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Physical Review A

Electric field enhancement of depolarization of excited states

Munir Hasan Nayfeh, G. Barry Hillard, Wallace L. Glab

Published Dec 1, 1985• 2 citations
Publisher

Abstract

Our calculations show that an external dc electric field can enhance by many orders of magnitude the depolarization cross section of highly excited atoms by charged particles. The enhancement is due to the fact that the electric field extends and shifts the electronic charge distribution along its direction, thus effectively creating a giant electric dipole in the atom.

DOI
10.1103/physreva.32.3324

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Electric-field modification of two-photon, two-color, quadrupole-dipole depolarization spectra in atomic Cs

B. V. Dobrydnev, Mark D. Havey

An earlier study of the 6s${\mathrm{}}^{2}$${\mathit{S}}_{1/2}$\ensuremath{\rightarrow}5d${\mathrm{}}^{2}$${\mathit{D}}_{\mathit{j}}$\ensuremath{\rightarrow}11p${\mathrm{}}^{2}$${\mathit{P}}_{3/2}$ two-photon, dipole-quadrupole transition in Cs is extended by including the effect of an external static electric field. The dependence of the absorption spectrum on the relative polarizations of the two light sources is found to be greatly modified by a moderately sized electric field, the predominant effect being mixing of the resonant 6p${\mathrm{}}^{2}$${\mathit{P}}_{\mathit{j}}$ levels into the ground 6s${\mathrm{}}^{2}$${\mathit{S}}_{1/2}$ level. Compact theoretical expressions, parametrized in terms of the electric-field strength and the relative transition matrix elements through the 5d${\mathrm{}}^{2}$${\mathit{D}}_{\mathit{j}}$ multiplet levels, are given. Results are presented for the electric-field dependence of a linear depolarization ratio, which is very sensitive to these quantities. \textcopyright{} 1996 The American Physical Society.

Physical Review A•Nov 1, 1996•2 citations
Our calculations show that an external dc electric field can enhance by many orders of magnitude the depolarization cross section of highly excited atoms by charged particles. The enhancement is due to the fact that the electric field extends and shifts the electronic charge distribution along its direction, thus effectively creating a giant electric dipole in the atom.
In this article, the atom excitation suppression is studied in two mechanisms. The first mechanism for excitation suppression is caused by an external DC electric field. The second mechanism is due to the energy shift caused by an electric field generated by free charges, which are created by ionizing atoms. The latter mechanism is known as the Coulomb blockade. Here, the Coulomb forces originate from ions created by ionizing atoms with a UV laser. The interaction, which causes the suppression, is treated theoretically as dipole–charge interactions. In the model, the charge is an ion, and the dipole is an atom. From measurements, we use 85Rb atoms. The valence electron and the ion core are the two poles of an electric dipole. The interaction potential energy between the ion and the atom is proportional to 1R2, and the frequency shift caused by this interaction is proportional to 1R4, where R is the distance between the ion and the dipole considered. This research is motivated by potential applications for quantum information storage, remote control, creating hot plasmas using cold atoms, as well as electronic devices.
A resonance, induced by a DC field in a two-photon transition of an atom between states with opposite parity, results in a number of new effects related to the polarization of photons. These effects are caused by the interference of the non-resonant second-order dipole-forbidden amplitude and of a resonant part of the DC field-induced third-order amplitude. The linear and circular dichroism for the cross section of the process is revealed and analysed in detail for a two-photon excitation of the state from the ground state with a resonance on an state, induced by a DC electric field. The numerical data for alkali atoms demonstrate that the effects have quantitative characteristics of sufficiently large magnitudes and may be observed in experiments.
An earlier study of the 6s2{\mathrm{}}^{2}2S1/2{\mathit{S}}_{1/2}S1/2​\ensuremath{\rightarrow}5d2{\mathrm{}}^{2}2Dj{\mathit{D}}_{\mathit{j}}Dj​\ensuremath{\rightarrow}11p2{\mathrm{}}^{2}2P3/2{\mathit{P}}_{3/2}P3/2​ two-photon, dipole-quadrupole transition in Cs is extended by including the effect of an external static electric field. The dependence of the absorption spectrum on the relative polarizations of the two light sources is found to be greatly modified by a moderately sized electric field, the predominant effect being mixing of the resonant 6p2{\mathrm{}}^{2}2Pj{\mathit{P}}_{\mathit{j}}Pj​ levels into the ground 6s2{\mathrm{}}^{2}2S1/2{\mathit{S}}_{1/2}S1/2​ level. Compact theoretical expressions, parametrized in terms of the electric-field strength and the relative transition matrix elements through the 5d2{\mathrm{}}^{2}2Dj{\mathit{D}}_{\mathit{j}}Dj​ multiplet levels, are given. Results are presented for the electric-field dependence of a linear depolarization ratio, which is very sensitive to these quantities. \textcopyright{} 1996 The American Physical Society.