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Journal of Experimental and Theoretical Physics Letters

Resonance structure of doubly-charged-ion production during laser dielectronic ionization of atoms

І. І. Бондар, В. В. Суран

Published Dec 1, 1998• 12 citations
Publisher

Abstract

The resonance structure of doubly-charged-ion production during the ionization of Ba atoms by infrared radiation (color-center laser radiation) is identified. It is shown that this structure is due to the excitation of states of the neutral Ba atom which are strongly perturbed as a result of the Stark effect under conditions such that the dynamic polarizability has large absolute values and depends strongly on the frequency of the radiation.

DOI
10.1134/1.567802

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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Jun 15, 2007•0 citations
The resonance structure of doubly-charged-ion production during the ionization of Ba atoms by infrared radiation (color-center laser radiation) is identified. It is shown that this structure is due to the excitation of states of the neutral Ba atom which are strongly perturbed as a result of the Stark effect under conditions such that the dynamic polarizability has large absolute values and depends strongly on the frequency of the radiation.
Experimental investigations of resonant structure in doubly charged ion (A 2+ ) formation were carried out during Sr and Ba atom ionization by infrared laser radiation (ω = 8400-9100 cm -1 ). It has been shown that in this case the mechanism of ion formation is a two-electron process - the ions are produced immediately from the neutral atoms. It has been found for the first time that the resonant structure in A 2+ ion formation in such conditions is due to the excitation and ionization of neutral-atom mixed states. The atomic-state mixing in this case results from the Stark effect provided that the polarizability of these states is very high.
The influence of the Stark effect on multiphoton ionization of Ba atoms under conditions when the dynamic polarizability depends strongly on the frequency of the laser radiation is investigated. It is found that for some electric field strengths ε of the laser radiation this effect gives rise to resonance peaks in the Ba + ion yield as a function of the laser radiation frequency at frequencies corresponding to single-photon transitions between the excited states. These frequencies can differ substantially from the frequencies corresponding to the conventional multiphoton excitation of these states from the ground states of the atoms. Peaks in the ion yield as a function of ε behave differently from the conventional Stark effect—their position on the frequency scale does not depend strongly on ε . The conditions under which such an induced resonance structure appears are determined.
The formation of singly and doubly charged ions upon nonlinear ionization of barium atoms is studied as a function of the frequency and intensity of a 8800-8920-cm−1 IR color center laser. Barium atoms are ionized via the four-photon resonance with the strongly perturbed bound 6p 2 1 D 2 state. Doubly charged barium ions are produced by a two-electron mechanism. It is found that the probability of the formation of doubly charged ions under these conditions linearly depends on the laser radiation intensity.
The process of formation of doubly charged ions upon multiphoton ionization of barium atoms by linearly and circularly polarized radiation of dye lasers is studied in the frequency range from 16 600 to 17 900 cm-1. A large number of resonance maxima in the yield of Ba+ and Ba2+ ions were observed upon tuning the radiation frequency. It is unambiguously proved that most resonance maxima in the yield of Ba2+ ions are associated with the resonance transitions in the spectrum of Ba+ ions. This fact confirms the cascade mechanism of formation of Ba2+ ions in the frequency range of localization of these maxima. But the number of the resonant maxima in Ba2+ ions yield do not identified by transitions both in spectra of Ba atom and Ba+ ion. This fact indicates on realization of the noncascade mechanism of Ba2+ ions formation in the frequency range of these maxima.