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Journal of Physics C Solid State Physics

On the dynamic structure factor in one-dimensional Heisenberg magnets

H.-J. Mikeska, W. Pesch

Published Jan 14, 1979• 4 citations
Publisher

Abstract

The authors have evaluated an expression obtained previously for the dynamical spin correlation function of a linear Heisenberg antiferromagnet. The authors discuss the results in relation to both recent neutron scattering experiments and recent computations for finite chains with S= 1 / 2 . It is concluded that contributions to the dynamical structure factor from many accumulating low-frequency excitations provide the high-frequency strength required from sum rule arguments for small wavevectors.

DOI
10.1088/0022-3719/12/1/009

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The authors have evaluated an expression obtained previously for the dynamical spin correlation function of a linear Heisenberg antiferromagnet. The authors discuss the results in relation to both recent neutron scattering experiments and recent computations for finite chains with S= 1 / 2 . It is concluded that contributions to the dynamical structure factor from many accumulating low-frequency excitations provide the high-frequency strength required from sum rule arguments for small wavevectors.
The exact expression derived by Bougourzi, Couture, and Kacir for the two-spinon contribution to the dynamic spin structure factor S(q,\ensuremath{\omega}) of the one-dimensional s=1/2 Heisenberg antiferromagnet at T=0 is evaluated for direct comparison with finite-chain transition rates (N\ensuremath{\leqslant}28) and an approximate analytical result previously inferred from finite-N data, sum rules, and Bethe ansatz calculations. The two-spinon excitations account for 72.89% of the total intensity in S(q,\ensuremath{\omega}). The singularity structure of the exact result is determined analytically and its spectral-weight distribution evaluated numerically over the entire range of the two-spinon continuum. The leading singularities of the frequency-dependent spin autocorrelation function, static spin structure factor, and q dependent susceptibility are determined via sum rules. The impact of the non-two-spinon excitations on the integrated intensity, the susceptibility, the frequency moments, and the Euclidian time representation of S(q,\ensuremath{\omega}) is studied on the basis of finite-size data.
The author calculates the dynamical structure factors of a two-dimensional Heisenberg antiferromagnet at T=0, to order 1/(2S) 2 , taking careful account of the umklapp processes. It is shown that, for the transverse spin part, the terms of order 1/(2S) 2 give rise to a broad sideband peak of three-magnon excitations, whose intensity is small but not negligible. For the longitudinal spin part, the terms of order 1/(2S) 2 modify noticeably the spectral shape of the continuum of two-magnon excitations as a function of frequency. These results could be observed in future neutron scattering experiments.
We consider the anisotropic Heisenberg spin-1/2 chain in a transverse magnetic field at zero temperature. We first determine all components of the dynamical structure factor by combining exact results with a mean-field approximation recently proposed by Dmitriev et al. [JETP 95, 538 (2002)]. We then turn to the small anisotropy limit, in which we use field theory methods to obtain exact results. We discuss the relevance of our results to neutron scattering experiments on the one-dimensional Heisenberg chain compound Cs2CoCl4.{\mathrm{Cs}}_{2}{\mathrm{CoCl}}_{4}.Cs2​CoCl4​.
