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Optica Acta International Journal of Optics

A Multilevel System in an Asymptotically Strong Field

A. Melikyan

Published Jul 1, 1981• 1 citation
Publisher

Abstract

The behaviour of a multilevel system in a strong field is considered, when the interaction energy is much greater than the energy of one quantum and the latter is of the same order as the level spacing of the system. In the case of a monochromatic field the zero-order approximation for quasi-energy is found to be the diagonal matrix element of the unperturbed hamiltonian over the interaction operator eigenfunctions. The asymptotes to the quasi-energy spectrum for the hamiltonian with arbitrary periodic time dependence are also obtained.

DOI
10.1080/713820662

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The behaviour of a multilevel system in a strong field is considered, when the interaction energy is much greater than the energy of one quantum and the latter is of the same order as the level spacing of the system. In the case of a monochromatic field the zero-order approximation for quasi-energy is found to be the diagonal matrix element of the unperturbed hamiltonian over the interaction operator eigenfunctions. The asymptotes to the quasi-energy spectrum for the hamiltonian with arbitrary periodic time dependence are also obtained.
A strong laser field interacting with an atom or a molecule can induce a coherent process which includes a large number of energy levels. If we can find a transformation which eliminates the explicit time dependence of the interaction Hamiltonian (for example, the rotating-wave approximation), we can reduce the dynamic problem to the consideration of eigenvalues and eigenvectors of the Hamiltonian. However, the complexity of an arbitrary multilevel Hamiltonian usually forces us to use numerical methods, and, therefore, not much general understanding about multilevel systems can be achieved. We consider the multilevel problems in a more general setting. Our approach is based on the observation that an arbitrary Hamiltonian matrix can be transformed into a tridiagonal form by unitary transformation.1 A tridiagonal form represents a ladder-type multilevel system. From all W-level systems the ladder configuration is the simplest in the sense that the number of level connections is the smallest possible. This means that the most effective analysis of a given multilevel system can be achieved using the transformation to ladder configuration. The spectral analysis of ladders is facilitated by the connections to orthogonal polynomials and continued fractions. The investigations about the spectral properties of ladders are reported.
The problem of the interaction of a quantum system having discrete states, with a classical oscillating field, is reexamined as a problem in the solution of the time-dependent Schrodinger equation with a periodic Hamiltonian. A method is presented for approximating the time-dependent Hamiltonian with a time-independent one in the weak oscillating field case. With the aid of Floquet's theorem the problem is exactly converted to one with a time-independent Hamiltonian represented by an infinite matrix. The approximation of only two states then permits finding the resonance line shape by perturbation theory for both single and multiple quantum transitions with equal ease. The simple case of only two states connected by an off diagonal sinusoidal perturbation is studied in detail, and a complete description of the average transition probability is found for the strong oscillating field case. A few more complex cases are discussed. A deeper understanding of the analysis is obtained by examining the theory with the oscillating field quantized. Experimental verification of the theory could best be obtained by the methods of atomic beam spectroscopy at radio frequencies.
The spectrum of resonance fluorescence from laser-driven multi-level systems is investigated and especially its asymptotic frequency dependence in the wings. Analytical results are presented and the transitions within multilevel systems are classified into three categories according to the asymptotic frequency dependence of their spectra. Under certain conditions an arbitrarily fast asymptotic fall-off behaviour of the spectrum is found which, for intermediately strong driving fields, leads to subnatural linewidths. Numerical examples are presented to illustrate the analytical results.
A perturbation theory is developed for constructing the quasi-energy operator Q of the Tavis-Cummings Hamiltonian, which includes the interaction of atoms with a classical quasi-monochromatic field. The operator Q of the first order in the interaction δ of an atom with a resonator mode has a form of the generalized Tavis-Cummings Hamiltonian (in the interaction representation) to which the oppositely rotating terms with a changed interaction constant are added. Such a Hamiltonian has a singularity in the dimensionless amplitude σ of a classical field. In the vicinity of this singularity, the Hamiltonian spectrum tends to a continuous one, while the degree of squeezing of field quadratures (in its eigenstates) increases infinitely. In the case of one atom and the biharmonic perturbation, the operator Q is obtained up to the third order of the perturbation theory. The spectral problem for Q is studied. The features of the dependence of the quasi-energy spectrum on σ are explained by the presence of an efficient barrier between the regions of the “coordinate” space. It is found that the above-mentioned singularity corresponds to the beginning of the parametric resonance zone. Analytic expressions for the top and bottom of this zone in the δσ plane are presented.
A perturbation series is derived for the Schr\"odinger equation where the perturbation is permitted to go to \ensuremath{\infty}. Such an asymptotic series can be obtained in a representation where the time evolution of the states is due to the unperturbed part of the Hamiltonian of the problem and the time evolution of the observables is determined by the perturbation, contrary to the interaction picture. The equivalence between the series given by such a picture, and an asymptotic perturbation scheme is given. The method is applied to a spin-1/2 particle in a two-component magnetic field, one component of which, considered as a perturbation, can be time varying. Choosing a constant perturbation we show the equivalence between the exact solution and the approximate one when a component of the magnetic field is much larger than the other. In this case the limit t\ensuremath{\rightarrow}\ensuremath{\infty} cannot be taken, as mixed-secular terms appear in the asymptotic series. Taking a linear time-varying dependence for a component of the magnetic field, we get a nonanalytic asymptotic series.
We prove that, for a quantum system that undergoes a strong perturbation, the solution of the leading order equation of the strong field approximation (M.Frasca, Phys. Rev. A, {\bf 45}, 43 (1992)) can be derived by the adiabatic approximation. In fact, it is shown that greatest is the perturbation and more similar the quantum system is to an adiabatic one, the solution being written as a superposition of eigenstates of the time-dependent perturbation.A direct consequence of this result is that the solution of the Schrödinger equation in the interaction picture, in the same approximation for the perturbation, coincides with the one of the leading order of the strong field approximation. The limitation due to the requirement that the perturbation has to commute at different times is so overcome. Computational difficulties could arise to go to higher orders. Beside, the method is not useful for perturbations that are constant in time. In such a case a small time series is obtained, indicating that this approximation is just an application to quantum mechanics of the Kirkwood-Wigner expansion of statistical mechanics. The theory obtained in this way is applied to a time-dependent two-level spin model, already considered for the study of the Berry's phase, showing that a geometrical phase could arise if a part of the hamiltonian is considered as a strong perturbation. No adiabatic approximation is taken on the parameters of the hamiltonian, while their cyclicity is retained.