Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Physical Review A

Low-intensity limit of the laser cooling of a multistate atom

Sung Mi Yoo, Juha Javanainen

Published Mar 1, 1992• 22 citations
Publisher

Abstract

We adapt an earlier semiclassical theory of laser cooling of an arbitrary multistate atom [J. Javanainen, Phys. Rev. A 44, 5857 (1991)] to the limit of low light intensity. The formal theory is implemented analytically on a computer using mathematica. Expressions of light-pressure force and diffusion are provided for ${\mathit{j}}_{1}$=1/2\ensuremath{\rightarrow}${\mathit{j}}_{2}$=3/2 and ${\mathit{j}}_{1}$=1\ensuremath{\rightarrow}${\mathit{j}}_{2}$=2 atoms in a one-dimensional optical confinement area in which the pair of counterpropagating waves has orthogonal polarizations. In our models the cooling temperature decreases as the level degeneracy increases.

DOI
10.1103/physreva.45.3071

Related papers

Numerical experiments in semiclassical laser-cooling theory of multistate atoms

Juha Javanainen

We describe a numerical implementation of our semiclassical laser-cooling theory [J. Javanainen, Phys. Rev. A 44, 5857 (1991)] for an arbitrary multilevel atom and light field. There is satisfactory agreement between experiments and temperatures obtained from Langevin-equation simulations of the motion of an atom subject to light-pressure force and the accompanying diffusion in three-dimensional (3D) optical molasses in which there are three orthogonal pairs of counterpropagating waves with a common linear polarization for the two beams in a pair, but orthogonal polarizations between the pairs. However, the velocity distribution of the atoms is anisotropic and may deviate strongly from a Gaussian, heterodyne spectra may have a sideband, and the atomic density may be a maximum at the maximum of the potential of the dipole forces of the molasses beams. Subsequent velocity-linearized analysis of atomic damping and diffusion shows that the damping tensor may have a negative eigenvalue corresponding to heating in large regions of space, even though the light is red tuned for cooling. It is also found that the position-averaged damping and diffusion tensors make a poor predictor of the temperature obtained in Langevin-equation simulations and real experiments. Based on additional simulations of a simple 1D model, we formulate a hypothesis that connects our findings. The key idea is that an atom trapped in a minimum of the potential of the dipole forces is subject to a weaker-than-average damping, and therefore tends to boil out of the trap.

Physical Review A•Nov 1, 1992•54 citations

Laser cooling theory of multistate atoms

Juha Javanainen

In the limit of asymptotically small photon momentum, a Fokker–Planck equation for the center-of-mass Wigner function suffices to describe laser cooling of an atom. We have devised a procedure to compute the light pressure force and the diffusion tensor for an atom with an arbitrary level structure, traveling with an arbitrary velocity in any given three-dimensional light field. The scheme is based on solving a set of differential equations closely related to the density matrix equations of motion encountered in conventional recoilless laser spectroscopy. Computer programs have been written that automatically construct and solve the required equations from broad specifications of the problem, such as energies and angular momenta of the atomic levels. A Langevin equation stochastic simulation has been implemented to solve the Fokker-Planck equation of laser cooling using the computed force and diffusion. Comparisons of optical-molasses experiments and simulations carried out for a model sodium atom with a J = 2→J = 3 transition show qualitative similarities such as sub-Doppler limit temperatures, but the quantitative agreement of theory and experiment is not satisfactory.

Annual Meeting Optical Society of America•Jan 1, 1990•0 citations

Semiclassical laser-cooling theory for a trapped multistate ion

Juha Javanainen, Sung Mi Yoo

We present a semiclassical laser-cooling theory for an ion bound in a quadratic potential well, allowing for an arbitrary internal level scheme of the ion and an arbitrary polarization of the light field. The special case that the ion moves in a region much smaller than the wavelength of the exciting light (Lamb-Dicke limit), as well as an additional low-intensity limit, are worked out in detail. Explicit general expressions are given for the damping and diffusion tensors of the center-of-mass motion of the ion, and the light-induced renormalization of the mechanical oscillation frequencies is discussed. The formalism is implemented analytically using a computer program mathematica for an ion with a j=1/2\ensuremath{\rightarrow}j=3/2 transition moving in a one-dimensional optical molasses consisting of two counterpropagating laser beams with perpendicular linear polarizations (lin \ensuremath{\perp} lin). For a weakly bound ion at negligible saturation, the greatest lower limit of excitation energy turns out to be (33/20${)}^{1/2}$-1/2\ensuremath{\approxeq}0.78 vibrational quanta above the zero-point energy.

