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Physics of Particles and Nuclei Letters

Local spin magnetization around the Zn ion which is doped in the CuO2 plane

Zlata Kovačević

Published Sep 1, 2007• 0 citations
Publisher

Abstract

The local static spin susceptibility at neighbor sites from vacant Cu in the CuO 2 plane was obtained. Calculations were performed using one of the variants of the memory function method. Charge-transfer and spin-flip correlation functions were expressed in the framework of the T-matrix formalism in terms of the corresponding Green functions for the ideal t-J model on the square lattice.

DOI
10.1134/s154747710705010x

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The local static spin susceptibility at neighbor sites from vacant Cu in the CuO 2 plane was obtained. Calculations were performed using one of the variants of the memory function method. Charge-transfer and spin-flip correlation functions were expressed in the framework of the T-matrix formalism in terms of the corresponding Green functions for the ideal t-J model on the square lattice.
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A microscopic theory of resonant states for the Zn-doped CuO_2 plane in superconducting phase is formulated within the effective t-J model. In the model derived from the original p-d model Zn impurities are considered as vacancies for the d states on Cu sites. In the superconducting phase in addition to the local static perturbation induced by the vacancy a dynamical perturbation appears which results in frequency-dependent perturbation matrix. By employing the T-matrix formalism for the Green functions in terms of the Hubbard operators the local density of electronic states with d-, p- and s-symmetry is calculated.
Different roles of Zn2+^{2+}2+ and Li+^{+}+ impurities in the CuO2_22​ plane in undoped cuprate compounds
A planar Mott insulator with easy plane Néel order can be mapped onto a Gutzwiller-projected spin Hall state. The in-plane substitution of Zn2+^{2+}2+ and Li+^{+}+ for Cu2+^{2+}2+ brings zero modes around the spin vacancy. The Gutzwiller projection precludes single particle excitations, however, preserves the zero modes which have a local spin moment for Zn2+^{2+}2+ and a local charged hole for Li+^{+}+, respectively. While the local spin moment for Zn2+^{2+}2+ is screened by the long-range spin correlations, the active charge degree of freedom for Li+^{+}+ impurity twists the spin background with long ranged disturbances. This proposal explains the very different roles of the Zn2+^{2+}2+ and Li+^{+}+ impurities on the magnetic perturbations in the CuO2_22​ plane in the undoped cuprate compounds.
A relaxation-function theory for the dynamic spin susceptibility in the $t\text{\ensuremath{-}}J$ model is presented. By a sum-rule-conserving generalized mean-field approximation (GMFA), the two-spin correlation functions of arbitrary range, the staggered magnetization, the uniform static susceptibility, and the antiferromagnetic correlation length are calculated in a wide region of hole doping and temperatures. A good agreement with available exact diagonalization (ED) data is found. The correlation length is in reasonable agreement with neutron-scattering experiments on ${\text{La}}_{2\ensuremath{-}\ensuremath{\delta}}{\text{Sr}}_{\ensuremath{\delta}}{\text{CuO}}_{4}$. Going beyond the GMFA, the self-energy is calculated in the mode-coupling approximation. The spin dynamics at arbitrary frequencies and wave vectors is studied for various temperatures and hole doping. At low doping a spin-wave-type behavior is found as in the Heisenberg model, while at higher doping a strong damping caused by hole hopping occurs, and a relaxation-type spin dynamics is observed in agreement with the ED results. The local spin susceptibility and its $\ensuremath{\omega}/T$ scaling behavior are calculated in a reasonable agreement with experimental and ED data.
We present a spin-rotation-invariant Green-function theory for the dynamic spin susceptibility in the spin-1/2 antiferromagnetic t - J Heisenberg model on the honeycomb lattice. Employing a generalized mean-field approximation for arbitrary temperatures and hole dopings, the electronic spectrum of excitations, the spin-excitation spectrum and thermodynamic quantities (two-spin correlation functions, staggered magnetization, magnetic susceptibility, correlation length) are calculated by solving a coupled system of self-consistency equations for the correlation functions. The temperature and doping dependence of the magnetic (uniform static) susceptibility is ascribed to antiferromagnetic short-range order. Our results on the doping dependencies of the magnetization and susceptibility are analyzed in comparison with previous results for the t - J model on the square lattice.
The dynamical spin susceptibility χ( q , ω), of the t-J model in two-dimensional square lattice have been studied based on the mean field approximation to the slave-boson formalism. The static spin susceptibility, χ( q , 0), and Im χ( q , ω) at various energy, ω, have been calculated. We found; 1) χ(0, 0) has only weak temperature dependence 2) T 1 T ∝( T +θ) for T≳0.1JT\gtrsim0.1{J}T≳0.1J with θ linearly dependent on the doping rate, δ 3) T 1 T has a minimum at T =(0.1∼0.2) J 4) Im χ( q , ω) at q = Q ≡(π, π) has a gap like structure as a function of ω if the temperature is low. All these are consistent with experimental results.