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Physical Review A

Atomic collisions in the presence of laser radiation: Time dependence and the asymptotic wave function

Paul L. DeVries, Thomas F. George

Published Sep 1, 1982• 5 citations
Publisher

Abstract

A time-dependent, wave-packet description of atomic collisions in the presence of laser radiation is extracted from the more conventional time-independent, stationary-state description. This approach resolves certain difficulties of interpretation in the time-independent approach which arise in the case of asymptotic near resonance. In the two-state model investigated, the approach predicts the existence of three spherically scattered waves in this asymptotically near-resonant case.

DOI
10.1103/physreva.26.1419

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A time-dependent, wave-packet description of atomic collisions in the presence of laser radiation is extracted from the more conventional time-independent, stationary-state description. This approach resolves certain difficulties of interpretation in the time-independent approach which arise in the case of asymptotic near resonance. In the two-state model investigated, the approach predicts the existence of three spherically scattered waves in this asymptotically near-resonant case.
Atom-laser interaction is at the heart of the vibrant field of quantum optics. The dynamical properties of a moving atom submitted to a laser radiation are strongly \ninfluenced by the position- and time-dependence of the latter. The full physical state of the atom must include information about the centre-of-mass motion and the internal structure of the atom. It is challenging to obtain a complete description of the full state of the atom. However, there exists an alternative approach to the dynamics of an atom in the presence of a laser, which is based on the concept of matter-wave absorption. \n \nIn this thesis, we theoretically study the nonrelativistic one-dimensional motion of an electrically neutral quantum particle in the presence of a thin time-dependent absorber, representing the laser radiation. Our aim is to better understand the precise connection between time-dependent matter-wave absorption and the interaction between an atom and a localised time-dependent laser. \n \nOur analysis is based on two different approaches to the problem. The first one describes the moving atom by a two-level system, and represents the laser radiation \nby an off-diagonal δ-potential. The second model treats the atom as a structureless particle, and describes the laser by a time-dependent absorbing barrier. While the \nformer model can be derived from first principles, the treatment of the absorbing barrier in the latter model lacks a rigorous quantum mechanical justification. The \nmain outcome of our work is to provide a solid physical ground for the absorber model, by explicitly connecting it to the δ-potential model. We have thus extended \nthe range of theoretical tools useful for investigating the effects of time-dependent laser radiation on quantum matter.
The density-matrix approach is used to describe the dynamics of thallium-type dressed atoms in a gaseous environment. The effects of spatial degeneracy are accounted for. It is shown that the stationary contribution to the spectrum is not always dominant and may even be negligible. Thus, a consistent description requires the use of the time-dependent spectrum such as that of Eberly and Wodkiewicz (1977). In this connection a new interpretation of the experiment on near resonant scattering of light on thallium-type atoms is proposed.
A modified perturbation theory is developed for the calculation of the time-dependent wave function describing the propagation of an atom in a two-mode laser field. With the mode frequencies nearly equal, a first approximation is obtained that reproduces and extends known results, for both resonant and nonresonant transitions. This lowest-order solution sums terms that describe the absorption of a photon from one mode and emission into the other, leaving the total number of photons unchanged and shifting the momentum of the atom accordingly. Corrections are generated by expansion of a resolvent from which the nearly degenerate states have been projected out. These approximate solutions are used to construct asymptotic states in a formulation of atom-atom scattering in the two-mode field. In close analogy with the soft-photon approximation, a ``soft-pair'' approximation is developed based on the dominance of those asymptotic interactions in which the transfer of energy from the field to the atom is small, allowing one to relate the scattering amplitude in the presence of the field to the field-free amplitude. When the atomic ground state and an excited state are closely coupled by the field, the asymptotic wave function can have mixed parity allowing for long-range contributions to the effective potential. In addition to an enhancement of forward-scattering probabilities, this leads to a threshold anomaly that is analyzed here, in the resonant case, with the aid of a modified effective-range theory.
In the first paper of this series a formal theory of atomic scattering of electrons in the presence of an intense electromagnetic field was given. Cross sections, near the forward direction, between atomic states (modified by the laser) were obtained. However, it was assumed that the atom could not emit spontaneous radiation. In this paper the effect of spontaneous radiation is included, and it is shown that in most cases the measured cross section will be a weighted average of the two different cross sections starting from the two different initial states which are those atomic states resonantly linked by the laser. The Born approximation for the scattering is obtained, and it is shown that for the simplest description of the spontaneous radiation field the effect of the laser on the cross sections is simply to multiply them by a factor which depends upon the laser detuning.
Two-body scattering is analyzed using a time-dependent formalism and wave packets of arbitrary shape as the initial wavefunctions. In particular, the case of single-channel resonant scattering is discussed in some detail. In addition to the usual amplitudes resulting from the potential term and the resonant term, a third amplitude is found which interferes with the other two. Another interesting result is that in this formalism the final state is not necessarily represented by spherical outgoing waves, but can be interpreted instead as two separate outgoing wave packets whose shape is different from the initial packets. The Wigner time delay is obtained as a natural consequence of the analysis, and the resonant cross sections are expressed as density matrices constructed from the wave packets.