Physical Review A•Nov 1, 1993•8 citations

One-dimensional laser cooling below the Doppler limit

Vladimir Finkelstein, P. R. Berman, Jingzhong Guo

A theoretical analysis is given for one-dimensional laser cooling below the Doppler limit of J=1/2 ground-state atoms. The laser field consists of a pair of counterpropagating, linearly polarized, low-power beams, whose polarization directions differ by an angle \ensuremath{\theta} (0\ensuremath{\le}\ensuremath{\theta}\ensuremath{\le}\ensuremath{\pi}/2). For \ensuremath{\theta}\ensuremath{\ll}1, the effective optical-pumping time is shown to increase strongly near the nodes of the standing wave, and the cooling force can be much larger than that for \ensuremath{\theta}=\ensuremath{\pi}/2. Moreover, for \ensuremath{\theta}\ensuremath{\ll}1, it can be shown that the stimulated part of the atomic diffusion is reduced considerably as compared with that for \ensuremath{\theta}=\ensuremath{\pi}/2. As a consequence it is possible to achieve an equilibrium atomic distribution that, for \ensuremath{\theta}\ensuremath{\ll}1, is characterized by a mean kinetic energy that is lower than that predicted to occur for \ensuremath{\theta}=\ensuremath{\pi}/2. The equilibrium velocity distribution is not necessarily Maxwellian, and thus the temperature of the atomic ensemble may not be well defined. The achievable kinetic energy is so small that the cooled atoms may be trapped in the vicinity of the laser-field nodes.

Physical Review A•Feb 1, 1992•48 citations

Laser cooling below the Doppler limit by polarization gradients: simple theoretical models

Jean Dalibard, Claude N. Cohen-Tannoudji

We present two cooling mechanisms that lead to temperatures well below the Doppler limit. These mechanisms are based on laser polarization gradients and work at low laser power when the optical-pumping time between different ground-state sublevels becomes long. There is then a large time lag between the internal atomic response and the atomic motion, which leads to a large cooling force. In the simple case of one-dimensional molasses, we identify two types of polarization gradient that occur when the two counterpropagating waves have either orthogonal linear polarizations or orthogonal circular polarizations. In the first case, the light shifts of the ground-state Zeeman sublevels are spatially modulated, and optical pumping among them leads to dipole forces and to a Sisyphus effect analogous to the one that occurs in stimulated molasses. In the second case (σ+−σ− configuration), the cooling mechanism is radically different. Even at very low velocity, atomic motion produces a population difference among ground-state sublevels, which gives rise to unbalanced radiation pressures. From semiclassical optical Bloch equations, we derive for the two cases quantitative expressions for friction coefficients and velocity capture ranges. The friction coefficients are shown in both cases to be independent of the laser power, which produces an equilibrium temperature proportional to the laser power. The lowest achievable temperatures then approach the one-photon recoil energy. We briefly outline a full quantum treatment of such a limit.

Journal of the Optical Society of America B•Nov 1, 1989•1,272 citations

Operator description of laser cooling below the Doppler limit

Gerard Nienhuis, P. van der Straten, S-Q. Shang

We give a general theoretical description of radiative forces on atoms in a monochromatic radiation field. The driven transition has a lower level consisting of several substates, and we consider the limit of low velocities and weak intensities. This situation comprises the schemes where cooling to temperatures below the Doppler limit is possible. After expressing the atomic dipole in terms of the polarizability tensor, we obtain an expression of the force as the sum of the radiation pressure, the dipole force, and a contribution from the gradient of the polarization. This latter contribution contains a part resulting from redistribution of photons between the plane waves that compose the field, and a part resulting from fluorescence. We express the average force and the momentum-diffusion tensor in terms of a closed evolution equation for the lower-state density matrix. We show by a scaling argument that in any case of cooling, the final temperature goes down linearly with the intensity, until the recoil limit is approached. The description is valid for a weak and monochromatic, but otherwise arbitrary field, and it allows for the presence of an external magnetic field, and of hyperfine splitting. It is applicable to cooling in one, two, or three dimensions. We give numerical results for the average force in a number of specific cases of two counterrunning plane waves.

