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Nature China

Photonics: Forbidden light

Felix Cheung

Published Jan 6, 2010• 0 citations
Publisher
DOI
10.1038/nchina.2009.247

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High-harmonic generation in solids provides a powerful window into light-driven electron dynamics on attosecond timescales, yet the role of quantum fluctuations of the driving field remains largely unexplored. Here, we show that the quantum state of light offers a nonclassical degree of freedom for controlling strong-field dynamics in quantum materials. Using graphene driven by bicircular quantum light composed of counterrotating ω and 2 ω components, we theoretically predict that squeezing-induced fluctuations break the dynamical symmetry of the classical bicircular field and activate otherwise forbidden harmonics. By analyzing the helicity-resolved harmonic spectra, we uncover robust polarization signatures uniquely dictated by the squeezed mode's profile, including a relative-phase-controlled helicity switching in the lowest orders. Crucially, second-order intensity correlations reveal that these forbidden harmonics exhibit strongly enhanced, super-Poissonian photon-number fluctuations, confirming that they inherit and directly transduce the nonclassical statistics of the squeezed driving vacuum. Our findings establish forbidden harmonics as high-fidelity optical probes of the quantum state of light and provide additional opportunities at the intersection of quantum optics, strong-field physics, and lightwave engineering in quantum materials.
When a resonance associated with electromagnetically induced transparency in an atomic ensemble is modulated by an off-resonant standing light wave, a band of frequencies can appear for which light propagation is forbidden. We show that dynamic control of such a band gap can be used to coherently convert a propagating light pulse into a stationary excitation with nonvanishing photonic component. This can be accomplished with high efficiency and negligible noise even at the level of few-photon quantum fields thereby facilitating possible applications in quantum nonlinear optics and quantum information.