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Physical Review Letters

Spontaneous symmetry breaking in quantum frustrated antiferromagnets

P. Azaria, Bertrand Delamotte, D. Mouhanna

Published Apr 19, 1993• 64 citations
Publisher

Abstract

We show that the spontaneous symmetry breaking mechanism in quantum antiferromagnets is due to the collapse, in the thermodynamical limit, of an infinite set of excited states onto the ground state. We characterize both the nature and the scaling of the relevant tower of states for the quantum antiferromagnet on the triangular lattice. Comparison with recent numerical results for the S=1/2 case gives strong support for the existence of long range order in this system.

DOI
10.1103/physrevlett.70.2483

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We show that the spontaneous symmetry breaking mechanism in quantum antiferromagnets is due to the collapse, in the thermodynamical limit, of an infinite set of excited states onto the ground state. We characterize both the nature and the scaling of the relevant tower of states for the quantum antiferromagnet on the triangular lattice. Comparison with recent numerical results for the S=1/2 case gives strong support for the existence of long range order in this system.
We consider a quantum many-body system on a lattice which exhibits a spontaneous symmetry breaking in its infinite volume ground states, but in which the corresponding order operator does not commute with the Hamiltonian. Typical examples are the Heisenberg antiferromagnet with a Néel order, and the Hubbard model with a (superconducting) off-diagonal long range order. In the corresponding finite system, the symmetry breaking is usually “obscured ” by “quantum fluctuation ” and one gets a symmetric ground state with a long range order. In such a situation, Horsch and von der Linden proved that the finite system has a low-lying eigenstate whose excitation energy is not more than of order N −1, where N denotes the number of the sites in the lattice. Here we study the situation where the broken symmetry is a continuous one. For a particular set of states (which are orthogonal to the ground state and with each other), we prove bounds for their energy expectation values. The bounds establish that there exist ever increasing numbers of low-lying eigenstates whose excitation energies are bounded by a constant times N −1. A crucial feature of the particular low-lying
We calculate the order parameter m in the infinite-range isotropic-interaction quantum model of antiferromagnetism due to Lieb and Mattis (LM). The Hamiltonian H1{\mathit{H}}_{1}H1​ in this model contains pure Heisenberg interactions. m is the mean value of the z component msz{\mathit{m}}_{\mathit{s}}^{\mathit{z}}msz​ of the staggered spin per particle ms{\mathbf{m}}_{\mathit{s}}ms​ in the ground state of H1{\mathit{H}}_{1}H1​ plus a symmetry-breaking term HB{\mathit{H}}_{\mathit{B}}HB​ due to an infinitesimal staggered field B in the thermodynamic limit (TL). We find a value of \ensuremath{\surd}3 for the ratio r=m/m0{\mathit{m}}_{0}m0​, m0{\mathit{m}}_{0}m0​ being the root-mean-square value of msz{\mathit{m}}_{\mathit{s}}^{\mathit{z}}msz​ for B==0 in the TL. m and m0{\mathit{m}}_{0}m0​ measure, respectively, the spontaneous symmetry breaking and the amount of long-range order in the symmetry-unbroken state. This value is expected on the basis of our recent argument that r= \ensuremath{\surd}3 if ms{\mathbf{m}}_{\mathit{s}}ms​ behaves in the TL as a classical vector with no magnitude fluctuations---behavior that we show holds for the Lieb-Mattis model. The addition to H1{\mathit{H}}_{1}H1​ of a small easy-axis anisotropic term is also discussed briefly. These studies allow calculation of the size dependence of quantities that we have recently shown to become lower bounds on m in the TL (bounds that are valid for short-range-interaction models as well). In the LM model, low-lying energy eigenstates with excitation energies of order ${\mathit{N}}^{\mathrm{\ensuremath{-}}1}$, where N is the number of spins, form a continuum (with no gap) in the TL. These are closely related to similar states shown to exist for the nearest-neighbor isotropic Heisenberg antiferromagnet. We show that this continuum has a density of states that is O(N0{\mathit{N}}^{0}N0); i.e., it is not extensive.
Motivated by recent experiments that require more complicated macroscopic wave functions in the condensed matters, we make numerical study on a XY quantum antiferromagnet on a finite triangular lattice using the variational Monte Carlo method and the stochastic state selection method. One of our purpose is a numerical confirmation on dominance of a Nambu-Goldstone boson in low energy excitation. For another purpose, we calculate energy, an expectation value of a symmetry breaking operator and structure functions of spin by fixing a quantum number of the symmetry. These calculations are made for states that become degenerate in an infinitely large lattice. By numerical calculations we confirm existence of a Nambu-Goldstone boson, and find dependence of a square of the quantum number for the above quantities. Using these results we can discuss on complicated macroscopic wave functions in quantum spin systems.
We present a mathematically simple procedure to explain spontaneous symmetry breaking in quantum systems. The procedure is applicable to a wide range of models and can be easily used to explain the existence of a symmetry broken state in crystals, antiferromagnets, and even superconductors. It has the advantage that it automatically brings to the fore the main players in spontaneous symmetry breaking: the symmetry-breaking field, the thermodynamic limit, and the global excitations of a “thin” spectrum.
Frustration on the triangular lattice has long been a source of intriguing and often debated phases in many-body systems. Although symmetry analysis has been employed, the role of the seemingly trivial parity symmetry has received little attention. In the work described in this Letter, we show that phases induced by frustration are systematically shaped by an implicit rule of thumb associated with spontaneous parity breaking in weak longitudinal field. This principle enables us to anticipate and rationalize the regimes and conditions under which nontrivial phases emerge. For the spin-SSS antiferromagnetic XXZ model, we demonstrate that a controversial parity-broken phase appears at intermediate values of SSS. In bilayer systems, enhanced frustration leads to additional phases, such as supersolids, whose properties can be classified by their characteristic parity features. Benefiting from our improved tensor network contraction techniques, we confirm these results through large-scale tensor-network calculations. This study offers an alternative viewpoint and a systematic approach for examining the interplay between spin, symmetry, and frustration in many-body systems.