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Physical Review A

Distortionless optical pulse propagation in a three-level medium

Joseph Hayden Higginbotham, Robert T. Deck, D. G. Ellis

Published Nov 1, 1977• 4 citations
Publisher

Abstract

We report on computer-generated solutions to the coupled matter-field equations which provide the first evidence for distortionless optical pulse propagation in an absorbing medium of three-level atoms. The associated phenomenon represents the three-level equivalent of self-induced transparency in two-level atoms. Results have application to the propagation of short, coherent optical pulses in a medium in which the atoms have two distinct transition frequencies in near resonance with the pulse carrier frequency. We relate in particular to the case of pulse propagation in a magnetically perturbed sodium vapor where the pulse carrier frequency is tuned near the frequencies of the well-known sodium $D$ lines. Here we obtain particular solutions corresponding to three and five peak pulses with "areas" of approximately $6\ensuremath{\pi}$ and $10\ensuremath{\pi}$, respectively. The solutions are strongly supported by a number of analytical results. In particular, simple algebraic relations are found which give the populations of the levels in terms of the field variables.

DOI
10.1103/physreva.16.2089

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Quantum Electronics•Feb 28, 2000•10 citations
We report on computer-generated solutions to the coupled matter-field equations which provide the first evidence for distortionless optical pulse propagation in an absorbing medium of three-level atoms. The associated phenomenon represents the three-level equivalent of self-induced transparency in two-level atoms. Results have application to the propagation of short, coherent optical pulses in a medium in which the atoms have two distinct transition frequencies in near resonance with the pulse carrier frequency. We relate in particular to the case of pulse propagation in a magnetically perturbed sodium vapor where the pulse carrier frequency is tuned near the frequencies of the well-known sodium DDD lines. Here we obtain particular solutions corresponding to three and five peak pulses with "areas" of approximately 6\ensuremathπ6\ensuremath{\pi}6\ensuremathπ and 10\ensuremathπ10\ensuremath{\pi}10\ensuremathπ, respectively. The solutions are strongly supported by a number of analytical results. In particular, simple algebraic relations are found which give the populations of the levels in terms of the field variables.
The coherent propagation of two optical short pulses through a resonant medium consisting of two three-level atoms in the configuration is investigated. A self-consisting analytical solution without steady state or adiabatic approximations is presented. The electric field in the model studied consists of two co-propagating plane waves, each of which is in near resonance with a transition in the absorber. The density matrix of two three level atoms is studied. Also, the reduced density matrices are stated. The present approach for the semiclassical treatment of resonant coherent interactions in three-level atoms represents a generalization of the Maxwell- Bloch equations for a two-level system. The Maxwell-Bloch equations reduced to the non-linear pendulum equation. The solution shows that the two pulses can propagate simultaneously without loss under some conditions about the pulses and the medium. The propagation of the two pulses through the medium without any constrains approves the self -induced transparency (SIT) phenomenon.
Quantum coherence and interference in atomic systems can lead to interesting optical phenomena such as nonabsorbing resonances, lasing without inversion, generating an ultrahigh index of refraction without absorption, propagation of light pulses without losses. In the last-named is given the title transparency. Up to now it is known some types of transparency in multi-level resonant media. One of them is electromagnetically induced transparency (EIT). The phenomenon of EIT in the propagation of laser radiation through an absorbing medium has been recently investigated and explained in terms of quantum coherence and interference for multi-level atomic system. For instance in the (Lambda) -system, if the atomic medium is prepared in a quantum superposition of states, matched pulses, i.e., a pair of optical pulses whose amplitude and phase have a well defined relation, propagate without absorption. The mechanism of coherent population trapping is responsible for EIT in a (Lambda) -system. There is another, well known mechanism for creating transparency in a two-state atom: self-induced transparency, or SIT. Here, a single pulse whose area (the integral of its Rabi frequency over time) is 2(pi) is applied to the medium. Such a pulse causes the atoms to cycle smoothly from the ground to the excited state and then back again. In principle, such a pulse can propagate over long distances. SIT can be generalized to multi-level systems and multiple quasi-monochromatic fields. Generalization of SIT in a (Lambda) -system was obtained in reference 2. In this report we present a new type of transparency (combined transparency). This type describes propagation of laser pulse through a (Lambda) -type medium where the initial atomic state is prepared in the form of spatially varying coherent superposition of low-energetic states (initial coherency gradient). The common envelope behaves as usual 2(pi) hyperbolic secant pulse, but the ratio between the components of frequencies transitions 1> yields 3> and 2> yields 3> changes due to coherent Raman scattering so (phi) equals atan(E1/E2) equals (pi) /2-Gz, where z is the coordinate, G is the constant determined by both the incident pulse parameters and the initial coherence between the atomic states. Our solution demonstrates a direct connection of EIT in adiabatic regime to the SIT effects. This type of a transparency is given the title screw-type transparency, because for the given form of incident pulse (pitch of screw) medium is transparent, if medium's the initial coherence gradient is correspondingly prepared (thread on a engine nut). Besides a transparency, this phenomenon contains a transformation of the incident pulse frequency during the process of the propagation. This property of the phenomena can be result in a complete conversion of the frequency.
The authors develop a theoretical analysis which describes coherent nonlinear resonant effects where two optical pulses of different frequencies undergo two-photon self-induced transparency (two-photon SIT) in an inhomogeneously broadened three-level system. The field (Maxwell) and atomic (Schrodinger; density matrix representation) equations are coupled in a self-consistent manner by virtue of the resultant macroscopic polarizations at the two frequencies. This treatment is accomplished under circumstances where atomic coherence plays a predominant role. The resulting equations yield a new two-photon area theorem which gives first the intensity dependent, two-photon absorption law analogous to Beer's law for the one-photon transition. Secondly, a 2 pi Lorentzian pulse solution is derived which propagates without loss at the modified pulse velocity.
Resonant absorbing media having many atoms within a cubic resonance wavelength can exhibit large frequency chirps in pulse propagation due to dipole-dipole interactions among the atoms. Analytic solutions are obtained for invariant pulse propagation in such a medium consisting of interacting two-level atoms. Departures from the McCall-Hahn results include nonhyperbolic secant pulse shapes and different than 2π-area pulses. In addition, the excitation of the medium is comparatively suppressed for the same group velocity. The results are interpreted to suggest new experiments.
The spatial and temporal dynamics of two short pulses propagating in an optically dense medium of resonant three-level Λ-atoms is investigated numerically and analytically. The maximum coherence for the Raman transition due to coherent population trapping. It is shown that, at the initial stage of propagation, the waveforms of such pulses only slightly change along the length of the medium, which may considerably exceed the length of linear absorption for a single weak pulse. As the length of the absorbing medium increases, the energy of the probe (first) pulse is completely transferred into the second (control) pulse.