The moderately damped regime in Josephson junctions (JJ) is quite common in devices characterized by low critical currents and, therefore, by low Josephson energies. Measurements of the switching current distribution (SCD) are a direct way of determining the phase dynamics in the nontrivial case of moderate damping, which is becoming more common with advances in nanopatterning superconductors and in materials science for fabricating hybrid systems. We report measurements of SCDs, in both the thermal and quantum regimes for moderately damped YBaCuO grain boundary biepitaxial JJs. A direct transition from a phase diffusion regime to macroscopic quantum tunnelling occurs at about 130 mK. The crossover to the quantum regime is determined by the magnetic field and the phase dynamics can be described by a fully consistent set of junction parameters obtained by numerical simulation.
We investigate the phase dynamics of moderately damped NbN/AlN/NbN Josephson junctions and we present experimental results on detailed aspects of phase diffusion processes. We measure both single escape and multiple escape and retrapping events obtaining a crossover temperature T* from Kramers to phase diffusion switching. We observe a clear dependence of the crossover temperature T* by the bias current ramp rate, while the damping factor Q remains the same. The measured effect is in strong agreement with theoretical predictions reported by Fenton and Warburton.
We have studied the temperature dependence of escape phenomena in various underdamped Josephson junctions (JJs). The junctions had different Josephson coupling energies E J which were relatively small, but larger than the charging energy E C . Upon increasing the temperature T , we first observe the usual cross-over between macroscopic quantum tunnelling and thermally activated (TA) behaviour at temperatures k B T ∼ ℏω p , where ω p is the plasma frequency of the junction. Increasing T further, the width of the switching current distribution has, counterintuitively, a non-monotonic temperature dependence. This can be explained by the novel cross-over from TA behaviour to underdamped phase diffusion. We show that this cross-over is expected to occur at temperatures such that k B T ∼ E J (1 − 4/π Q ) 3 /2, where Q is the quality factor of the junction at the plasma frequency, in agreement with experiment. Our findings can be compared with detailed model calculations which take into account dissipation and level quantization in a metastable well. Particular attention is paid to the sample with the smallest E J , which shows extensive phase diffusion even at the lowest temperatures. This sample consists of a dc-SQUID and a single JJ close to each other, such that the SQUID acts as a tunable inductive protection for the single junction from fluctuations of a dissipative environment. By varying the flux through the dc-SQUID, we present, for the first time, experimental evidence of the escape of a JJ from the phase diffusion regime to the free running state in a tunable environment. We also show that in the zero voltage state the losses mainly occur at frequencies near the plasma resonance.
The topic of the PhD project is a comparative study of phase dynamics and macroscopic quantum phenomena in moderately damped NbN, YBaCuO grain boundary (GB) Josephson junctions (JJs) and hybrid devices. This type of research activity responds to the needs of better identifying phase dynamics in JJs in the moderately damped regime, which is going to be more and more common in hybrid nanostructures. Issues on a more detailed understanding of coherence, dissipation and noise in the various devices have a relevant role in the progress of quantum circuits.
In the last few years, studies of phase dynamics and macroscopic quantum phenomena have been extended to junctions composed of materials other than the traditional low critical temperature superconductors (LTS) and to novel types of structures with unconventional barriers composed for instance of graphene sheets or of grain boundaries. Progress in engineering new materials into junctions and in understanding and controlling the physics of interfaces may offer novel solutions for junctions of superior quality and complementary functionalities, and therefore may lead in the long run to improve also specific qubit performances.
For LTS JJs, once the barrier thickness and the critical current density (Jc) have been fixed, a reduction in its size unavoidably leads to a lowering of the critical current and determines a quite different phase dynamics re-normalized to the new scaling energy. Lower critical currents Ic result in lower Josephson energies EJ, and higher levels of dissipation are expected. The range of the energy dynamical parameters is significantly enlarged, and it is technologically easier to reproducibly realize nontrivial configurations. These devices are characterized by intermediate levels of dissipation (moderately damped regime) and by phase diffusion phenomena. The low Jc limit seems to be characteristic also of all futuristic nanohybrids devices incorporating nanowires, and the moderately damped regime (MDR) is intrinsically more common than it could be expected.
Measurements of switching current distribution (SCD) in these last years have turned to be standard tools to investigate phase dynamics in unconventional and hybrid systems and nanostructures. High critical temperature superconductors (HTS) are an example of unconventional systems, because of the d-wave order parameter symmetry and of the presence of low-energy quasiparticles, which are expected to induce high level of dissipation and as a consequence to spoil macroscopic quantum coherence. A comparative study in systems so different and complementary is of great interest.
During the PhD program, we have performed measurements of SCD, both in the thermal and quantum regime down to 20 mK, on moderately damped NbN/MgO/NbN JJs and on YBCO biepitaxial GB JJs. The NbN JJs exhibit a crossover from thermal activation (TA) to macroscopic quantum tunneling (MQT) regime at about 90 mK. After the MQT saturation, the width of the SCD follows the expected dependence in the TA regime. Deviations are evident in proximity and above the crossover temperature T* (about 1.6K) where we find effects of anti-correlation between the bath temperature and thermal fluctuations since the width of the histograms starts to collapse, and indications of a transition to a third regime called phase diffusion (PD) are evident, such as the change of the switching distributions symmetry.
