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Physical Review A

Operator description of laser cooling below the Doppler limit

Gerard Nienhuis, P. van der Straten, S-Q. Shang

Published Jul 1, 1991• 81 citations
Publisher

Abstract

We give a general theoretical description of radiative forces on atoms in a monochromatic radiation field. The driven transition has a lower level consisting of several substates, and we consider the limit of low velocities and weak intensities. This situation comprises the schemes where cooling to temperatures below the Doppler limit is possible. After expressing the atomic dipole in terms of the polarizability tensor, we obtain an expression of the force as the sum of the radiation pressure, the dipole force, and a contribution from the gradient of the polarization. This latter contribution contains a part resulting from redistribution of photons between the plane waves that compose the field, and a part resulting from fluorescence. We express the average force and the momentum-diffusion tensor in terms of a closed evolution equation for the lower-state density matrix. We show by a scaling argument that in any case of cooling, the final temperature goes down linearly with the intensity, until the recoil limit is approached. The description is valid for a weak and monochromatic, but otherwise arbitrary field, and it allows for the presence of an external magnetic field, and of hyperfine splitting. It is applicable to cooling in one, two, or three dimensions. We give numerical results for the average force in a number of specific cases of two counterrunning plane waves.

DOI
10.1103/physreva.44.462

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We give a general theoretical description of radiative forces on atoms in a monochromatic radiation field. The driven transition has a lower level consisting of several substates, and we consider the limit of low velocities and weak intensities. This situation comprises the schemes where cooling to temperatures below the Doppler limit is possible. After expressing the atomic dipole in terms of the polarizability tensor, we obtain an expression of the force as the sum of the radiation pressure, the dipole force, and a contribution from the gradient of the polarization. This latter contribution contains a part resulting from redistribution of photons between the plane waves that compose the field, and a part resulting from fluorescence. We express the average force and the momentum-diffusion tensor in terms of a closed evolution equation for the lower-state density matrix. We show by a scaling argument that in any case of cooling, the final temperature goes down linearly with the intensity, until the recoil limit is approached. The description is valid for a weak and monochromatic, but otherwise arbitrary field, and it allows for the presence of an external magnetic field, and of hyperfine splitting. It is applicable to cooling in one, two, or three dimensions. We give numerical results for the average force in a number of specific cases of two counterrunning plane waves.
We present two cooling mechanisms that lead to temperatures well below the Doppler limit. These mechanisms are based on laser polarization gradients and work at low laser power when the optical-pumping time between different ground-state sublevels becomes long. There is then a large time lag between the internal atomic response and the atomic motion, which leads to a large cooling force. In the simple case of one-dimensional molasses, we identify two types of polarization gradient that occur when the two counterpropagating waves have either orthogonal linear polarizations or orthogonal circular polarizations. In the first case, the light shifts of the ground-state Zeeman sublevels are spatially modulated, and optical pumping among them leads to dipole forces and to a Sisyphus effect analogous to the one that occurs in stimulated molasses. In the second case (σ+−σ− configuration), the cooling mechanism is radically different. Even at very low velocity, atomic motion produces a population difference among ground-state sublevels, which gives rise to unbalanced radiation pressures. From semiclassical optical Bloch equations, we derive for the two cases quantitative expressions for friction coefficients and velocity capture ranges. The friction coefficients are shown in both cases to be independent of the laser power, which produces an equilibrium temperature proportional to the laser power. The lowest achievable temperatures then approach the one-photon recoil energy. We briefly outline a full quantum treatment of such a limit.
In the limit of asymptotically small photon momentum, a Fokker–Planck equation for the center-of-mass Wigner function suffices to describe laser cooling of an atom. We have devised a procedure to compute the light pressure force and the diffusion tensor for an atom with an arbitrary level structure, traveling with an arbitrary velocity in any given three-dimensional light field. The scheme is based on solving a set of differential equations closely related to the density matrix equations of motion encountered in conventional recoilless laser spectroscopy. Computer programs have been written that automatically construct and solve the required equations from broad specifications of the problem, such as energies and angular momenta of the atomic levels. A Langevin equation stochastic simulation has been implemented to solve the Fokker-Planck equation of laser cooling using the computed force and diffusion. Comparisons of optical-molasses experiments and simulations carried out for a model sodium atom with a J = 2→J = 3 transition show qualitative similarities such as sub-Doppler limit temperatures, but the quantitative agreement of theory and experiment is not satisfactory.
