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Optics and Spectroscopy

On certain regularities of the response of a medium upon generation of the triple frequency of a few-period laser pulse in the case of its passage through an optically thin nonlinear layer

Svetlana A. Varentsova, Tatiana M. Lysak, Vyacheslav A. Trofimov

Published Sep 1, 2008• 0 citations
Publisher

Abstract

The response of a medium at the triple frequency under the action of few-period laser pulses is considered within the framework of the thin-optical-layer approximation for the case where the triple frequency is close to the natural frequency of the linear oscillator. It is shown that a bistable dependence of the polarization amplitudes on the external action amplitude simultaneously appears at both the natural frequency and the frequency of the external action. This allows one, in particular, to reveal the presence of bistability of the regime of third harmonic generation in a physical experiment by using the transmitted radiation of the acting pulse. A decrease in the duration of the pulse incident on the medium leads to an increase in the hysteresis loops. The effect of the absolute phase of a short pulse on the spectral composition of the response of the medium is studied. For pulses of medium duration, in addition to the resonant response of the medium, the presence of the dynamic response of the medium at the triple frequency was revealed, despite a detuning of the latter from the resonance. The presence of this frequency in the spectrum of the response of the medium results in the dependence of the resonant response of the medium on the absolute phase even for a sufficiently long pulse containing tens oscillations of the electric field strength under the pulse envelope. To obtain the dynamics of the spectral lines from the results of computer simulation, the Fourier-Gabor method is used, the applicability of which is demonstrated by the comparison of the results obtained on its basis with the corresponding analytical dependences.

