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Physical Review Letters

Effects of Entanglement on the Scattering Intensity of Neutron Compton Scattering by a Proton Pair in Solids

Hidehiko Sugimoto, 寛之 結城, Aiko Okumura

Published Apr 29, 2005• 17 citations
Publisher

Abstract

We calculate scattering functions S(q-->,omega) of neutron Compton scattering (NCS) for a proton (deuteron) pair in the entangled state caused by the indistinguishability of particles. From the calculation, it is concluded that the effect of entanglement on the scattering intensity is undetectable in NCS experiments because of their high energy transfer and broad energy resolution.

DOI
10.1103/physrevlett.94.165506

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We calculate the scattering function of neutrons, $S(\stackrel{P\vec}{q},\ensuremath{\omega})$, from a pair of nuclei in entangled states caused by the quantum-mechanical indistinguishability of particles. From the calculation, the conditions for detecting the entanglement of protons in solids by neutron scattering experiments are clarified. Our conclusion is that the entangled state of a proton pair, if it exists, can be observed by performing neutron scattering experiments at very low temperatures for elastic scattering and with high energy resolution for inelastic scattering.

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Nuclei and electrons in condensed matter and/or molecules are usually entangled, due to the prevailing electromagnetic interactions. Usually, the “environment” of a microscopic scattering system (e.g., a proton) causes an ultrafast decoherence, thus making atomic and/or nuclear entanglement effects not directly accessible to experiments. However, neutron Compton scattering (NCS) and electron Compton scattering represent ultrafast techniques operating in the sub-femtosecond timescale, thus opening a way for investigation of such dehoherence and short-lived entanglement phenomena of atoms in molecules and condensed matter. The experimental context of NCS and a new striking scattering effect from protons (H-atoms) in several condensed systems and molecules are described. In short, one observes an “anomalous” decrease of scattering intensity from protons, which seem to become partially “invisible” to the neutrons. The experiments apply large energy (several electronvolts) and momentum (10–200 Å −1 transfers, and the collisional (or scattering) time between the neutron and a struck proton is only 100–1000 attoseconds long. Similar results are also obtained with electron-atom Compton scattering at large momentum transfers. As an example, we present new NCS experimental results from a single crystal, which also provide new physical insights into the attosecond quantum dynamics of protons in molecules and condensed matter. Theoretical discussions and models are presented which show that the effect under consideration is caused by the non-unitary time evolution (due to decoherence) of open quantum systems during the ultrashort, but finite, time-window of the neutron-proton scattering process. The conceptual connection with the well known Quantum Zeno Effect is pointed out. The experimental results, together with their qualitative interpretation “from first principles,” show that epithermal neutrons being available at spallation sources, and electron spectrometers providing large momentum transfers, may represent novel tools for investigation of thus far unknown physical and chemical attosecond phenomena.

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Abstract The conventional theory of non-relativistic neutron beam scattering from many-body systems treats the beam essentially as a classical system, because the neutron dynamical variables are captured in the main theoretical formulas (e.g. time-correlation functions) not as quantum mechanical operators but as c-numbers only. This simplification results in the full decoupling of the probe particles’ dynamics from the quantum dynamics of the scatterer. Further, neutrons’ wavefunctions are represented with plane waves, and thus the concept of neutron’s finite coherence length in momentum space becomes irrelevant. Making contact with modern quantum theoretical approaches (e.g., quantum entanglement, Feynman paths, “which-path information” versus interference, Weak Values theory) new observable effects of non-relativistic quantum beam scattering may be exposed and/or predicted, such as a surprising intensity deficit in neutron Compton scattering (NCS) of epithermal neutrons from protons of H-containing materials. Here, the NCS-intensity deficit observed in scattering from liquid C6H6 is discussed and interpreted from first principles, in the general frame of Weak Values theory. Moreover, based on Feynman’s didactical argument that there isn’t any interference between distinguishable neutron paths, we show that this NCS-effect cannot be interpreted as being caused by destructive interference of neutron paths scattered from entangled (two or a few) protons, as was earlier proposed by some authors.