We extend the kinetic theory of the laser cooling of atoms to four multilevel atomic schemes: (3+5)-, (5+7)-, (7+9)-, and (9+11)-level atom. In all four atomic schemes the atoms are considered to be excited by two counterpropagating circularly polarized laser waves. A comparison of four multilevel atomic schemes shows that the even-order multiphoton processes are responsible for the narrow structures near zero velocity in the atomic coherences, atomic populations, dipole radiation forces, and the diffusion coefficients. The even-order multiphoton processes in a multilevel atom with a big number of magnetic sublevels are shown to produce the velocity structures, which are much narrower than that produced by the two-photon processes in a (3+5)-level atom. It is found that the multiphoton processes enhance the radiation force at low velocities and the friction produced by the force at a negative detuning. The even-order multiphoton processes caused by the laser waves are identified as the basic physical mechanism responsible for the sub-Doppler laser cooling of atoms. The temperature of laser-cooled atoms is derived for all four models and found to be lower for atomic schemes with a larger number of magnetic sublevels.
A theoretical analysis is given for 1-D laser cooling below the Doppler limit of J = 1/2 ground- state atoms. The laser field consists of a pair of counterpropagating, linearly polarized low- power beams, whose polarization directions differ by an angle θ (0 ≤ θ ≤ π/2). For θ ≪ 1, the effective optical pumping time is shown to increase strongly near the nodes of the standing wave and the cooling force can be much larger than that for θ ~1. Moreover, for θ ≪ 1, it can be shown that the stimulated part of the atomic diffusion is reduced considerably as compared with that for θ ~ 1. As a consequence it is possible to achieve an equilibrium atomic distribution that, for θ ≪ 1, is characterized by a mean kinetic energy lower than that predicted to occur for θ = π/2. The equilibrium velocity distribution is not necessarily Maxwellian and thus the temperature of the atomic ensemble may not be well defined. The achievable kinetic energy is so small that the cooled atoms are trapped in the vicinity of the laser field nodes. An explanation for these effects is given in terms of Sisyphus cooling.
A theoretical analysis is given for one-dimensional laser cooling below the Doppler limit of J=1/2 ground-state atoms. The laser field consists of a pair of counterpropagating, linearly polarized, low-power beams, whose polarization directions differ by an angle \ensuremath{\theta} (0\ensuremath{\le}\ensuremath{\theta}\ensuremath{\le}\ensuremath{\pi}/2). For \ensuremath{\theta}\ensuremath{\ll}1, the effective optical-pumping time is shown to increase strongly near the nodes of the standing wave, and the cooling force can be much larger than that for \ensuremath{\theta}=\ensuremath{\pi}/2. Moreover, for \ensuremath{\theta}\ensuremath{\ll}1, it can be shown that the stimulated part of the atomic diffusion is reduced considerably as compared with that for \ensuremath{\theta}=\ensuremath{\pi}/2. As a consequence it is possible to achieve an equilibrium atomic distribution that, for \ensuremath{\theta}\ensuremath{\ll}1, is characterized by a mean kinetic energy that is lower than that predicted to occur for \ensuremath{\theta}=\ensuremath{\pi}/2. The equilibrium velocity distribution is not necessarily Maxwellian, and thus the temperature of the atomic ensemble may not be well defined. The achievable kinetic energy is so small that the cooled atoms may be trapped in the vicinity of the laser-field nodes.
It is conventional to describe the motion of an atom in a laser field (and other D.C fields) by a Fokker-Planck equation which is characterized by a force and a diffusion coefficient. Gordon and Ashkin have obtained a result for the diffusion coefficient in a spherically symmetric approximation. We have recently treated it as a second order tensor and have gotten a different result. The tensor has three terms. The leading term arises from the recoil of the atom during fluorescence, the second comes from gradients of the laser intensity and the D.C. fields and the last comes from a combination of the recoil term and gradients. The trace of our leading term agrees with the result of Gordon and Ashkin but there is no agreement at all with the other terms. The calculation was performed for a traveling wave laser and is being extended now to a standing wave laser by a graduate student. The experiment being undertaken here will use a swept laser frequency to compensate for the change in resonance frequency (due to the Doppler effect) of the atom as it slows down.