DOI
10.1134/s0030400x08090154

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The response of a medium at the triple frequency under the action of few-period laser pulses is considered within the framework of the thin-optical-layer approximation for the case where the triple frequency is close to the natural frequency of the linear oscillator. It is shown that a bistable dependence of the polarization amplitudes on the external action amplitude simultaneously appears at both the natural frequency and the frequency of the external action. This allows one, in particular, to reveal the presence of bistability of the regime of third harmonic generation in a physical experiment by using the transmitted radiation of the acting pulse. A decrease in the duration of the pulse incident on the medium leads to an increase in the hysteresis loops. The effect of the absolute phase of a short pulse on the spectral composition of the response of the medium is studied. For pulses of medium duration, in addition to the resonant response of the medium, the presence of the dynamic response of the medium at the triple frequency was revealed, despite a detuning of the latter from the resonance. The presence of this frequency in the spectrum of the response of the medium results in the dependence of the resonant response of the medium on the absolute phase even for a sufficiently long pulse containing tens oscillations of the electric field strength under the pulse envelope. To obtain the dynamics of the spectral lines from the results of computer simulation, the Fourier-Gabor method is used, the applicability of which is demonstrated by the comparison of the results obtained on its basis with the corresponding analytical dependences.
We investigate the problem of resonant re flection and transmission of an ultrashort light pulse passing through a medium consisting of two-level atoms. We show that for a thin layer it is important to take into account the difference between the external macroscopic field and the field acting on the individual atoms within the medium. The local field correction leads to an inversion dependent resonant frequency. In thin layers this generates a new mechanism of nonlinear transparency induced by the dynamical frequency shift. When the excitation frequency is larger than the original resonant frequency, then the transmission of the layer exhibits bistable behavior.
Refraction of a double-frequency optical pulse at the interface between two linear dielectrics containing a thin film of resonant atoms is considered. The dynamics of the system is treated based on the model of three-level atoms with the V -type energy diagram. Refraction of short and long (compared with the Rabi oscillation period) pulses is analyzed with allowance for local-field effects. In both cases, the shape of the pulse corresponding to one carrier wave frequency is shown to depend on the energy of the pulse with the other carrier wave frequency. In particular, both the frequency and the depth of the amplitude modulation arising in the refracted pulse are changed.
We study the self-action of an amplitude-modulated beam in a two-level saturable absorbing medium. We also consider the radial quadratic dependence of the linear refraction index to apply the results to doped waveguides. As the modulation period approaches the relaxation times, the medium response is no more instantaneous, so that one should solve the full set of Maxwell-Bloch equations. We propose a second-order scheme with the Gauss-Laguerre transformation of the transverse field pattern. A simplified approach based on the synchronous interaction approximation is used for thin layers. We analyze the transient behavior of the medium response and its manifestation in the modulation of the beam diffracting after a thin saturable absorber. Nonlinear distortions of the modulation signal passed through a doped waveguide appear to be unexpectedly small compared with those of the local polarization and population difference.
Abstract Recent progress in generation of optical pulses of durations comparable to one optical cycle has presented great opportunities for studies of the fundamental processes in matter as well as time-resolved spectroscopy of ultrafast processes in nonlinear media. It opened up a new area of research in modern ultrafast nonlinear optics and led to appearance of the attosecond science. In parallel, a new research area related to emission from resonant media excited by superluminally propagating ultrashort bursts of electromagnetic radiation has been actively developed over the last few years. In this paper, we review our recent results on theoretical analysis of the Cherenkov-type radiation of a resonant medium excited by few-cycle optical pulses propagating at superluminal velocity. This situation can be realized when an electromagnetic pulse with a plane wavefront incidents on a straight string of resonant atoms or a spot of light rotates at very large angular frequency and excites a distant circular string of resonant dipoles. Theoretical analysis revealed some unusual and remarkable features of the Cherenkov radiation generated in this case. This radiation arises in a transient regime which leads to the occurrence of new frequencies in the radiation spectrum. Analysis of the characteristics of this radiation can be used for the study of the resonant structure properties. In addition, a nonlinear resonant medium excited at superluminal velocity can emit unipolar optical pulses, which can be important in ultrafast control of wave-packet dynamics of matter. Specifics of the few-cycle pulse-driven optical response of a resonant medium composed of linear and nonlinear oscillators is discussed.
The nonstationary pump-probe interaction between short laser pulses propagating in a resonant optically dense coherent medium is considered. Special attention is paid to the case where the density of two-level particles is high enough that a considerable part of the energy of relatively weak external laser fields can be coherently absorbed and reemitted by the medium. Thus, the field of the medium reaction plays a key role in the interaction processes, which leads to collective behavior of an atomic ensemble in the strongly coupled light-matter system. Such behavior results in fast excitation interchanges between the field and a medium in the form of optical ringing, which is analogous to polariton beating in solid-state optics. This collective oscillating response, which can be treated as successive beats between light wave packets of different group velocities, is shown to significantly affect the propagation and amplification of the probe field under its nonlinear interaction with a nearly copropagating pump pulse. Depending on the probe-pump time delay, the probe transmission spectra show the appearance of either a specific doublet or coherent dip. The widths of these features are determined by the density-dependent field-matter coupling coefficient and increase during the propagation. Besides that, the widths of the coherent features, which appear close to resonance in the broadband probe spectrum, exceed the absorption-line width, since under the strong-coupling regime, the frequency of optical ringing exceeds the rate of incoherent relaxation. Contrary to stationary strong-field effects, the density- and coordinate-dependent transmission spectra of the probe manifest the importance of collective oscillations and cannot be obtained in the framework of a single-atom model.
Coherent responses of resonance atom layer to short optical pulse excitation are numerically considered. The inhomogeneous broadening of one-photon transition, the near dipole-dipole interaction, and the substrate dispersion are involved in analysis. Under certain intensity of incident pulses, a strong coherent interaction in the form of sharp spikes of superradiation is observed in transmitted radiation. The Lorentz field correction and the substrate dispersion weaken the effect, providing additional spectral shifts. Specific features of photon echo in the form of multiple echoes to a double or triple pulse excitation in the presence ofnear dipole-dipole interaction is discussed.