Inelastic neutron scattering experiments are commonly used to unveil how excitations on Heisenberg spin models play a role in dynamical correlations functions. For a certain class of materials, like CsCoCl3_33​ or CsCoBr3_33​ salts, it turns out that their magnetic properties are fairly well approximated by quasi-one dimensional XXZ models, which enjoy the property of quantum integrability. In these instances, one can in principle use their underlying algebraic structure to describe very precisely how excitations, the so-called spinons, participate in dynamical correlations functions. Even though the available theories (either algebraic Bethe ansatz or quantum group approach) provide all the needed physical quantities such as form factors, complete set of eigenstates and spectrum, it is typically a rather daunting task, however, to obtain sufficiently simple analytical expressions for computing Dynamical Structure Factors (DSFs), valuable, e.g., for parameters estimation based on experimental data. This is particularly the case for the longitudinal DSF of the XXZ model, which has eluded a formal mathematical treatment thus far. Using the quantum group approach, we present here an exact and simple expression of the 2-spinon longitudinal DSF and show our results to be consistent with the expected sum rules and the isotropic and Ising antiferromagnet limiting cases.
A theoretical approach to the one-dimensional isotropic Heisenberg model at low temperatures is presented which uses rotationally invariant combinations of spin operators only and is thus adapted to treat correctly effects resulting from the absence of long-range order in these systems. Analytic expressions for space- and time-dependent spin correlation functions are given for small values of TJS2\frac{T}{J{S}^{2}}JS2T​ and 1S\frac{1}{S}S1​. The results include an expression for the spin correlation function in the antiferromagnetic ground state and a discussion of changes in line shape, due to quantum effects, for short-wavelength magnons as observed in neutron scattering experiments.
We calculate the dynamic structure factor $S(\mathbit{k},\ensuremath{\omega})$ in the paramagnetic regime of quantum Heisenberg ferromagnets for temperatures TTT close to the critical temperature Tc{T}_{c}Tc​ using our recently developed functional renormalization group approach to quantum spin systems. In d=3d=3d=3 dimensions, we find that for small momenta $\mathbit{k}$ and frequencies $\ensuremath{\omega}$ the dynamic structure factor assumes the scaling form $S(\mathbit{k},\ensuremath{\omega})=(\ensuremath{\tau}TG(\mathbit{k})/\ensuremath{\pi})\mathrm{\ensuremath{\Phi}}(k\ensuremath{\xi},\ensuremath{\omega}\ensuremath{\tau})$, where $G(\mathbit{k})$ is the static spin-spin correlation function, $\ensuremath{\xi}$ is the correlation length, and the characteristic timescale $\ensuremath{\tau}$ is proportional to ${\ensuremath{\xi}}^{5/2}$. We explicitly calculate the dynamic scaling function $\mathrm{\ensuremath{\Phi}}(x,y)$ and find satisfactory agreement with neutron scattering experiments probing the critical spin dynamics in EuO and EuS. Precisely at the critical point where $\ensuremath{\xi}=\ensuremath{\infty}$, our result for the dynamic structure factor can be written as $S(\mathbit{k},\ensuremath{\omega})={(\ensuremath{\pi}{\ensuremath{\omega}}_{k})}^{\ensuremath{-}1}{T}_{c}G(\mathbit{k}){\mathrm{\ensuremath{\Psi}}}_{c}(\ensuremath{\omega}/{\ensuremath{\omega}}_{k})$, where ${\ensuremath{\omega}}_{k}\ensuremath{\propto}{k}^{5/2}$. We find that ${\mathrm{\ensuremath{\Psi}}}_{c}(\ensuremath{\nu})$ vanishes as ${\ensuremath{\nu}}^{\ensuremath{-}13/5}$ for large $\ensuremath{\nu}$, and as ${\ensuremath{\nu}}^{3/5}$ for small $\ensuremath{\nu}$. While the large-frequency behavior of ${\mathrm{\ensuremath{\Psi}}}_{c}(\ensuremath{\nu})$ is consistent with calculations based on mode-coupling theory and with perturbative renormalization group calculations to second order in $\ensuremath{\epsilon}=6\ensuremath{-}d$, our result for small frequencies disagrees with previous calculations. We argue that until now, neither experiments nor numerical simulations have been sufficiently accurate to determine the low-frequency behavior of ${\mathrm{\ensuremath{\Psi}}}_{c}(\ensuremath{\nu})$. We also calculate the low-temperature behavior of $S(\mathbit{k},\ensuremath{\omega})$ in one- and two-dimensional ferromagnets and find that it satisfies dynamic scaling with exponent z=2z=2z=2 and exhibits a pseudogap for small frequencies.