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arXiv:2110.08894 · Physical Review A

Effective two-level approximation of a multilevel system driven by coherent and incoherent fields

Romain Veyron, Vincent Mançois, Jean-Baptiste Gérent, Guillaume Baclet, Philippe Bouyer, Simon Bernon

Published Apr 7, 2022• 5 citations
arXivHTMLPDF

Abstract

The numerical simulation of multiple scattering in dense ensembles is the mostly adopted solution to predict their complex optical response. While the scalar- and vectorial-light-mediated interactions are accurately taken into account, the computational complexity still limits current simulations to the low saturation regime and ignores the internal structure of atoms. Here, we propose to go beyond these restrictions, at constant computational cost, by describing a multilevel system by an effective two-level system that best reproduces the coherent and total scattering properties in any saturation regime. The correspondence of our model is evaluated for different experimentally realistic conditions such as the modification of the driving field polarization, the presence of stray magnetic fields, or an incoherent resonant electromagnetic field background. The trust interval of the model is quantified for the ${\mathrm{D}}_{2}$ line of $^{87}\mathrm{Rb}$ atoms, but it could be generalized to any closed transition of a multilevel quantum system.

DOI
10.1103/physreva.105.043105

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The numerical simulation of multiple scattering in dense ensembles is the mostly adopted solution to predict their complex optical response. While the scalar- and vectorial-light-mediated interactions are accurately taken into account, the computational complexity still limits current simulations to the low saturation regime and ignores the internal structure of atoms. Here, we propose to go beyond these restrictions, at constant computational cost, by describing a multilevel system by an effective two-level system that best reproduces the coherent and total scattering properties in any saturation regime. The correspondence of our model is evaluated for different experimentally realistic conditions such as the modification of the driving field polarization, the presence of stray magnetic fields, or an incoherent resonant electromagnetic field background. The trust interval of the model is quantified for the D2{\mathrm{D}}_{2}D2​ line of 87Rb^{87}\mathrm{Rb}87Rb atoms, but it could be generalized to any closed transition of a multilevel quantum system.
In this paper, we study the modification of coherent scattering processes in dense ensembles. Using absorption imaging, we experimentally demonstrate that the absorption cross section in dense 87Rb^{87}\mathrm{Rb}87Rb cold atom ensembles is reduced, with respect to the single-particle response. This reduction is linearly dependent on the optical density and well reproduced by a one-dimensional model of coherent field propagation in an ensemble of quantum two-level systems that self-consistently incorporates multiple scattering contribution. Our model shines light upon the key role of incoherent scattering on the modification of the optical response of dense ensembles and leads to a generalization of the Beer-Lambert law. Our result applies to any effective two-level system ensemble and allows for quantitative and absolute in situ absorption imaging.
The local-field effects are considered which are feasible in a dense ensemble of resonant atoms modeled by multilevel quantum systems. Our approach is based on the generalized two-level system [V.S. Butylkin, A.E. Kaplan, and Yu.G. Khronopulo, Zh. \'Eksp. Teor. Fiz. 59, 921 (1970)]. Making use of this model, we take account of the nonresonant polarization and Stark shift of the absorption line due to the difference in linear polarizabilities of atoms in ground and excited states. With near dipole-dipole interaction and quadratic Stark effect included simultaneously, new features of the hysteresis behavior of the population difference as a function of the external-field intensity are predicted.
We propose and develop a method for theoretical description of circularly (elliptically) polarized optical pulse resonant coherent interactions with two-level atoms. The method is based on the time-evolution equations of a two-level quantum system in the presence of a time-dependent dipole perturbation for electric dipole transitions between states with total angular-momentum projection difference $(\ensuremath{\Delta}{J}_{z}=\ifmmode\pm\else\textpm\fi{}1)$ excited by a circularly polarized electromagnetic field [Feynman et al., J. Appl. Phys. 28, 49 (1957)]. The adopted real-vector representation approach allows for coupling with the vectorial Maxwell's equations for the optical wave propagation and thus the resulting Maxwell pseudospin equations can be numerically solved in the time domain without any approximations. The model permits a more exact study of the ultrafast coherent pulse propagation effects taking into account the vector nature of the electromagnetic field and hence the polarization state of the optical excitation. We demonstrate self-induced transparency effects and formation of polarized solitons. The model represents a qualitative extension of the well-known optical Maxwell-Bloch equations valid for linearly polarized light and a tool for studying coherent quantum control mechanisms.
