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Physical Review Letters

Interfering entangled photons of different colors

Todd S. Larchuk, Richard A. Campos, John Rarity, P. R. Tapster, Eric Jakeman, Bahaa E. A. Saleh, Malvin Carl Teich

Published Mar 15, 1993• 63 citations
Publisher

Abstract

We have observed unusual second- and fourth-order interference patterns when entangled photons with center-wavelength differences \ensuremath{\approxeq}40 nm are mixed together at single or dual Mach-Zehnder interferometers. The difference frequency of the photons appears directly in the spectrum of the coincidence rate. This phase-sensitive behavior can reveal center-frequency differences from zero to hundreds of THz.

DOI
10.1103/physrevlett.70.1603

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We have observed unusual second- and fourth-order interference patterns when entangled photons with center-wavelength differences \ensuremath{\approxeq}40 nm are mixed together at single or dual Mach-Zehnder interferometers. The difference frequency of the photons appears directly in the spectrum of the coincidence rate. This phase-sensitive behavior can reveal center-frequency differences from zero to hundreds of THz.
Pairs of 826.8-nm correlated photons, generated by parametrically down-converting 413.4-nm krypton-ion laser light, are directed into a single Mach-Zehnder interferometer such that each photon of the pair enters a different input port. The rate of coincidence at the two output ports displays oscillations (as the path-length difference is swept) with a spatial period equal to the 413-nm wavelength of the pump photons, and with a visibility of 62% when the path-length difference exceeds the coherence length of the individual photon beams. This unequivocally demonstrates the nonclassical and entangled nature of the two-photon state.
A pair of light quanta with different colors (155.9-nm difference in center wavelength) generated from parametric down-conversion was injected collinearly into one input port of a Mach-Zehnder interferometer. Coincidence interference behavior was studied over a wide range of optical path differences of the interferometer. A measurement of 75% interference visibility with oscillation of the pump frequency for a large optical path difference of the interferometer (43 cm) is the signature of a quantum two-photon entangled state, which reflects both particle and wave nature of the light quanta in one experiment.
We present theoretical and experimental second- and fourth-order interference patterns for entangled photons of different colors entering single and dual Mach-Zehnder interferometers in which dispersive elements have been deliberately placed. Although photon wave packets are generally broadened, as well as delayed, by passage through dispersive optical elements, coincidence measurements made with entangled photon pairs can be free of such broadening. This occurs for materials with particular dispersive behavior, as well as when the dispersion is balanced in both arms. This nonlocal behavior arises from the entanglement in the frequencies of the down-converted pair photons. We also show that nonlocal pump-frequency oscillations are present in the coincidence rate patterns for long path-length-difference times, confirming the robustness of this phenomenon in the presence of dispersion. However, the magnitude of these oscillations is reduced when an arbitrary dispersive material is used in an unbalanced configuration. Difference-frequency oscillations are also robust in the presence of dispersion, although they decay for large path-length-difference times.
A new fourth-order interference experiment has been carried out and analyzed theoretically in classical and in quantum terms. Two photons produced in the process of parametric down-conversion provide the two inputs to a Mach-Zehnder type of interferometer, while two photodetectors coupled to a coincidence counter measure the output. The coincidence rate, after subtraction of accidentals, exhibits a cosine variation with the optical path difference, in agreement with quantum mechanics, but in disagreement with a classical analysis. By contrast, when two coherent light beams from a He:Ne laser are used as inputs to the interferometer, no fourth-order interference is observed.
A two-color quantum-entangled photon source is used to produce fourth-order interference. Because the period of the interference is produced by the frequency difference of the entangled photons, problems associated with counting fringes can be avoided. This also permits measurements at a virtual wavelength, which can prevent problems associated with transmission or absorption when such a longer wavelength may be needed. The interference wavelength can be varied with a geometry change in the beam path without any change in the source wavelength. The entangled photons are produced using an argon ion laser at 351 nanometers and a type I BBO crystal. The interference is detected in coincidence using four photomultiplier tubes.
A new fourth-order interference experiment based on detecting photon pairs in coincidence has been carried out. A Mach-Zehnder type of interferometer is used, with the two photons generated simultaneously in the process of down-conversion as inputs and two photon counting detectors at the two outputs. The optical path difference can be varied piezoelectrically. It is found that the coincidence counting rate, after subtraction of accidentals, exhibits a sinusoidal variation with the optical path difference as predicted by quantum mechanics, but in violation of the laws of classical optics. This is another non-classical interference effeet. By contrast, two light beams derived from a He:Ne laser used as inputs to the interferometer, do not produce any fourth order interference.