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Solid State Communications

Nonlinear optical phenomena in coherent phase of 2D exciton system

Yu. E. Lozovik, I. L. Kurbakov, I.V. Ovchinnikov

Published Apr 7, 2003• 12 citations
Publisher
DOI
10.1016/s0038-1098(03)00128-5

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We consider many-photon coherent emission governed by coherent recombination of many excitons from Bose condensate. Momentum conservation makes photons simultaneously created in the coherent recombination of several excitons from the condensate have zero sum momentum. Many-photon correlations in the processes of simultaneous many-photon production (photons squeezing) could be detected by photon counting experiments with several detectors spatially arranged in an appropriate way, i.e., by Hanbury-Brown-Twiss-like experiments. We analyze the stimulated processes of N-exciton coherent recombination from the condensate resonantly induced by $N\ensuremath{-}1$ external laser beams with momenta ${\mathbf{k}}_{1},{\mathbf{k}}_{2},\dots{},{\mathbf{k}}_{N\ensuremath{-}1}.$ Such stimulated processes must reveal themselves through a unidirectional beam with recoil momentum ${\mathbf{k}}_{N}=\ensuremath{-}{\ensuremath{\sum}}_{i=1}^{N\ensuremath{-}1}{\mathbf{k}}_{i}.$ In particular, two-exciton coherent recombination from the condensate stimulated by a laser beam effectively acts in a three-dimensional (3D) exciton system as a laser beam backscattering from exciton Bose condensate. For 2D coherent exciton systems besides the backscattering stimulated two-exciton coherent recombination has an additional manifestation---anomalous beam transmission with the only change in the sign of in-plane momentum component of inducing laser beam. We estimate the rates of many-photon coherent emission from a 3D system of Cu2O{\mathrm{Cu}}_{2}\mathrm{O}Cu2​O excitons and from a 2D exciton system in GaAs/AlGaAs coupled quantum wells. The estimations show that these nonlinear optical effects are experimentally observable.
The idea of the design is proposed for the photonic quantum gates (PG) with their input/output properties based on nonlinear optical dynamics of 2D arrays of two-level systems (TLS) in the resonance field of coherent optical pulses. As a particular example of the 2D medium with functions of the PG we consider the GaAs/AlGaAs-based 2D excitonic structures. By methods of femtosecond chronopolarimetry of delayed photoreflection. we have studied the energy and phase relaxation rates and the biexciton binding energy in these structures and have shown that the GaAs/AlGaAs MQW can serve as a good basis for building the PG.
Turbulence and chaos in a semiconductor crystal? These are just some of the intriguing predictions of nonlinear optics with coherent excitons. In this chapter we discuss some aspects of nonlinear coherent optics with the participation of the excitons, photons, and biexcitons. As in many nonlinear systems, these effects arise because of feedback mechanisms, i.e., the light impinging on the system affects the electronic states, which in turn affect the dielectric constant of the medium through which the light passes. These effects are closely related to the phenomena of self-organization [1-8] and optical bistability [7-10] and self-pulsations and the appearance of chaos [2-6]. The cooperative nonlinear coherent processes in optical systems have recently attracted much attention [7-20]. These investigations have stimulated the development of new mathematical methods [21-31] and have opened up possibilities for many new applications. The theoretical and the experimental investigations in these directions give rise to the theory of solitons [32∧2] and lead to the new developments in the optics of ultrashort pulses [43-58]. Ultrafast phenomena such as self-induced transparency and nutation are related to the propagation of solitons and pulse trains, whereas the transient stages of the ultrashort lightpulse penetration in the media are described by area theorems. These coherent ultrafast phenomena typically take place during intervals of time less than the relaxation time, i.e., femtoseconds to picoseconds in typical solids. Collisions and incoherent scattering processes destroy the coherent evolution of the excited particles. But if coherent macroscopic states of the excitons, photons, and biexcitons have been formed because of spontaneous or induced BEC, in this case one can consider their time evolution over intervals of time much greater than the relaxation time.