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Physical Review B

Effects of entanglement on elastic and inelastic scattering functions for neutron scattering from a pair of nuclei in solids

Hidehiko Sugimoto, Aiko Okumura, 寛之 結城

Published Jan 25, 2006• 14 citations
Publisher

Abstract

We calculate the scattering function of neutrons, $S(\stackrel{P\vec}{q},\ensuremath{\omega})$, from a pair of nuclei in entangled states caused by the quantum-mechanical indistinguishability of particles. From the calculation, the conditions for detecting the entanglement of protons in solids by neutron scattering experiments are clarified. Our conclusion is that the entangled state of a proton pair, if it exists, can be observed by performing neutron scattering experiments at very low temperatures for elastic scattering and with high energy resolution for inelastic scattering.

DOI
10.1103/physrevb.73.014305

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Searching for entanglement in final polarization states of the neutron-proton scattering

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arXiv:2505.14401•May 20, 2025•0 citations
We calculate the scattering function of neutrons, S(\stackrel{P\vec}{q},\ensuremath{\omega}), from a pair of nuclei in entangled states caused by the quantum-mechanical indistinguishability of particles. From the calculation, the conditions for detecting the entanglement of protons in solids by neutron scattering experiments are clarified. Our conclusion is that the entangled state of a proton pair, if it exists, can be observed by performing neutron scattering experiments at very low temperatures for elastic scattering and with high energy resolution for inelastic scattering.
It is shown that quantum entanglement in condensed matter can be observed with scattering experiments if the energy resolution of the experiments enables a clear separation between the elastic scattering and the scattering from the excitations in the system. These conditions are not satisfied in recent deep inelastic neutron scattering experiments from hydrogen-containing systems that have been interpreted as showing the existence of quantum entanglement for short times in, for example, water at room temperature. It is shown that the theory put forward to explain these experiments is inconsistent with the first-moment sum rule for the Van Hove scattering function and we suggest that the theory is incorrect. The experiments were performed using the unique EVS spectrometer at ISIS and suggestions are made about how the data and their interpretation should be re-examined.
Several recent experiments on liquid and solid samples containing protons or deuterons show an interesting anomaly, which is a shortfall in the intensity of energetic neutrons scattered by the samples. Previously we demonstrated that quantum correlations in the spatial and spin degrees of freedom of the hydrogen isotopes lead to entanglement in scattering and a reduction in the scattered intensity. The viability of short-lived quantum correlations as the cause of the observed anomalies is further explored and found to be entirely feasible. General features of the basic premiss, that quantum entanglement reduces the scattered signal, are discussed and the interpretation of the neutron scattering experiments is set in context to related work on other systems. For the experiments in question, the duration of a scattering event, τ s , is a fraction of a femtosecond which is extremely short compared to solid-state relaxation times. Increasing τ s , by suitably changing experimental conditions, restores the intensity to the standard value calculated from the single atom cross-section and concentration of particles. Our physical picture of the restoration is evolution with increasing τ s from a pure state of the particles (described by a wavefunction) to a mixed state (described by a density matrix) that is created, through decoherence, by steadily engaging the solid-state environment of the particles.
Abstract Quantum entanglement in scattering processes has most often been treated in general terms only. A few examples of detailed calculations exist for atomic systems but for nuclear processes it is an almost unexplored area, although it may be important for interpretation of some measured quantities. The present treatment is a study of the time-development of the deuteron-like compound state created in the n – p scattering process. The increase and decay of neutron–proton entanglement in this state is calculated for low transferred momenta over the atto-second range. It is well known that the very high value for the bound proton cross sections ( σ = 81.9 barns) is caused by a specific feature in the deuteron, a virtual 0+ state close to its binding level. In scattering this state causes a negative phase shift δ s in the outgoing neutron wave function, increasing linearly with the transferred momentum. This phase shift is produced during a short-lived virtual energy transfer Δ E in exciting the 0+ state and Δ E is estimated here from the ratio of the phase shift δ observed and the time Δ t it takes to create the entanglement. It is further argued that the nuclear excitation decreases after the n – p encounter in proportion to the degree of n – p entanglement calculated, i.e. as long as the scattering state has deuteron characteristics. This phase shift is neglected in low energy neutron scattering text-books (which are based on the Fermi pseudo potential) and may be negligible for thermal neutron scattering, but will be important already at epithermal energies (0.1–1 eV). The phase shift has measurable consequences in interpretation of INS (inelastic neutron scattering) since its associated energy shift increases quadratically with the transferred momentum. It explains quantitatively certain anomalies found in scattering on water, where water vibration modes are excited far below the expected transferred momentum limit. This paper ends with a short discussion about quantum entanglement in scattering processes in general, with the present example as a starting point.
We investigate polarization states of the outgoing neutron-proton (npnpnp) pair in elastic polarized neutron and proton scattering, aiming to find unambiguous evidence for entanglement of their spin states. To obtain complete information about these states, we calculate, using the high-precision nucleon-nucleon potential AV18, the final polarizations of the neutron and proton as well as their spin correlation coefficients, which unequivocally define the corresponding spin density matrix. We compute all terms contributing to polarizations and spin correlations, e.g., not only induced polarizations and correlations resulting from unpolarized npnpnp scattering but also contributions from single polarization and correlation transfers from individual polarized incoming nucleons and, for the first time, allotment to both quantities stemming from a doubly spin polarized initial state. We find that for the most part the final spin states are statistical mixture of states. The only pure states occur for highly polarized incoming neutrons and protons with maximal polarizations. By quantifying the degree of entanglement through entanglement power and concurrence, we observed that the entanglement of impure final states increases with energy. Among the pure spin states resulting from incoming states with maximal neutron and proton polarizations, we found, at Elab=100{E}_{\mathrm{lab}}=100Elab​=100 MeV, cases of strongly entangled Bell-type states with only a small admixture of entanglement-spoiling contributions.
We investigate polarization states of the outgoing neutron-proton (npnpnp) pair in elastic polarized neutron and proton scattering, aiming to find unambiguous evidence for entanglement of their spin states. To obtain complete information about these states, we calculate, using the high precision nucleon-nucleon potential AV18, the final polarizations of the neutron and proton as well as their spin correlation coefficients, which unequivocally define the corresponding spin density matrix. We compute all terms contributing to polarizations and spin correlations, e.g. not only induced polarizations and correlations resulting from unpolarized npnpnp scattering, but also contributions from single polarization and correlation transfers from individual polarized incoming nucleons, and, for the first time, allotment to both quantities stemming from a doubly spin polarized initial state. We find that for the most part the final spin states are statistical mixture of states.The only pure states occur for highly polarized incoming neutrons and protons with maximal polarizations. By quantifying the degree of entanglement through entanglement power and concurrence, we observed that the entanglement of impure final states increases with energy. Among the pure spin states resulting from incoming states with maximal neutron and proton polarizations, we found, at Elab=100E_{lab}=100Elab​=100~MeV, cases of strongly entangled Bell-type states with only a small admixture of entanglement-spoiling contributions.