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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

Spatiotemporal dynamics of Raman coherence in hydrogen-filled hollow core photonic crystal fibers

Anton Husakou, Yingying Wang, Brian J. Mangan, Fetah Benabid

Published May 1, 2011• 0 citations
Publisher

Abstract

The sidebands of stimulated Raman scattering initiated from vacuum fluctuations in hollow-core photonic crystal fiber filled with Raman gas exhibit surprisingly strong self- and mutual coherence [1] as well as persistence of coherence for much longer than the dephasing time T2[2]. This opens new prospects in a number of applications such as attosecond pulse generation and optical waveform synthesis. However, the spatiotemporal coherence dynamics underlying these results is not fully investigated and no rigorous theoretical simulation is available. This contribution discusses theoretical and experimental results that study this issue and explains the long-lived effect of the coherence on a delayed probe pulse in the pump-probe setup.

DOI
10.1109/cleoe.2011.5942710

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•May 7, 2018•10 citations
The sidebands of stimulated Raman scattering initiated from vacuum fluctuations in hollow-core photonic crystal fiber filled with Raman gas exhibit surprisingly strong self- and mutual coherence [1] as well as persistence of coherence for much longer than the dephasing time T2[2]. This opens new prospects in a number of applications such as attosecond pulse generation and optical waveform synthesis. However, the spatiotemporal coherence dynamics underlying these results is not fully investigated and no rigorous theoretical simulation is available. This contribution discusses theoretical and experimental results that study this issue and explains the long-lived effect of the coherence on a delayed probe pulse in the pump-probe setup.
We present the results of an experimental and numerical investigation into temporally nonlocal coherent interactions between ultrashort pulses, mediated by Raman coherence, in a gas-filled kagome-style hollow-core photonic-crystal fiber. A pump pulse first sets up the Raman coherence, creating a refractive index spatiotemporal grating in the gas that travels at the group velocity of the pump pulse. Varying the arrival time of a second, probe, pulse allows a high degree of control over its evolution as it propagates along the fiber through the grating. Of particular interest are soliton-driven effects such as self-compression and dispersive wave (DW) emission. In the experiments reported, a DW is emitted at $\ensuremath{\sim}300\phantom{\rule{0.16em}{0ex}}\mathrm{nm}$ and exhibits a wiggling effect, with its central frequency oscillating periodically with pump-probe delay. The results demonstrate that a strong Raman coherence, created in a broadband guiding gas-filled kagome photonic-crystal fiber, can be used to control the nonlinear dynamics of ultrashort probe pulses, even in difficult-to-access spectral regions such as the deep and vacuum ultraviolet.
We present an experimental and theoretical study of the stimulated Raman emission in hollow-core kagome waveguides in a pump-probe arrangement. We perform an experimental investigation of the power of the Stokes signal from the probe, which is below the stimulated Raman scattering threshold, as a function the pump-probe delay time. The results show the Stokes power to increase with pump-probe delay, reaching a maximum at 10 ns, and to decrease afterward. In view of a coherence decay time of only 0.25 ns, we demonstrate a surprisingly slow reduction of Stokes signal with the characteristic time much longer than the coherence decay time by a factor of up to 40. The numerical investigations explain the observed phenomenon as a result of the spatiotemporal dynamics of the probe pulse and Raman coherence. We show that the increase of the characteristic time can be related to the spatial position of the intense sideband generation event and its dependence on the pump-probe delay.
Stimulated Raman scattering is investigated in a slightly multimode gas-filled hollow-core photonic crystal fiber. Although, second-order Stokes light appears in the fundamental mode below a certain threshold energy, it is observed to switch to a two-lobed higher order mode above this threshold. Conversion to the higher order mode is made possible by the creation of a two-lobed moving coherence wave in the gas that provides both phase-matching and a strong intermodal pump-Stokes overlap. A theoretical model is developed, based on this physical interpretation that agrees quantitatively with the experimental results. The results suggest new opportunities for all-fiber gas-based nonlinear processes requiring phase-matching, such as coherent anti-Stokes Raman scattering, as well as providing a means (for example) of efficiently converting light from a higher order pump mode to a fundamental Stokes mode.
Backward stimulated Raman scattering in gases provides a promising route to the compression and amplification of a Stokes seed pulse by counter-propagating against a pump pulse, as has been demonstrated already in various platforms, mainly in free space. However, the dynamics governing this process when seeded by noise has not yet been investigated in a fully controllable collinear environment. Here we report, to the best of our knowledge, the first unambiguous observation of efficient noise-seeded backward stimulated Raman scattering in a hydrogen-filled hollow-core photonic crystal fiber. At high gas pressures, when the backward Raman gain is comparable to, but lower than, the forward gain, we report quantum conversion efficiencies exceeding 40% to the backward Stokes at 683 nm from a narrowband 532 nm pump. Efficiency increases to 65% when the backward process is seeded by a small amount of back-reflected forward-generated Stokes light. At high pump powers, the backward Stokes signal, emitted in a clean fundamental mode and spectrally pure, is unexpectedly always stronger than its forward-propagating counterpart. We attribute this striking observation to the unique temporal dynamics of the interacting fields, which cause the Raman coherence (which takes the form of a moving fine-period Bragg grating) to grow in strength toward the input end of the fiber. A good understanding of this process, together with the rapid development of novel anti-resonant-guiding hollow-core fibers, may lead to improved designs of efficient gas-based Raman lasers and amplifiers operating at wavelengths from the ultraviolet to the mid-infrared.