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arXiv:2110.12505 · Physical Review Research

Quantitative absorption imaging: The role of incoherent multiple scattering in the saturating regime

Romain Veyron, Vincent Mançois, Jean-Baptiste Gérent, Guillaume Baclet, Philippe Bouyer, Simon Bernon

Published Jul 13, 2022• 12 citations
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Abstract

In this paper, we study the modification of coherent scattering processes in dense ensembles. Using absorption imaging, we experimentally demonstrate that the absorption cross section in dense $^{87}\mathrm{Rb}$ cold atom ensembles is reduced, with respect to the single-particle response. This reduction is linearly dependent on the optical density and well reproduced by a one-dimensional model of coherent field propagation in an ensemble of quantum two-level systems that self-consistently incorporates multiple scattering contribution. Our model shines light upon the key role of incoherent scattering on the modification of the optical response of dense ensembles and leads to a generalization of the Beer-Lambert law. Our result applies to any effective two-level system ensemble and allows for quantitative and absolute in situ absorption imaging.

DOI
10.1103/physrevresearch.4.033033

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In this paper, we study the modification of coherent scattering processes in dense ensembles. Using absorption imaging, we experimentally demonstrate that the absorption cross section in dense 87Rb^{87}\mathrm{Rb}87Rb cold atom ensembles is reduced, with respect to the single-particle response. This reduction is linearly dependent on the optical density and well reproduced by a one-dimensional model of coherent field propagation in an ensemble of quantum two-level systems that self-consistently incorporates multiple scattering contribution. Our model shines light upon the key role of incoherent scattering on the modification of the optical response of dense ensembles and leads to a generalization of the Beer-Lambert law. Our result applies to any effective two-level system ensemble and allows for quantitative and absolute in situ absorption imaging.
Absorption imaging with quasi-resonant laser light is a commonly used technique for probing ultra-cold atomic gases in various geometries. In this paper, we investigate some non-trivial aspects of this method when applying the method to in situ diagnosis of a quasi-two-dimensional (2D) gas. Using Monte Carlo simulations we study the modification of the absorption cross-section of a photon when it undergoes multiple scattering in the gas. We determine the variations of the optical density with various parameters, such as the detuning of the light from the atomic resonance and the thickness of the gas. We compare our results to the known 3D result (the Beer–Lambert law) and outline the specific features of the 2D case.
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Absorption imaging with quasi-resonant laser light is a commonly used technique for probing ultra-cold atomic gases in various geometries. In this paper, we investigate some non-trivial aspects of this method when applying the method to in situ diagnosis of a quasi-two-dimensional (2D) gas. Using Monte Carlo simulations we study the modification of the absorption cross-section of a photon when it undergoes multiple scattering in the gas. We determine the variations of the optical density with various parameters, such as the detuning of the light from the atomic resonance and the thickness of the gas. We compare our results to the known 3D result (the Beer–Lambert law) and outline the specific features of the 2D case.
We measure the coherent scattering of low-intensity, near-resonant light by a cloud of laser-cooled two-level rubidium atoms with a size comparable to the wavelength of light. We isolate a two-level atomic structure by applying a 300-G magnetic field. We measure both the temporal and the steady-state coherent optical response of the cloud for various detunings of the laser and for atom numbers ranging from 5 to 100. We compare our results to a microscopic coupled-dipole model and to a multimode, paraxial Maxwell-Bloch model. In the low-intensity regime, both models are in excellent agreement, thus validating the Maxwell-Bloch model. Comparing to the data, the models are found in very good agreement for relatively low densities ($n/{k}^{3}\ensuremath{\lesssim}0.1$), while significant deviations start to occur at higher density. This disagreement indicates that light scattering in dense, cold atomic ensembles is still not quantitatively understood, even in pristine experimental conditions.
The main objective of this research is to study a particular case of light-matter interaction: the scattering of light in dense atomic samples.The regime of high atomic densities is represented by samples where the distance between neighboring atoms is on the order of the wavelength associated with the atomic transition.In this regime, short-range atomic interactions cannot be neglected, and in these systems, we expect to observe significant modifications in collective effects such as subradiance or superradiance.Overall, the propagation of light through this type of system is not well-known to the scientific community, and the existing models work to describe very specific situations.To pave the way for achieving our overall goal, this work proposes an experimental setup to obtain a dense cloud of 88 Sr, which is the chemical species we work with in our laboratory.For this purpose, atoms previously trapped using a Magneto-Optical Trap are transferred to a Crossed Optical Dipole Trap.During the optimization and characterization of the optical trap, problems were encountered in producing an image with quantitative information of the atomic ensemble and in transferring a large number of atoms in a very small trapping volume.These problems were resolved with the implementation of a Phase Contrast Imaging system and the implementation of an Optical Molasses as an additional cooling step.Under these conditions, we obtained a cloud that can be suitable for conducting studies on collective effects, transitioning from the dilute to the dense regime.The initial experiments, once our atomic ensemble was prepared, involve measuring the coherent transmission of a low-intensity beam through the cloud.For this purpose, incident light near the resonance of a dipolar transition of the type J = 0 ↔ J = 1 of 88 Sr is used, interacting with a homogeneous region of the sample.Simulations of this type of process can be performed using the Coupled Dipole Model, which describes the overall response of light scattering by the sample considering dipole-dipole interactions mediated by light.With this work, we aim to advance the understanding of density effects by comparing the coherent optical response of the dense cloud with the theory based on the Coupled Dipole Model.
Quantum gas microscopes have become a major element for quantum simulations using ultra-cold atoms in optical lattices. They are for example used to observe long-range order such as anti-ferromagnetic correlations in far field optical lattices using density and spin resolved microscopy. Decreasing the period of such lattice offer interesting perspective to increase atom-atom interaction energies and engineer atom-light coupling that our group tackles via the hybridization of cold atoms and nano-structured surfaces.In this poster, we will present how such type of sub-wavelength lattice potentials can be generated by trapping atoms in proximity (tens to hundreds of nanometers) of a nano-structured surface. At such atom to surface distance, the attractive Casimir-Polder force can be compensated by a doubly dressed state trapping method that I will discuss. Such method additionally offers solutions to overcome the diffraction limit of conventional imaging that become critical for sub-wavelength lattices. In this work, I will present the experimental characterization of a sub-wavelength resolution absorption imaging applicable to quantum gas detection. This method requires a quantitative determination of the atom number of dense clouds which has been characterized in this work and demonstrate that the scattering cross section reduces linearly with the optical density. Modelling the propagation of light in dense cloud we show that this reduction can be attributed to re-scattering of the incoherent part of the resonant fluorescence spectrum.The poster will additionally present an update on our recent work on the spectroscopy of Acetylene in sealed hollow core fibers.