In this paper, we study the modification of coherent scattering processes in dense ensembles. Using absorption imaging, we experimentally demonstrate that the absorption cross section in dense $^{87}\mathrm{Rb}$ cold atom ensembles is reduced, with respect to the single-particle response. This reduction is linearly dependent on the optical density and well reproduced by a one-dimensional model of coherent field propagation in an ensemble of quantum two-level systems that self-consistently incorporates multiple scattering contribution. Our model shines light upon the key role of incoherent scattering on the modification of the optical response of dense ensembles and leads to a generalization of the Beer-Lambert law. Our result applies to any effective two-level system ensemble and allows for quantitative and absolute in situ absorption imaging.In this paper, we study the modification of coherent scattering processes in dense ensembles. Using absorption imaging, we experimentally demonstrate that the absorption cross section in dense $^{87}\mathrm{Rb}$ cold atom ensembles is reduced, with respect to the single-particle response. This reduction is linearly dependent on the optical density and well reproduced by a one-dimensional model of coherent field propagation in an ensemble of quantum two-level systems that self-consistently incorporates multiple scattering contribution. Our model shines light upon the key role of incoherent scattering on the modification of the optical response of dense ensembles and leads to a generalization of the Beer-Lambert law. Our result applies to any effective two-level system ensemble and allows for quantitative and absolute in situ absorption imaging.

arXiv:2110.12505Physical Review ResearchJul 13, 202212 citations

Coherent scattering from coupled two level systems

Thomas Nutz, Samuel T. Mister, Petros Androvitsaneas +5 more

We study the resonance fluorescence properties of an optically active spin 1/2 system, elucidating the effects of a magnetic field on the coherence of the scattered light. We derive a master equation model for this system that reproduces the results of a two level system (TLS) while also being applicable to a spin system with ground state coupling. This model is then solved analytically in the weak excitation regime. The inclusion of spin dynamics in our model alters the properties of the coherently scattered light at a fundamental level. For a TLS the coherence properties are known to be determined by the input laser. We show that spin scattered light inherits the coherence properties of the spin. This mapping allows us to measure spin dynamics and coherence time through direct measurement of the scattered fields. Furthermore, we show the ability to resolve sub-natural linewidth zeeman splittings. Along with representing an invaluable tool for spin spectroscopy understanding the coherence properties of the spin-scattered field will be vital for spin-photon based quantum technologies.We study the resonance fluorescence properties of an optically active spin 1/2 system, elucidating the effects of a magnetic field on the coherence of the scattered light. We derive a master equation model for this system that reproduces the results of a two level system (TLS) while also being applicable to a spin system with ground state coupling. This model is then solved analytically in the weak excitation regime. The inclusion of spin dynamics in our model alters the properties of the coherently scattered light at a fundamental level. For a TLS the coherence properties are known to be determined by the input laser. We show that spin scattered light inherits the coherence properties of the spin. This mapping allows us to measure spin dynamics and coherence time through direct measurement of the scattered fields. Furthermore, we show the ability to resolve sub-natural linewidth zeeman splittings. Along with representing an invaluable tool for spin spectroscopy understanding the coherence properties of the spin-scattered field will be vital for spin-photon based quantum technologies.

arXiv:2306.08439Jun 14, 20230 citations

Coherent Modified Scattering of Light

Chandrasekhara Venkata Raman, C. S. Venkateswaran

NatureDec 1, 19380 citations

In this paper, we study the modification of coherent scattering processes in dense ensembles. Using absorption imaging, we experimentally demonstrate that the absorption cross section in dense

^{87}\mathrm{Rb}

cold atom ensembles is reduced, with respect to the single-particle response. This reduction is linearly dependent on the optical density and well reproduced by a one-dimensional model of coherent field propagation in an ensemble of quantum two-level systems that self-consistently incorporates multiple scattering contribution. Our model shines light upon the key role of incoherent scattering on the modification of the optical response of dense ensembles and leads to a generalization of the Beer-Lambert law. Our result applies to any effective two-level system ensemble and allows for quantitative and absolute in situ absorption imaging.