- and anomalous-density condensates. In the leading order of the AF loop expansion (LOAF) we find two critical temperatures in the phase diagram: the critical temperature Tc{T}_{c}Tc​, where the atom Bose-Einstein condensate (BEC) appears first, and the temperature ${T}^{\ensuremath{\star}}>{T}_{c}$, which indicates the onset of superfluidity and the appearance of a diatom condensate in the system. In this context, the Josephson relation shows that the superfluid density is related to the square of a second-order parameter, the anomalous density, $\ensuremath{\langle}A\ensuremath{\rangle}\ensuremath{\langle}\ensuremath{\varphi}\ensuremath{\varphi}\ensuremath{\rangle}$, which can be thought of as a diatom condensate analogous to the Cooper-pair condensate discussed in the BCS approach to dilute Fermi gases. This is in contrast with the corresponding result in the Bose gas theory without a diatom condensate, which predicts that the superfluid density is proportional to the square of the usual atom BEC condensate, $\ensuremath{\langle}\ensuremath{\varphi}\ensuremath{\rangle}$. In the region between Tc{T}_{c}Tc​ and ${T}^{\ensuremath{\star}}$ the anomalous-density Green's function contains a zero energy-momentum state corresponding to a Goldstone state. This is a two-particle state with U(1) charge two. Our findings are consistent with the prediction that in the temperature range between Tc{T}_{c}Tc​ and ${T}^{\ensuremath{\star}}$ a fraction of the system is in the superfluid state in the absence of the usual atom BEC condensate. This situation is similar to the case of dilute Fermi gases, where the superfluid density is proportional to the square of the gap parameter. The Josephson relation relies on the existence of zero energy and momentum excitations showing the intimate relationship between superfluidity and the Goldstone theorem.