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Journal of Experimental and Theoretical Physics Letters

Resonance fluorescence of a two-level atom in a feedback loop

V. A. Tomilin, Leonid V. Il'ichov

Published Jan 1, 2012• 12 citations
Publisher

Abstract

The resonance fluorescence spectrum of a two-level atom in a classical light field, whose phase is changed by a feedback system by π after the detection of each spontaneous photon, has been calculated. The spectrum resembles the well-known Rautian-Mollow triplet. However, the sidebands become sharply asymmetric at a nonzero frequency detuning of the light field from the atomic resonance transition. In addition, the spectrum retains the pronounced triplet shape even beyond the secular approximation, when the sidebands of the Rautian-Mollow structure become unresolved in the absence of the feedback.

DOI
10.1134/s0021364011210119

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Resonance fluorescence statistics of a two-level atom in feedback loop

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Statistics of photoemission events into the components of a triplet of resonance fluorescence of a two-level atom in a classical optical field, the phase of which changes by π upon the detection of spontaneous photon, is compared with the case when the feedback is absent. In contrast to the known problem on the statistics of resonance fluorescence of a two-level atom, a grouping of photocounts should be observed in each separate side component of the triplet. Anticorrelation of photoemission into side components is also predicted, and the type of correlations between the emission into the central component of the triplet and into any of the side ones can be controlled by varying the detuning of the radiation frequency from the resonant value.

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The resonance fluorescence spectrum of a two-level atom in a classical light field, whose phase is changed by a feedback system by π after the detection of each spontaneous photon, has been calculated. The spectrum resembles the well-known Rautian-Mollow triplet. However, the sidebands become sharply asymmetric at a nonzero frequency detuning of the light field from the atomic resonance transition. In addition, the spectrum retains the pronounced triplet shape even beyond the secular approximation, when the sidebands of the Rautian-Mollow structure become unresolved in the absence of the feedback.
Statistics of photoemission events into the components of a triplet of resonance fluorescence of a two-level atom in a classical optical field, the phase of which changes by π upon the detection of spontaneous photon, is compared with the case when the feedback is absent. In contrast to the known problem on the statistics of resonance fluorescence of a two-level atom, a grouping of photocounts should be observed in each separate side component of the triplet. Anticorrelation of photoemission into side components is also predicted, and the type of correlations between the emission into the central component of the triplet and into any of the side ones can be controlled by varying the detuning of the radiation frequency from the resonant value.
A theoretical analysis of the resonance fluorescence of a two‐level atom in a classical monochromatic field with feedback phase switching depending on the fluorescence triplet component which the last spontaneously emitted photon belongs to is presented. The considered feedback loop is a hybrid quantum‐classical system. Statistics of photoemissions into the triplet components is investigated as well as correlations between the components. In contrast to the well‐known resonance fluorescence of a two‐level atom without feedback phase switching, a bunching of photocounts is predicted in each side‐band, and successive photoemissions into different side‐bands manifest antibunching. The type of the statistics can efficiently be controlled by the frequency detuning of the external field. In many points the considered feedback scheme provides drastically different statistical features of fluorescence when compared with the scheme of frequency‐unselective feedback phase switching. image
The statistics of photoemission events of a pair of closely spaced two-level atoms is calculated in a classical light field whose phase is changed by π after the detection of each spontaneous photon. This statistics is compared with the statistics in the case when the feedback is missing. In both cases, one can observe noticeable antibunching of photons in the range of parameters where no antibunching is observed in a single-atom system. The feedback substantially increases the antibunching. This effect manifests itself more strongly in relatively weak fields and for considerable frequency detunings.
We investigate the resonance fluorescence features of a small ensemble of closely packed and moderately laser-pumped two-level emitters at resonance. The mean distance between any two-level radiators is smaller than the corresponding emission wavelength, such that the dipole-dipole interactions are not negligible. We have found that under the secular approximation, the collective resonance fluorescence spectrum consists of 2 N + 1 spectral lines, where N is the number of emitters from the sample. The 2 N spectral sidebands, symmetrically located around the generalized Rabi frequency with respect to the central line at the laser frequency, are distinguishable if the dipole-dipole coupling strength is larger than the collective spontaneous decay rate. This way, one can estimate the radiators number within the ensemble via measuring of the spontaneously scattered collective resonance fluorescence spectrum. Contrarily, if the dipole-dipole coupling is of the order of or smaller than the cooperative spontaneous decay rate, but still non-negligible, the spectrum turns into a Mollow-like fluorescence spectrum, where the two sidebands' spectral lines broaden proportional to the dipole-dipole coupling strength. Published by the American Physical Society 2024
Resonance fluorescence from atomic systems consists of a single spectral peak that evolves into a Mollow triplet for a strong excitation field. Photons from different peaks of the triplet show distinct timing correlations that make the fluorescence a useful light source for quantum information purposes. We characterize the fluorescence of a single optically trapped 87Rb^{87}\mathrm{Rb}87Rb atom that is excited resonantly at different power levels. Second-order correlation measurements reveal the single photon nature of the fluorescence concurrently with Rabi oscillations of a strongly excited atom. The asymmetry in correlations between photons from two sidebands of the fluorescence spectrum when the atom is exposed to an off-resonant field indicates that there is a preferred time ordering of the emitted photons from different sidebands.
We investigate the fluorescence spectrum of a two-level system driven by a monochromatic classical field by the Born-Markovian master equation based on a unitary transformation. The main purpose is to understand the effects of counter-rotating-wave terms of the driving on spectral features of the fluorescence. We have derived an analytical expression for the fluorescence spectrum, which is different from Mollow's theory, while Mollow's result on resonance is the limiting case of ours in moderately weak driving regimes. Our results demonstrate precisely that the counter-rotating-wave terms of the driving play an important role in the fluorescence spectrum for intense driving: (i) the counter-rotating coupling suppresses the red sideband in the Mollow triplet and it enhances the blue one in explicitly contrast to the well-known equal intensity of the sideband in Mollow's theory, (ii) the higher-order Mollow triplets appear as a characteristic spectral feature arising from counter-rotating-wave terms of the driving, and (iii) a significant frequency shift of the sidebands is observed, which depends on both the detuning and driving strength.