Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Optical properties of cesium 6S-8S two-photon transitions

Yi-Chi Lee, Yingyu Chen, Yi-Hsiu Chang, Chin‐Chun Tsai, Hsiang‐Chen Chui

Published Aug 1, 2009• 0 citations
Publisher

Abstract

The light shift and linewidth of cesium 6S-8S two-photon transitions are measured in the system. The light shift is -8.60 Hz/(mW/mm2) which is in good agreement with theoretical result. The linewidth is about 1.51 MHz.
DOI
10.1109/cleopr.2009.5292317

Related papers

Polarization and pressure effects in caesium 6S–8S two-photon spectroscopy

Yi-Chi Lee, Yi-Hsiu Chang, Yingyu Chen +2 more

This work analyses the effects of polarization and pressure in caesium 6S–8S two-photon spectroscopy. The linewidth was broadened and the frequency was shifted by a change of polarization states. The frequency shift and the linewidth broadening of the caesium 6S–8S two-photon transition were measured as a function of laser power using one single-frequency Ti:sapphire ring cavity laser, two caesium cells and two quarter-wave plates to ensure polarization states of light, and we showed that the linewidth cannot be evaluated just by fitting data to a Lorentzian shape. As determined by fitting the data to a Voigt profile, the natural linewidth is independent of the polarization states of the pump beams, the laser power and the pressure. Caesium 6S–8S two-photon transitions pumped by a circularly polarized beam have narrower linewidths and smaller shifts than those pumped by a linearly polarized beam. The light shift obtained by pumping with the circularly polarized beam is −6.75(57) Hz (mW mm −2 ) −1 , and that obtained by pumping with a linearly polarized beam is −7.25(45) Hz (mW mm −2 ) −1 . These results agree closely with theoretical calculations. The pressure shift is −588(387) Hz mPa −1 . This work shows how to evaluate two-photon transitions with a Voigt profile, and then helps us to understand two-photon transitions with different polarization states, and improve the signal quality obtained when they are used as frequency markers.

Journal of Physics B Atomic Molecular and Optical Physics•Nov 22, 2010•10 citations

Absolute frequency of cesium 6S-8S hyperfine transition by two-photon interfered spectrum

Chien-Ming Wu, Tze-Wei Liu, Ray‐Kuang Lee +1 more

We present a novel two-photon spectrum in which the transition amplitude was interfered with phase-modulated radiation. We demonstrate the application of our resolved spectrum by determining the absolute frequency of cesium 6S-8S hyperfine transitions.

•Jan 1, 2013•0 citations

Theoretical and experimental study of the 6S-8S two-photon absorption cross-section in cesium atoms

Michael Caracas Núñez, Miguel A. Gonzalez, Mayerlin Núñez Portela

The probability of a two-photon absorption (TPA) process is quantified by means of the TPA cross-section. In this work the TPA cross-section for the 6 S 1/2 → 8 S 1/2 transition in cesium (Cs) atoms is obtained from a theoretical and experimental approach. It is calculated using second order perturbation theory including hyperfine structure and Doppler broadening for a thermal atomic vapor. The theoretical values for the TPA cross-sections of the two allowed hyperfine transitions are σ ~ 3,3 =3.10×10 −24 cm 4 /W and σ ~ 4,4 =3.65×10 −24 cm 4 /W. An experiment is set up to measure these cross-sections based on the quadratic dependence between the TPA transition rate and the intensity of the laser light. Values of σ ~ 3,3 =(3.6±1.1)×10 −24 cm 4 /W and σ ~ 4,4 =(4.6±1.1)×10 −24 cm 4 /W are obtained from the measurements. The results show an agreement between theory and experiment. To the best of our knowledge, this is the first time that these cross-sections are reported.

Optics Express•Aug 14, 2023•4 citations

Absolute hyperfine energy levels and isotope shift of Rb 5S–6S two-photon transition

Seth Orson, Carson McLaughlin, M. D. Lindsay +1 more

Abstract Using a Rb cell and a wavemeter, with a Doppler-free two-photon transition near 993 nm, we have measured the four hyperfine components (two isotopes, Δ F = 0) of the 5S–6S transition, finding the absolute energies of those transitions to a spectral resolution of 0.002 cm −1 = 60 MHz. We find the (87 minus 85) isotope shift of the 5S–6S transition to be +94(12) MHz. Using our single frequency cw laser with focused intensity up to 10 4 W cm −2 at the cell, we find no AC Stark or light shift of the lines at 6 MHz spectral resolution. We find no density shift of the lines at 6 MHz spectral resolution, for a range of Rb atom densities from 3 × 10 11 to 5 × 10 13 atoms/cm 3 .

Journal of Physics B Atomic Molecular and Optical Physics•Sep 8, 2021•4 citations

Two-photon Fourier spectroscopy with femtosecond light pulses

Marco Bellini, A. Bartoli, Theodor W. Hänsch

We demonstrate a Fourier spectrometer that uses intense ultrashort laser pulses. By exciting the 6S(1/2) - 8S(1/2) two-photon transition in atomic cesium vapor, we are able to measure the small hyperfine splitting of the 8S(1/2) excited state. This technique, combining a high spectral resolution with the high peak intensities available to femtosecond laser systems, may offer intriguing opportunities for the study of multiphoton transitions and for spectroscopy in the short-wavelength region.