Physical Review A•Jul 1, 1991•81 citations
We adapt an earlier semiclassical theory of laser cooling of an arbitrary multistate atom [J. Javanainen, Phys. Rev. A 44, 5857 (1991)] to the limit of low light intensity. The formal theory is implemented analytically on a computer using mathematica. Expressions of light-pressure force and diffusion are provided for j1{\mathit{j}}_{1}j1​=1/2\ensuremath{\rightarrow}j2{\mathit{j}}_{2}j2​=3/2 and j1{\mathit{j}}_{1}j1​=1\ensuremath{\rightarrow}j2{\mathit{j}}_{2}j2​=2 atoms in a one-dimensional optical confinement area in which the pair of counterpropagating waves has orthogonal polarizations. In our models the cooling temperature decreases as the level degeneracy increases.
We describe a numerical implementation of our semiclassical laser-cooling theory [J. Javanainen, Phys. Rev. A 44, 5857 (1991)] for an arbitrary multilevel atom and light field. There is satisfactory agreement between experiments and temperatures obtained from Langevin-equation simulations of the motion of an atom subject to light-pressure force and the accompanying diffusion in three-dimensional (3D) optical molasses in which there are three orthogonal pairs of counterpropagating waves with a common linear polarization for the two beams in a pair, but orthogonal polarizations between the pairs. However, the velocity distribution of the atoms is anisotropic and may deviate strongly from a Gaussian, heterodyne spectra may have a sideband, and the atomic density may be a maximum at the maximum of the potential of the dipole forces of the molasses beams. Subsequent velocity-linearized analysis of atomic damping and diffusion shows that the damping tensor may have a negative eigenvalue corresponding to heating in large regions of space, even though the light is red tuned for cooling. It is also found that the position-averaged damping and diffusion tensors make a poor predictor of the temperature obtained in Langevin-equation simulations and real experiments. Based on additional simulations of a simple 1D model, we formulate a hypothesis that connects our findings. The key idea is that an atom trapped in a minimum of the potential of the dipole forces is subject to a weaker-than-average damping, and therefore tends to boil out of the trap.
In the limit of asymptotically small photon momentum, a Fokker–Planck equation for the center-of-mass Wigner function suffices to describe laser cooling of an atom. We have devised a procedure to compute the light pressure force and the diffusion tensor for an atom with an arbitrary level structure, traveling with an arbitrary velocity in any given three-dimensional light field. The scheme is based on solving a set of differential equations closely related to the density matrix equations of motion encountered in conventional recoilless laser spectroscopy. Computer programs have been written that automatically construct and solve the required equations from broad specifications of the problem, such as energies and angular momenta of the atomic levels. A Langevin equation stochastic simulation has been implemented to solve the Fokker-Planck equation of laser cooling using the computed force and diffusion. Comparisons of optical-molasses experiments and simulations carried out for a model sodium atom with a J = 2→J = 3 transition show qualitative similarities such as sub-Doppler limit temperatures, but the quantitative agreement of theory and experiment is not satisfactory.
We present a semiclassical laser-cooling theory for an ion bound in a quadratic potential well, allowing for an arbitrary internal level scheme of the ion and an arbitrary polarization of the light field. The special case that the ion moves in a region much smaller than the wavelength of the exciting light (Lamb-Dicke limit), as well as an additional low-intensity limit, are worked out in detail. Explicit general expressions are given for the damping and diffusion tensors of the center-of-mass motion of the ion, and the light-induced renormalization of the mechanical oscillation frequencies is discussed. The formalism is implemented analytically using a computer program mathematica for an ion with a j=1/2\ensuremath{\rightarrow}j=3/2 transition moving in a one-dimensional optical molasses consisting of two counterpropagating laser beams with perpendicular linear polarizations (lin \ensuremath{\perp} lin). For a weakly bound ion at negligible saturation, the greatest lower limit of excitation energy turns out to be (33/20)1/2{)}^{1/2})1/2-1/2\ensuremath{\approxeq}0.78 vibrational quanta above the zero-point energy.
