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IEEE Journal of Quantum Electronics

Intracavity optical bistability due to thermally induced changes in absorption and refraction

M. Dagenais, Alisa Surkis, Wayne F. Sharfin, Herbert G. Winful

Published Sep 1, 1985• 10 citations
Publisher

Abstract

Optical bistability in the presence of an optically induced absorption is observed when a thin 13 μm CdS sample is inserted between two mirrors of 90 percent reflectivity. In our experiment, a modulated CW laser of about 15 mW peak power is tuned on each side of theAfree exciton resonance in CdS, and the transmission characteristics are studied. A theoretical calculation is presented and good agreement is obtained.

DOI
10.1109/jqe.1985.1072817

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Applied Physics Letters•Dec 15, 1983•105 citations
Optical bistability in the presence of an optically induced absorption is observed when a thin 13 μm CdS sample is inserted between two mirrors of 90 percent reflectivity. In our experiment, a modulated CW laser of about 15 mW peak power is tuned on each side of theAfree exciton resonance in CdS, and the transmission characteristics are studied. A theoretical calculation is presented and good agreement is obtained.
Optical bistability in the presence of an optically induced absorption is observed when a thin 13-μm CdS sample is inserted between two mirrors of 90 % reflectivity, in our experiment, a modulated cw laser of ~15-mW peak power is tuned on each side of the free exciton resonance in CdS, and the transmission characteristics are studied. A theoretical calculation including both absorptive and dispersive effects is presented and good agreement is obtained. The absorption coefficient and the index of refraction of the material are connected by Kramers-Kronig relations. Propagation effects are taken into account. Sufficiently long pulses (40 ms) are considered to allow the thermally induced absorption to occur. For detunings above the free exciton resonance, we predict that counterclockwise hysteresis loops will first be observed as the intensity rises; for detunings below the free exciton resonance, only clockwise hysteresis loops are predicted. These predictions were experimentally verified. Power levels of the order of 5–10 mW were sufficient to observe bistability. Cavity effects were also observed.
We report the observation of an intensity-dependent refractive-index nonlinearity in CdS due to a resonance state where an excitonic molecule is created by induced absorption of light. The refractive indexnas a function of the incident laser photon energyEis measured directly by light refraction in thin crystal prisms. A renormalized dielectric function describes the measuredn(E)spectra well. This strong refractive-index nonlinearity is well suited to produce an optical bistability and to further strengthen the evidence of CdS to be an important material for laser-induced dynamic gratings.
Abstract Thermally induced dispersive and absorptive optical bistability of CdS is investigated in a temperature range of 20 K to RT. The influence of the geometry of the crystals, e. g., thickness, surface area size, and resonator structure, on the hysteresis feature and switching behavior is investigated. The quality of the thermal contact between the sample and the heat sink strongly influences switch‐back times. Further, starting temperature, light spot diameter, and pulse intensity are varied in order to find a set of optimization criteria for this kind of optical bistability. Experimental results are in good agreement with model calculations.