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Laser Physics Letters

Line shapes of atomic transitions in excited dense gas

Vladimir A. Sautenkov

Published Sep 1, 2011• 20 citations
Publisher

Abstract

We discuss recently published results of experimental studies of dipole-dipole broadened line shapes in excited atomic vapors. The Lorentz local-field shift and self-broadened width were measured in optically excited potassium and rubidium vapors. Strong reduction of the shift and width was observed. This effect allowed resolve electromagnetically induced dressed states inside the self-broadened spectral profile. The experimental results were interpreted using well-known models of the dipole-dipole interactions.

DOI
10.1002/lapl.201110070

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We discuss recently published results of experimental studies of dipole-dipole broadened line shapes in excited atomic vapors. The Lorentz local-field shift and self-broadened width were measured in optically excited potassium and rubidium vapors. Strong reduction of the shift and width was observed. This effect allowed resolve electromagnetically induced dressed states inside the self-broadened spectral profile. The experimental results were interpreted using well-known models of the dipole-dipole interactions.
We study the frequency derivatives of selective reflection from high-density rubidium vapor using a hole-burning technique. Saturation dips are observed inside the self-broadened line shapes. The line self-broadening is a combination of static width and collision width. By analyzing saturation dips, we can separate power broadening and collision width. Our experimental results support the theory of inhomogeneous dipole-dipole induced broadening of transitions in a dense atomic gas, published by J. A. Leegwater and S. Mukamel [Phys. Rev. A 49 (1994) 146].
In this paper, our experimental studies of dipole-dipole interactions in excited resonance gases are discussed. In weakly excited gas the dipole broadening of optical transitions is proportional to its density N. A gas medium can be identified by its density N as rarefied gas, where dipole broadening of atomic transitions is much less than Doppler width, or as dense gas, where dipole broadening is much more than Doppler width. According to our experiments the dipole broadening in rarefied gas does not depend on the optical excitation. This behavior is in a good agreement with predictions of standard theory for impact atomic collisions. In excited dense gas we observed the strong reduction of the dipole broadening. These experimental results are not described by standard theory for impact collisions. We suggested a simple description of the optical properties for excited dense gas.
We have studied the resonant optical response of a dense atomic potassium vapor under conditions such that the response is strongly influenced by local-field effects. Our experimental results are in good agreement with the predictions of theory. We have also discovered a collision-induced shift of the potassium resonance lines given by \ensuremath{\Delta}${\mathrm{\ensuremath{\omega}}}_{\mathrm{c}\mathrm{o}\mathrm{l}=}$\ensuremath{\beta}N, where \ensuremath{\beta}=-5.0\ifmmode\times\else\texttimes\fi{}${10}^{\mathrm{\ensuremath{-}}8}$ ${\mathrm{sec}}^{\mathrm{\ensuremath{-}}1}$ cm3{\mathrm{cm}}^{3}cm3 for the 4 2^{2}2S1/2{\mathit{S}}_{1/2}S1/2​\ensuremath{\leftrightarrows}4 2^{2}2P1/2{\mathit{P}}_{1/2}P1/2​ transition and where \ensuremath{\beta}=-3.0\ifmmode\times\else\texttimes\fi{}${10}^{\mathrm{\ensuremath{-}}8}$ ${\mathrm{sec}}^{\mathrm{\ensuremath{-}}1}$ cm3{\mathrm{cm}}^{3}cm3 for the 4 2^{2}2S1/2{\mathit{S}}_{1/2}S1/2​\ensuremath{\leftrightarrows}4 2^{2}2S1/2{\mathit{S}}_{1/2}S1/2​\ensuremath{\leftrightarrows}4 2^{2}2P3/2{\mathit{P}}_{3/2}P3/2​ transition.
We study the dipole–dipole spectral broadening of a resonance line at high atomic densities when the self-broadening dominates. The selective reflection spectrum of a weak probe beam from the interface of the cell window and rubidium vapour is recorded in the presence of a far-detuned pump beam. The excitation due to the pump reduces the self-broadening. We found that the self-broadening reduction dependence on the pump power is atomic density independent. These results provide experimental evidence for the disordered exciton based theory of self-broadening, and can be useful for the description of the interaction of a strong optical field with a dense resonance medium.
Abstract Coherent narrow resonances in a homogeneously broadened contour of selective reflection from the interface between a cell window and high-density atomic rubidium vapor, where the dipole broadening greatly exceeds the Doppler width of the unresolved components of rubidium D2 line, are discussed. The formation of coherent resonances is caused by the coherent scattering of probe and pump optical fields from the oscillations of populations of the ground and excited states of atoms at the beat frequency. The width of each resonance depends on the population difference decay rate. Within a simple model conditions are found for observing resonances with a Lorentzian spectral profile. The experimentally recorded coherent resonances are described by a Lorentz function with fitting parameters in the form of amplitude, width, and spectral baseline. In the limit of zero optical saturation the measured half-width of a coherent resonance (HWHM) γres/2π is about 52 MHz, which greatly exceeds the radiative decay rate of the rubidium excited state 5P3/2.