Journal of Physics Conference Series•Nov 1, 2024•0 citations
We calculate scattering functions S(q-->,omega) of neutron Compton scattering (NCS) for a proton (deuteron) pair in the entangled state caused by the indistinguishability of particles. From the calculation, it is concluded that the effect of entanglement on the scattering intensity is undetectable in NCS experiments because of their high energy transfer and broad energy resolution.
We calculate the scattering function of neutrons, $S(\stackrel{P\vec}{q},\ensuremath{\omega})$, from a pair of nuclei in entangled states caused by the quantum-mechanical indistinguishability of particles. From the calculation, the conditions for detecting the entanglement of protons in solids by neutron scattering experiments are clarified. Our conclusion is that the entangled state of a proton pair, if it exists, can be observed by performing neutron scattering experiments at very low temperatures for elastic scattering and with high energy resolution for inelastic scattering.
Several recent experiments on liquid and solid samples containing protons or deuterons have shown an interesting anomaly, which is apparently absent when the hydrogen isotopes are replaced by heavier particles. The anomaly is a shortfall in the intensity of energetic neutrons scattered by the samples; specifically, the intensity per hydrogen isotope in bulk samples is smaller than the intensity for total scattering by an isolated hydrogen isotope. Short-lived correlations in the spatial and spin degrees of freedom of the hydrogen isotopes have been proposed as an explanation of the anomaly. The correlations involve entanglements of the degrees of freedom created by the requirements of quantum mechanics applied to identical particles. By using energetic neutrons to perform Compton scattering experiments on the hydrogen isotopes, the time scale of the experimental probe covers the region of ${10}^{\ensuremath{-}16}--{10}^{\ensuremath{-}15}\mathrm{s}$ where entangled states might still be expected to survive. The proposed explanation is pursued here by reporting the cross section for Compton scattering, also known as deep inelastic scattering, by two identical nuclei occupying nonequivalent states. The model reproduces the observed dependence of the cross section on energy transfer, in which intensity accumulates at the recoil energy of a single nucleus. Several features of the model demand that the intensity at the recoil energy is indeed less than the intensity for total scattering by an isolated nucleus. Although the pair approximation used here is unquestionably a first approximation to real many-body entanglements, it is a compelling explanation of all the observations, including the restoration of the normal cross section at longer observation times achieved by moving to longer scattering times.
We study spin-spin entanglement in the final state photon-nucleon system in Compton scattering, both at low energy below the pion threshold and at high energy in perturbative QCD to next-to-leading order. We first establish a no-go theorem showing that, for any spin-12\frac{1}{2}21​ target, entanglement cannot be generated in unpolarized Compton scattering if the scattering amplitudes are real. We then consider polarized Compton scattering off the electron, the proton and the neutron. At low energy, we uncover a rich variety of maximally entangled Bell states and their unitary equivalents realized across different regions of the kinematic plane. Interestingly, the proton and neutron targets exhibit distinct patterns of entanglement. In the neutron case, the electric and magnetic polarizabilities dramatically influence the pattern and even the existence of entanglement. This suggests that entanglement can serve as a novel tool for investigating the detailed electromagnetic properties of the nucleons.
It has been predicted that entanglement creation should be associated with a lowering of energy (as well as the well‐known decrease of entropy) for certain types of interaction potentials. This is a principally important question and it is shown here that np‐scattering has specific features that would make it suitable for experimental tests of this prediction using neutron scattering on hydrogen at high angles. For this purpose, the evolution of n‐p entanglement in Compton scattering on protons at epithermal energies (20–200 eV) is calculated over the separation distance 0–1 Å, corresponding to times up to 10−15 s after the collision. If an energy transfer is associated with the entanglement, it ought to be observable under these measurement conditions. © 2015 Wiley Periodicals, Inc.
Nuclei and electrons in condensed matter and/or molecules are usually entangled, due to the prevailing electromagnetic interactions. Usually, the “environment” of a microscopic scattering system (e.g., a proton) causes an ultrafast decoherence, thus making atomic and/or nuclear entanglement effects not directly accessible to experiments. However, neutron Compton scattering (NCS) and electron Compton scattering represent ultrafast techniques operating in the sub-femtosecond timescale, thus opening a way for investigation of such dehoherence and short-lived entanglement phenomena of atoms in molecules and condensed matter. The experimental context of NCS and a new striking scattering effect from protons (H-atoms) in several condensed systems and molecules are described. In short, one observes an “anomalous” decrease of scattering intensity from protons, which seem to become partially “invisible” to the neutrons. The experiments apply large energy (several electronvolts) and momentum (10–200 Å −1 transfers, and the collisional (or scattering) time between the neutron and a struck proton is only 100–1000 attoseconds long. Similar results are also obtained with electron-atom Compton scattering at large momentum transfers. As an example, we present new NCS experimental results from a single crystal, which also provide new physical insights into the attosecond quantum dynamics of protons in molecules and condensed matter. Theoretical discussions and models are presented which show that the effect under consideration is caused by the non-unitary time evolution (due to decoherence) of open quantum systems during the ultrashort, but finite, time-window of the neutron-proton scattering process. The conceptual connection with the well known Quantum Zeno Effect is pointed out. The experimental results, together with their qualitative interpretation “from first principles,” show that epithermal neutrons being available at spallation sources, and electron spectrometers providing large momentum transfers, may represent novel tools for investigation of thus far unknown physical and chemical attosecond phenomena.
Abstract The conventional theory of non-relativistic neutron beam scattering from many-body systems treats the beam essentially as a classical system, because the neutron dynamical variables are captured in the main theoretical formulas (e.g. time-correlation functions) not as quantum mechanical operators but as c-numbers only. This simplification results in the full decoupling of the probe particles’ dynamics from the quantum dynamics of the scatterer. Further, neutrons’ wavefunctions are represented with plane waves, and thus the concept of neutron’s finite coherence length in momentum space becomes irrelevant. Making contact with modern quantum theoretical approaches (e.g., quantum entanglement, Feynman paths, “which-path information” versus interference, Weak Values theory) new observable effects of non-relativistic quantum beam scattering may be exposed and/or predicted, such as a surprising intensity deficit in neutron Compton scattering (NCS) of epithermal neutrons from protons of H-containing materials. Here, the NCS-intensity deficit observed in scattering from liquid C6H6 is discussed and interpreted from first principles, in the general frame of Weak Values theory. Moreover, based on Feynman’s didactical argument that there isn’t any interference between distinguishable neutron paths, we show that this NCS-effect cannot be interpreted as being caused by destructive interference of neutron paths scattered from entangled (two or a few) protons, as was earlier proposed by some authors.