Optics Letters•Apr 15, 1997•74 citations

Isotope shift and hyperfine structure measurements of 4s 2S1/2→ 6s 2S1/2two-photon transition of potassium isotopes

P. V. Kiran Kumar, Manda V. Suryanarayana

Hyperfine splittings for the 39 K and 41 K isotopes and the isotope shift for the 4s 2 S 1/2 → 6s 2 S 1/2 two-photon transition have been measured using sub-Doppler fluorescence spectroscopy. We have accurately measured the transition isotope shift, and a discrepancy has been found in the earlier reported transition isotope shift value, which has been corrected. The resulting hyperfine splitting values of 418.2 (5) and 230.4 (1.3) MHz for the 39 K and 41 K isotopes respectively are in agreement with previous measurements. The precision of the absolute frequency values for the two-photon transition has been improved by about two orders. Our measured magnetic dipole constants for the upper 6 2 S 1/2 state for the 39 K and the 41 K isotopes are consistent with the earlier measured values.

Journal of Physics B Atomic Molecular and Optical Physics•Feb 18, 2011•12 citations
This work analyses the effects of polarization and pressure in caesium 6S–8S two-photon spectroscopy. The linewidth was broadened and the frequency was shifted by a change of polarization states. The frequency shift and the linewidth broadening of the caesium 6S–8S two-photon transition were measured as a function of laser power using one single-frequency Ti:sapphire ring cavity laser, two caesium cells and two quarter-wave plates to ensure polarization states of light, and we showed that the linewidth cannot be evaluated just by fitting data to a Lorentzian shape. As determined by fitting the data to a Voigt profile, the natural linewidth is independent of the polarization states of the pump beams, the laser power and the pressure. Caesium 6S–8S two-photon transitions pumped by a circularly polarized beam have narrower linewidths and smaller shifts than those pumped by a linearly polarized beam. The light shift obtained by pumping with the circularly polarized beam is −6.75(57) Hz (mW mm −2 ) −1 , and that obtained by pumping with a linearly polarized beam is −7.25(45) Hz (mW mm −2 ) −1 . These results agree closely with theoretical calculations. The pressure shift is −588(387) Hz mPa −1 . This work shows how to evaluate two-photon transitions with a Voigt profile, and then helps us to understand two-photon transitions with different polarization states, and improve the signal quality obtained when they are used as frequency markers.
The probability of a two-photon absorption (TPA) process is quantified by means of the TPA cross-section. In this work the TPA cross-section for the 6 S 1/2 → 8 S 1/2 transition in cesium (Cs) atoms is obtained from a theoretical and experimental approach. It is calculated using second order perturbation theory including hyperfine structure and Doppler broadening for a thermal atomic vapor. The theoretical values for the TPA cross-sections of the two allowed hyperfine transitions are σ ~ 3,3 =3.10×10 −24 cm 4 /W and σ ~ 4,4 =3.65×10 −24 cm 4 /W. An experiment is set up to measure these cross-sections based on the quadratic dependence between the TPA transition rate and the intensity of the laser light. Values of σ ~ 3,3 =(3.6±1.1)×10 −24 cm 4 /W and σ ~ 4,4 =(4.6±1.1)×10 −24 cm 4 /W are obtained from the measurements. The results show an agreement between theory and experiment. To the best of our knowledge, this is the first time that these cross-sections are reported.
Abstract Using a Rb cell and a wavemeter, with a Doppler-free two-photon transition near 993 nm, we have measured the four hyperfine components (two isotopes, Δ F = 0) of the 5S–6S transition, finding the absolute energies of those transitions to a spectral resolution of 0.002 cm −1 = 60 MHz. We find the (87 minus 85) isotope shift of the 5S–6S transition to be +94(12) MHz. Using our single frequency cw laser with focused intensity up to 10 4 W cm −2 at the cell, we find no AC Stark or light shift of the lines at 6 MHz spectral resolution. We find no density shift of the lines at 6 MHz spectral resolution, for a range of Rb atom densities from 3 × 10 11 to 5 × 10 13 atoms/cm 3 .
Hyperfine splittings for the 39 K and 41 K isotopes and the isotope shift for the 4s 2 S 1/2 → 6s 2 S 1/2 two-photon transition have been measured using sub-Doppler fluorescence spectroscopy. We have accurately measured the transition isotope shift, and a discrepancy has been found in the earlier reported transition isotope shift value, which has been corrected. The resulting hyperfine splitting values of 418.2 (5) and 230.4 (1.3) MHz for the 39 K and 41 K isotopes respectively are in agreement with previous measurements. The precision of the absolute frequency values for the two-photon transition has been improved by about two orders. Our measured magnetic dipole constants for the upper 6 2 S 1/2 state for the 39 K and the 41 K isotopes are consistent with the earlier measured values.