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Physical Review A

Coherence properties of entangled light beams generated by parametric down-conversion: Theory and experiment

Adel Joobeur, Bahaa E. A. Saleh, Todd S. Larchuk, Malvin Carl Teich

Published Jun 1, 1996• 126 citations
Publisher

Abstract

Using a multidimensional Gaussian approximation of the wave function for the signal and idler light generated by spontaneous parametric down-conversion, we derive analytical expressions for the second-order coherence function and the fourth-order coherence function (which is proportional to the signal-idler photon coincidence rate). The magnitudes of these functions are expressed as products of Gaussian functions of the azimuthal angles, the polar angles, and the time delay. Their widths determine six parameters: the coherence angles and coherence time, and the entanglement angles and entanglement time. We show how these parameters are governed by the pump-beam waist, the pump spectral width, and the crystal length. We thereby derive relations analogous to the van Cittert--Zernike theorem and the Siegert relation for thermal light. We show that the normalized photon coincidence rate decreases sharply as the signal and idler apertures become mismatched or misaligned. We experimentally confirm this latter prediction by using parametrically down-converted light obtained from a ${\mathrm{LiIO}}_{3}$ crystal pumped by ${\mathrm{Kr}}^{+}$-ion laser radiation at 413 nm. \textcopyright{}1996 The American Physical Society.

DOI
10.1103/physreva.53.4360

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Using a multidimensional Gaussian approximation of the wave function for the signal and idler light generated by spontaneous parametric down-conversion, we derive analytical expressions for the second-order coherence function and the fourth-order coherence function (which is proportional to the signal-idler photon coincidence rate). The magnitudes of these functions are expressed as products of Gaussian functions of the azimuthal angles, the polar angles, and the time delay. Their widths determine six parameters: the coherence angles and coherence time, and the entanglement angles and entanglement time. We show how these parameters are governed by the pump-beam waist, the pump spectral width, and the crystal length. We thereby derive relations analogous to the van Cittert--Zernike theorem and the Siegert relation for thermal light. We show that the normalized photon coincidence rate decreases sharply as the signal and idler apertures become mismatched or misaligned. We experimentally confirm this latter prediction by using parametrically down-converted light obtained from a LiIO3{\mathrm{LiIO}}_{3}LiIO3​ crystal pumped by Kr+{\mathrm{Kr}}^{+}Kr+-ion laser radiation at 413 nm. \textcopyright{}1996 The American Physical Society.
We investigate the amplitude and intensity spatiotemporal coherence and the photon coincidence rates of far-field down-converted light resulting from the interaction of a pump wave of finite spectral width with a nonlinear crystal of finite spatial width. We examine the interplay between energy and phase mismatches and their effects on the intrabeam and interbeam spatial and temporal coherence of the down-converted beams. We show that the down-converted light is spatially incoherent in the second order, and that the signal-idler fourth-order coherence extends over finite entanglement angles. We also study the effect of the apertures through which the down-converted light is collected, when they are centered at phase-matched or misaligned directions.
The spectral properties of entangled photon pairs generated via quasi-phased matching in spontaneous parametric down-conversion are proposed and demonstrated experimentally.A general mathematical model for evaluating the spectral properties is developed to obtain the spectrum shape and range of down-converted photons.The model takes into account the effects of phase mismatching due to non-ideal pumping and the relationship between crystal periodic modulation function and the incidence angle of the pump beam.The spectrum curve shape is determined by the discrete Fourier transform of a Gaussian pump beam and the integration of parametric down-conversion generated by an individual plane wave.An experiment is carried out with a PPLN non-linear crystal and dispersing optics, which shows a good consistency in their spectral ranges and shapes with our model predictions within the spectrum of 600-633 nm.This therefore illustrates that both the simulation model and the experimental process are reasonable.This novel method has potential applications in high-accuracy calibration in the wide spectrum using correlated photons.
In parametric down-conversion, a nonlinear crystal is pumped by a laser and spontaneous emission takes place in signal and idler modes according to the phase-matching conditions. A seed laser can stimulate the emission in the signal beam if there is mode overlap between them. This also enhances the emission in the idler beam, affecting its coherence properties. While the degree of coherence of the idler field as a function of the seed power has already been studied, the transverse coherence length has not yet been properly investigated. The transverse coherence length is a key parameter of optical beams that determines the beam divergence, for example. Here, we present a theoretical and experimental investigation of the transverse coherence length in stimulated down-conversion. In addition, we make a connection between stimulated down-conversion and partially coherent sources like the Gaussian-Schell model beams, and show that in general the idler field cannot be described with this model.
In the process of spontaneous parametric down-conversion, photons from a pump field are converted to signal and idler photon pairs in a nonlinear crystal. The reversed process, or up-conversion of these pairs back to single photons in a second crystal, is also possible. Here, we present experimental measurements of the up-conversion rate with a controlled time delay introduced between the signal and idler photons. As a function of delay, this rate presents a full width at half maximum of 27.9 fs under our experimental conditions, and we further demonstrate that group delay dispersion of the photon pairs broadens this width. These observations are in close agreement with our calculations, thus demonstrating an ultrafast, nonclassical correlation between the signal and idler waves.
Entangled-photon pairs (biphotons) generated by spontaneous optical parametric down-conversion exhibit a number of properties that are analogous to those of ordinary photons generated by incoherent sources. The spatial pump-field distribution and the two-particle wave function in the biphoton case play the respective roles of the source intensity distribution and the second-order coherence function in the incoherent case. The van Cittert--Zernike theorem, which is applicable for incoherent optical sources emitting independent photons, has a counterpart for biphotons. Likewise, the partial-coherence theory of image formation has an analogous counterpart for biphoton beams transporting spatial information. However, an underlying duality, rather than analogy, accompanies the mathematical similarity between incoherent and biphoton emissions if the comparison is made between the photon count rate in the incoherent case and the biphoton count rate in the entangled-photon case. The smaller the size of an incoherent source, the more separable is the coherence function and the more coherent is the field, and therefore the higher the visibility of ordinary interference fringes. In contrast, the narrower the size of a biphoton pump source, the more separable is the wave function and the less entangled is the field, and therefore the lower the visibility of biphoton interference fringes. This duality is similar to the complementarity between single and two-photon interference exhibited for biphotons.
Coherence properties of the down-converted beams generated in spontaneous parametric down-conversion are investigated in detail using an iCCD camera. Experimental results are compared with those from a theoretical model developed for pulsed pumping with a Gaussian transverse profile. The results allow us to tailor the shape of correlation area of the signal and idler photons using pump-field and crystal parameters. As an example, splitting of a correlation area caused by a two-peak pump-field spectrum is experimentally studied.