We investigate the amplitude and intensity spatiotemporal coherence and the photon coincidence rates of far-field down-converted light resulting from the interaction of a pump wave of finite spectral width with a nonlinear crystal of finite spatial width. We examine the interplay between energy and phase mismatches and their effects on the intrabeam and interbeam spatial and temporal coherence of the down-converted beams. We show that the down-converted light is spatially incoherent in the second order, and that the signal-idler fourth-order coherence extends over finite entanglement angles. We also study the effect of the apertures through which the down-converted light is collected, when they are centered at phase-matched or misaligned directions.
We investigate the amplitude and intensity spatiotemporal coherence and the photon coincidence rates of far-field down-converted light resulting from the interaction of a pump wave of finite spectral width with a nonlinear crystal of finite spatial width. We examine the interplay between energy and phase mismatches and their effects on the intrabeam and interbeam spatial and temporal coherence of the down-converted beams. We show that the down-converted light is spatially incoherent in the second order, and that the signal-idler fourth-order coherence extends over finite entanglement angles. We also study the effect of the apertures through which the down-converted light is collected, when they are centered at phase-matched or misaligned directions.
Using a multidimensional Gaussian approximation of the wave function for the signal and idler light generated by spontaneous parametric down-conversion, we derive analytical expressions for the second-order coherence function and the fourth-order coherence function (which is proportional to the signal-idler photon coincidence rate). The magnitudes of these functions are expressed as products of Gaussian functions of the azimuthal angles, the polar angles, and the time delay. Their widths determine six parameters: the coherence angles and coherence time, and the entanglement angles and entanglement time. We show how these parameters are governed by the pump-beam waist, the pump spectral width, and the crystal length. We thereby derive relations analogous to the van Cittert--Zernike theorem and the Siegert relation for thermal light. We show that the normalized photon coincidence rate decreases sharply as the signal and idler apertures become mismatched or misaligned. We experimentally confirm this latter prediction by using parametrically down-converted light obtained from a LiIO3 crystal pumped by Kr+-ion laser radiation at 413 nm. \textcopyright{}1996 The American Physical Society.
Here we investigate the all-optical control of spectral correlations in spontaneous parametric down-conversion. We show that when photon pairs are projected onto high-order spatial modes, the spatial structure of the pump field defines the phase-matching function of the nonlinear interaction. Thus, by structuring the pump field in both space and spectrum, the biphoton spectral correlations are fully controlled. Considering a standard periodically-poled crystal as the nonlinear medium, we show that the Gouy phase matching method proposed here can generate both spectrally uncorrelated and high-dimensional spectrally entangled photon pairs, similarly to what is achieved with aperiodically-poled crystals. Furthermore, we show that our method can generate a wider class of quantum states if the pump field is a spatiotemporal wavepacket, that is, if its spatial and spectral structures are correlated.
In theoretical and experimental work, we consider the process in which an entangled photon pair recombines into a single photon in a nonlinear crystal, with particular interest in the amplitude distribution and coherence properties of the up-converted light. It is found that the up-converted state has perfect mutual coherence with the pump that originally produced the photon pair in another nonlinear crystal and that the amplitude has the spatiotemporal structure of the original pump mode, filtered by a linear transfer function. These conclusions are drawn from leading-order calculations performed in the interaction picture, with the multimodal nature of all fields being fully accounted for. In our experimental results, we observe the spatial similarity between the up-converted light and the original pump mode; their mutual coherence is demonstrated through observation of fringes with near-unit visibility. The effects studied here have potential applications in quantum information processing and also confirm that the principle of path indistinguishability holds even under unusually extreme conditions.
Spontaneous parametric down-conversion (SPDC) can produce entangled photons from a nonlinear medium driven by a pump beam, and has thus been a key resource in photonic quantum technologies. Historically, the low efficiency of SPDC prompted the use of lasers, which are high-intensity light sources, as pump sources. However, the practical implementation of laser-driven systems faces an imminent energy bottleneck. Lasers typically have suboptimal energy efficiencies due to lasing thresholds and the technical demands of thermal management. As a result, laser-pumped entangled photon sources suffer from significant power overhead, rendering quantum devices less sustainable. Over the past few decades, light-emitting diodes (LEDs) have emerged as inexpensive and energy-efficient alternatives for high-intensity light sources. Since 2010, studies have shown that LEDs can drive SPDC and generate photon pairs. These results suggests the potential to replace lasers with ubiquitous and natural light sources to build environmentally friendly quantum devices. However, replacing lasers with other light sources entails a lack of coherence in all degrees of freedom (DoFs) of the pump beam, including spatial, temporal-spectral, and polarization, which may influence the resulting entanglement generated from SPDC. While earlier studies established that pump coherence in a specific DoF sets an upper bound for entanglement in that same DoF, the cross-influence between different DoFs has not been fully investigated. In this thesis, we study the influence of the pump's spatiotemporal coherence on the polarization entanglement generated from SPDC. First, we experimentally demonstrate that polarization-entangled two-photon states can be generated from SPDC pumped by spatiotemporally incoherent light emitted from an LED. Although the resulting entanglement appears lower than that of laser-pumped SPDC, we theoretically show that spatiotemporal incoherence does not fundamentally constrain polarization entanglement; rather, the reduction arises from a coupling between spatiotemporal and polarization DoFs introduced by the experimental setup. We determined experimentally that this cross-influence acts as a deterministic mapping from the spatial components of the pump to the two-photon polarization state. Because this mapping depends on technical aspects of the setup, we envisioned that it could be either (i) engineered to structure entanglement in higher dimensions, or (ii) compensated to reduce spatial distinguishability. Building on the latter, we show that by placing the nonlinear medium in a phase-compensated interferometric setup, SPDC pumped by spatially incoherent light can produce high polarization entanglement that violates local realism, even without postselecting the SPDC field for a single spatial mode. Finally, as a proof-of-principle demonstration of a truly environmentally friendly quantum light source, we demonstrate the generation of polarization-entangled two-photon states from SPDC pumped by a natural source - sunlight.
Normally, the signal and idler photons produced in the process of parametric down- conversion exhibit no second-order interference. However, in the presence of an external laser beam that follows the path of the signal photon and induces stimulated down-conversions, one would expect coherence to develop between the down-converted signal and idler beams. We have demonstrated the existence of this phenomenon in an experiment with two down-converters pumped by similar pump beams, in which two mutually coherent laser beams followed the paths of the two down-converted signal photons and induced coherence between the two down- converted idler beams. The induced coherence gives rise to observable interference effects, which are presented.
In the process of spontaneous parametric down-conversion, photons from a pump field are converted to signal and idler photon pairs in a nonlinear crystal. The reversed process, or up-conversion of these pairs back to single photons in a second crystal, is also possible. Here, we present experimental measurements of the up-conversion rate with a controlled time delay introduced between the signal and idler photons. As a function of delay, this rate presents a full width at half maximum of 27.9 fs under our experimental conditions, and we further demonstrate that group delay dispersion of the photon pairs broadens this width. These observations are in close agreement with our calculations, thus demonstrating an ultrafast, nonclassical correlation between the signal and idler waves.