A theoretical analysis is given for one-dimensional laser cooling below the Doppler limit of J=1/2 ground-state atoms. The laser field consists of a pair of counterpropagating, linearly polarized, low-power beams, whose polarization directions differ by an angle \ensuremath{\theta} (0\ensuremath{\le}\ensuremath{\theta}\ensuremath{\le}\ensuremath{\pi}/2). For \ensuremath{\theta}\ensuremath{\ll}1, the effective optical-pumping time is shown to increase strongly near the nodes of the standing wave, and the cooling force can be much larger than that for \ensuremath{\theta}=\ensuremath{\pi}/2. Moreover, for \ensuremath{\theta}\ensuremath{\ll}1, it can be shown that the stimulated part of the atomic diffusion is reduced considerably as compared with that for \ensuremath{\theta}=\ensuremath{\pi}/2. As a consequence it is possible to achieve an equilibrium atomic distribution that, for \ensuremath{\theta}\ensuremath{\ll}1, is characterized by a mean kinetic energy that is lower than that predicted to occur for \ensuremath{\theta}=\ensuremath{\pi}/2. The equilibrium velocity distribution is not necessarily Maxwellian, and thus the temperature of the atomic ensemble may not be well defined. The achievable kinetic energy is so small that the cooled atoms may be trapped in the vicinity of the laser-field nodes.
We present two cooling mechanisms that lead to temperatures well below the Doppler limit. These mechanisms are based on laser polarization gradients and work at low laser power when the optical-pumping time between different ground-state sublevels becomes long. There is then a large time lag between the internal atomic response and the atomic motion, which leads to a large cooling force. In the simple case of one-dimensional molasses, we identify two types of polarization gradient that occur when the two counterpropagating waves have either orthogonal linear polarizations or orthogonal circular polarizations. In the first case, the light shifts of the ground-state Zeeman sublevels are spatially modulated, and optical pumping among them leads to dipole forces and to a Sisyphus effect analogous to the one that occurs in stimulated molasses. In the second case (σ+−σ− configuration), the cooling mechanism is radically different. Even at very low velocity, atomic motion produces a population difference among ground-state sublevels, which gives rise to unbalanced radiation pressures. From semiclassical optical Bloch equations, we derive for the two cases quantitative expressions for friction coefficients and velocity capture ranges. The friction coefficients are shown in both cases to be independent of the laser power, which produces an equilibrium temperature proportional to the laser power. The lowest achievable temperatures then approach the one-photon recoil energy. We briefly outline a full quantum treatment of such a limit.
We give a general theoretical description of radiative forces on atoms in a monochromatic radiation field. The driven transition has a lower level consisting of several substates, and we consider the limit of low velocities and weak intensities. This situation comprises the schemes where cooling to temperatures below the Doppler limit is possible. After expressing the atomic dipole in terms of the polarizability tensor, we obtain an expression of the force as the sum of the radiation pressure, the dipole force, and a contribution from the gradient of the polarization. This latter contribution contains a part resulting from redistribution of photons between the plane waves that compose the field, and a part resulting from fluorescence. We express the average force and the momentum-diffusion tensor in terms of a closed evolution equation for the lower-state density matrix. We show by a scaling argument that in any case of cooling, the final temperature goes down linearly with the intensity, until the recoil limit is approached. The description is valid for a weak and monochromatic, but otherwise arbitrary field, and it allows for the presence of an external magnetic field, and of hyperfine splitting. It is applicable to cooling in one, two, or three dimensions. We give numerical results for the average force in a number of specific cases of two counterrunning plane waves.