In molecule optics, a matter wave of molecules is manipulated by a molecule-optical component made out of external, typically radiative, fields. The molecule-optical index of refraction, n, for a nonresonant IR laser pulse focused onto a molecular beam can be obtained from the energy conservation and wave properties of molecules. Experimentally measured values of n for benzene and nitric oxide agreed well with the calculated values. Since n depends on the properties of molecules as well as those of the laser field, a molecule prism composed of the focused nonresonant laser field can separate a multi-component molecular beam into several components according to their molecule-optical refractive indices n. We obtained a chromatographic resolution of 0.62 for the spatial separation of a mixture beam of benzene and nitric oxide using a focused Nd:YAG laser pulse as a molecule prism.In molecule optics, a matter wave of molecules is manipulated by a molecule-optical component made out of external, typically radiative, fields. The molecule-optical index of refraction, n, for a nonresonant IR laser pulse focused onto a molecular beam can be obtained from the energy conservation and wave properties of molecules. Experimentally measured values of n for benzene and nitric oxide agreed well with the calculated values. Since n depends on the properties of molecules as well as those of the laser field, a molecule prism composed of the focused nonresonant laser field can separate a multi-component molecular beam into several components according to their molecule-optical refractive indices n. We obtained a chromatographic resolution of 0.62 for the spatial separation of a mixture beam of benzene and nitric oxide using a focused Nd:YAG laser pulse as a molecule prism.

The Journal of Chemical PhysicsOct 24, 200338 citations

Optics and Interferometry with Na2 Molecules

Michael Chapman, Christopher R. Ekstrom, Troy D. Hammond +4 more

We have produced an intense, pure beam of sodium molecules ( ${\mathrm{Na}}_{2}$ ) by using light forces to separate the atomic and molecular species in a seeded supersonic beam. We used diffraction from a microfabricated grating to study the atomic and molecular sodium in the beam. Using three of these gratings, we constructed a molecule interferometer with fully separated beams and high contrast fringes. We measured both the real and imaginary parts of the index of refraction of neon gas for ${\mathrm{Na}}_{2}$ molecule de Broglie waves by inserting a gas cell in one arm of the interferometer.We have produced an intense, pure beam of sodium molecules ( ${\mathrm{Na}}_{2}$) by using light forces to separate the atomic and molecular species in a seeded supersonic beam. We used diffraction from a microfabricated grating to study the atomic and molecular sodium in the beam. Using three of these gratings, we constructed a molecule interferometer with fully separated beams and high contrast fringes. We measured both the real and imaginary parts of the index of refraction of neon gas for ${\mathrm{Na}}_{2}$ molecule de Broglie waves by inserting a gas cell in one arm of the interferometer.

Physical Review LettersJun 12, 1995146 citations

Refraction at the atomic level

Phil F. Schewe

Physics TodayJan 1, 20030 citations

Realization of phase dependent optical bistability in a quantum dot molecule via three-wave mixing

Donghui Wang

Abstract In this paper, we have proposed a new model based on the electron tunneling effect for controlling the optical bistability (OB) and optical multistability (OM) in a defect slab structure with a quantum dot molecule (QDM). Due to the presence of the electron tunneling effect, an additional weak signal beam can be generated in the system which makes the medium becomes phase dependent. We have studied the refractive index properties of the QDM via optical susceptibility of the propagated probe light. We have discussed the relative phase effect on negative refractive index (NRI) of the QDM nanostructure due to presence of electron tunneling. Then, by using the transfer matrix method, we have studied the transmission coefficient for NRI of the QDM nanostructure. Then, we have investigated the properties of transmitted light versus incident light for realizing the OB and OM. We have considered the relative phase effect on OB and OM properties of the transmitted beam and find that the switching between them is possible when electron tunneling is present in the quantum dot. Moreover, the optical thickness of the defect layer is also investigated on OB and OM in resonance and non-resonance conditions.Abstract In this paper, we have proposed a new model based on the electron tunneling effect for controlling the optical bistability (OB) and optical multistability (OM) in a defect slab structure with a quantum dot molecule (QDM). Due to the presence of the electron tunneling effect, an additional weak signal beam can be generated in the system which makes the medium becomes phase dependent. We have studied the refractive index properties of the QDM via optical susceptibility of the propagated probe light. We have discussed the relative phase effect on negative refractive index (NRI) of the QDM nanostructure due to presence of electron tunneling. Then, by using the transfer matrix method, we have studied the transmission coefficient for NRI of the QDM nanostructure. Then, we have investigated the properties of transmitted light versus incident light for realizing the OB and OM. We have considered the relative phase effect on OB and OM properties of the transmitted beam and find that the switching between them is possible when electron tunneling is present in the quantum dot. Moreover, the optical thickness of the defect layer is also investigated on OB and OM in resonance and non-resonance conditions.

Laser Physics LettersAug 9, 20224 citations

Molecular optics

Mariangela Gussoni, Chiara Castiglioni, M. Del Zoppo +1 more

Elsevier eBooksJan 1, 19933 citations

We have produced an intense, pure beam of sodium molecules (

{\mathrm{Na}}_{2}

) by using light forces to separate the atomic and molecular species in a seeded supersonic beam. We used diffraction from a microfabricated grating to study the atomic and molecular sodium in the beam. Using three of these gratings, we constructed a molecule interferometer with fully separated beams and high contrast fringes. We measured both the real and imaginary parts of the index of refraction of neon gas for

{\mathrm{Na}}_{2}

molecule de Broglie waves by inserting a gas cell in one arm of the interferometer.