Experimental data have been analyzed through numerical fitting of the switching probability and Monte Carlo simulations, and we found a good agreement with theoretical expectations based on multiple re-trapping processes, which strongly depend on the junction damping. The combined analysis of these three regimes allowed us to extract the fundamental parameters, which completely characterize the dynamics of such moderately damped NbN JJs. In addition, clear signatures of the PD regime have been detected and numerical methods have been developed to estimate the dissipation level in the MDR.
As a term of comparison, the studies on moderately damped systems have been also carried out on HTS junctions, which have different levels of intrinsic dissipation induced by low energy quasi-particles, and are for this reason of great impact as a reference.
In such JJs we have clearly observed a direct transition from the MQT to the PD regime. The width of the SCDs is constant below 100mK, which is a clearly indication of a quantum activation regime. Above 100mK the negative temperature derivative of the width is consistent with a diffusive motion due to multiple escape and re-trapping in the potential wells. Thermal behavior of the width has been fitted through numerical simulations, thus providing the estimate of the damping factor. These conclusions of a PD regime also in YBaCuO JJs are supported by data in presence of an externally applied magnetic field, and are consistent with the numerical outcomes.
Numerical simulations of the thermal behavior of the SCD width for different values of the quality factor ranging from 1 to 10 have been carried out. Such numerical simulations allow us to reconstruct a (Q, kBT/EJ) phase diagram summarizing the various activation regimes. The transition curve between the PD regime and the running state following thermal or quantum activation has been determined numerically by varying the damping factor Q as function of the ratio between the thermal energy and the Josephson energy. The result of the calculation is a universal curve. A phase diagram valid in a large range of dissipation conditions emerges as a functional guide to classify the switching behavior and to settle the fundamental junction parameters and energies in the MDR. It is therefore a reference for phase dynamics of novel types of junction and system for which the nature of the current induced transition from the superconducting to the normal state has not been completely clarified.
High quality epitaxial NbN/MgO/NbN Josephson junctions have been realized with MgO barriers up to a thickness of d = 1 nm. The junction properties coherently scale with the size of barrier, and low critical current densities down to 3 A/cm2 have been achieved for larger barriers. In this limit, junctions exhibit macroscopic quantum phenomena for temperatures lower than 90 mK. Measurements and junction parameters support the notion of a possible use of these devices for multiphoton quantum experiments, taking advantage of the fast non equilibrium electron-phonon relaxation times of NbN.
The observation of macroscopic quantum tunneling (MQT) manifests the quantumness of macroscopic variables, such as the phase difference across a Josephson junction (JJ). Since then, MQT has become a hallmark experiment to show the quantum nature of JJ-based devices. It has also paved a way to test other macroscopic quantum effects and has led to engineering a variety of artificial atoms, i.e., qubits. However, in the progress of quantum circuits for different applications, it is crucial to understand the influence of thermal and quantum fluctuations, dissipation, and noise to various quantum devices. Thus, the role of the factors mentioned above and the junction parameters
EJ (Josephson coupling energy) and
EC (charging energy) can be scrutinized by understanding the dynamics of the fictitious phase particle. Similarly, in the application perspective, Szilard engine based on SET device are too slow to convert heat into work and are not efficient in-terms of power performance. To overcome the drawbacks, we proposed a high-efficiency fast Szilard engine based on a flux logic device (FLD) and investigated its property numerically and optimize its performance. \\\\ In the first part of the dissertation, we studied the phase dynamics of moderately damped Josephson junctions. The time of flight technique is used to measure the switching current distributions (SCDs). Different dynamical states, thermal activation (TA), MQT, and phase diffusion (PD) are identified from SCDs through well-defined criteria. We observed unambiguous evidence of MQT when temperature is below
∼0.5-0.8 K. The importance of the tilt in the phase dynamics of the junctions, which has been overlooked in previous studies, is clarified. We found that the junction with larger
EJ but the same
ωp0 requires greater tilt and lower temperature to enter MQT regime. \\ \\ In the second part of the dissertation, to overcome the limitation of the SET based Szilard engine, we used superconducting quantum interference device (SQUID) as a one-bit flux logic cell to realize a fast Szilard engine for optimal power. In the past decade, due to technological advancement, the study of energy fluctuations in nano-scale systems such as optical or electrical traps and single-electron tunneling (SET) devices has transformed Szilard's engine to experimental realizations. However, the heat engine realized are slow to convert heat into work limiting their performance in speed and power. The SQUID-based flux logic device (FLD) has a high characteristic frequency,
ωp/2$\pi \sim
10^{10}$ Hz, making it an excellent candidate for realizing a high-efficiency Szilard engine with unprecedented performance. We showed that, on average, the proposed heat engine can extract k
BTln2 of heat per cycle from the thermal reservoir in the quasi-static (QS) limit. In addition, we showed that the FLD-based Szilard engine delivers maximum power when operated about 200 times faster than the threshold speed of quasi-static operation. Our result demonstrates that Szilard's engine's performance based on FLD exceeds other nano-device implementations by orders of magnitude. \\