Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Optical and Quantum Electronics

Theory of laser-induced amplitude and phase gratings including photoselection, orientational relaxation and population kinetics

A. Von Jena, H.E. Lessing

Published Sep 1, 1979• 73 citations
Publisher
DOI
10.1007/bf00619824

Related papers

Laser-induced dynamic gratings

V. M. Kenkre

Journal of the Optical Society of America B•Jan 1, 1987•3 citations

Effects of different population, orientation, and alignment relaxation rates in resonant four-wave mixing

Skip Williams, Larry A. Rahn, Richard N. Zare

We present a combined theoretical and experimental study on the effects of different population, orientation, and alignment relaxation rates in resonant four-wave mixing (RFWM). Signal generation in RFWM can be viewed as the formation of and scattering from laser-induced population, orientation, and alignment gratings. We show that the relative contributions from the upper-state and lower-state population, orientation, and alignment gratings to the observed output signal can be changed by varying the polarizations of the three input fields. A theory is developed to account for these changes in collisional environments where the three multipole moments of the total angular momentum distribution, i.e., the population, the orientation, and the alignment, relax unequally. This theory is applied to the OH radical in an atmospheric-pressure H2/O2/He flame for which we have measured the line profiles using high-resolution degenerate and nearly degenerate four-wave mixing. We find that orientation and alignment gratings relax more rapidly than population gratings for low rotational levels of OH in the presence of He but at essentially the same rate for high rotational levels. A discussion is presented of the importance of this effect in the interpretation of RFWM experiments.

The Journal of Chemical Physics•Mar 15, 1996•46 citations

Theoretical models of laser-induced processes

Stig Stenholm

AIP conference proceedings•Jan 1, 1995•0 citations

Fourth-order coherence-function theory of laser-induced molecular reorientational grating and population grating

Panming Fu, Zuhe Yu, Xin Mi +1 more

We have employed fourth-order coherence-function theory to study the influence of the partial-coherence properties of pump beams on the laser-induced gratings. First, we examine the formation of molecular reorientational grating. The different roles of phase fluctuation and amplitude fluctuation have been pointed out. A time-delayed method has been proposed to distinguish molecular reorientational grating from thermal grating. We then apply the fourth-order theory to study the Bragg reflection from a population grating. We obtain an analytic solution which enables us to make an extensive investigation on the temporal behaviour of the Bragg reflection signal. This study is especially helpful for elucidating the generation mechanism of population grating.

Journal de physique•Jan 1, 1987•15 citations

Theory of intensity and phase fluctuations of a homogeneously broadened laser

Hermann Haken

The European Physical Journal A•Sep 1, 1966•179 citations

Recording and decay of transient gratings in a system of saturable three-level centers

М. Г. Кучеренко, A. P. Rusinov

The kinetics of formation and relaxation of transient holographic gratings recorded in a system of saturable three-level centers is studied. Distortions in the shape of the profile of recorded and decaying structures of population and of the refractive index are taken into account. The analysis of the time dependences of diffraction efficiencies of different orders is performed for phase (thermal) and amplitude (concentration) gratings.

Optics and Spectroscopy•Dec 1, 2004•2 citations
We present a combined theoretical and experimental study on the effects of different population, orientation, and alignment relaxation rates in resonant four-wave mixing (RFWM). Signal generation in RFWM can be viewed as the formation of and scattering from laser-induced population, orientation, and alignment gratings. We show that the relative contributions from the upper-state and lower-state population, orientation, and alignment gratings to the observed output signal can be changed by varying the polarizations of the three input fields. A theory is developed to account for these changes in collisional environments where the three multipole moments of the total angular momentum distribution, i.e., the population, the orientation, and the alignment, relax unequally. This theory is applied to the OH radical in an atmospheric-pressure H2/O2/He flame for which we have measured the line profiles using high-resolution degenerate and nearly degenerate four-wave mixing. We find that orientation and alignment gratings relax more rapidly than population gratings for low rotational levels of OH in the presence of He but at essentially the same rate for high rotational levels. A discussion is presented of the importance of this effect in the interpretation of RFWM experiments.
We have employed fourth-order coherence-function theory to study the influence of the partial-coherence properties of pump beams on the laser-induced gratings. First, we examine the formation of molecular reorientational grating. The different roles of phase fluctuation and amplitude fluctuation have been pointed out. A time-delayed method has been proposed to distinguish molecular reorientational grating from thermal grating. We then apply the fourth-order theory to study the Bragg reflection from a population grating. We obtain an analytic solution which enables us to make an extensive investigation on the temporal behaviour of the Bragg reflection signal. This study is especially helpful for elucidating the generation mechanism of population grating.