We derive equations for the strongly coupled system of light and dense atomic ensembles. The formalism includes an arbitrary internal-level structure for the atoms and is not restricted to weak excitation of atoms by light. In the low-light-intensity limit for atoms with a single electronic ground state, the full quantum field-theoretical representation of the model can be solved exactly by means of classical stochastic electrodynamics simulations for stationary atoms that represent cold atomic ensembles. Simulations for the optical response of atoms in a quantum degenerate regime require one to synthesize a stochastic ensemble of atomic positions that generates the corresponding quantum statistical position correlations between the atoms. In the case of multiple ground levels or at light intensities where saturation becomes important, the classical simulations require approximations that neglect quantum fluctuations between the levels. We show how the model is extended to incorporate corrections due to quantum fluctuations that result from virtual scattering processes. In the low-light-intensity limit, we illustrate the simulations in a system of atoms in a Mott-insulator state in a two-dimensional optical lattice, where recurrent scattering of light induces strong interatomic correlations. These correlations result in collective many-atom subradiant and superradiant states and a strong dependence of the response on the spatial confinement within the lattice sites.
We measure the coherent scattering of low-intensity, near-resonant light by a cloud of laser-cooled two-level rubidium atoms with a size comparable to the wavelength of light. We isolate a two-level atomic structure by applying a 300-G magnetic field. We measure both the temporal and the steady-state coherent optical response of the cloud for various detunings of the laser and for atom numbers ranging from 5 to 100. We compare our results to a microscopic coupled-dipole model and to a multimode, paraxial Maxwell-Bloch model. In the low-intensity regime, both models are in excellent agreement, thus validating the Maxwell-Bloch model. Comparing to the data, the models are found in very good agreement for relatively low densities ($n/{k}^{3}\ensuremath{\lesssim}0.1$), while significant deviations start to occur at higher density. This disagreement indicates that light scattering in dense, cold atomic ensembles is still not quantitatively understood, even in pristine experimental conditions.
We study interactions of light with a sample of two-level atoms. Quantum statistical effects of degenerate boson and fermion gases are described by using the quantum field theory of atom-photon interactions, fully including the angular momentum degeneracies. Coupled propagation equations are given for light and matter fields, and plausible general simplifications are enumerated.^ In the limit of large atom-field detuning, multiple scattering of light and QED linewidths and line shifts may be ignored, and the propagation equations of light and matter fields may be decoupled. A general expression for the spectrum of the scattered light is derived, complete with the dependence on atomic level scheme, on various light polarizations, and on the geometry of the experiment. With these simplifications we are able to find distinct qualitative features in the spectrum of the scattered light in the case of both fermions and bosons that depend on the statistics of atoms. This is because for bosons (fermions), those scattering events in which an atom recoils to an already occupied state are enhanced (inhibited).^ As the driving light gets closer to the atomic resonance, multiple scattering and vacuum fluctuations of the electromagnetic fields should also be taken into account. We write the equations of motion for the excited state field operators by eliminating the vacuum electromagnetic field. It is always assumed that the driving external laser field is in the coherent state. We find in the limit of low light intensity, a hierarchy of equations of motion for correlation functions that contain one excited-atom field and one, two, three, etc., ground state atom fields. It is conjectured that the entire linear hierarchy may be solved by solving numerically the classical equations for the coupled system of electromagnetic fields and charged harmonic oscillators. We discuss the emergence of resonant dipole-dipole interactions and collective linewidths, and delineate the limits of validity of the column density approach in terms of non-cooperative atoms by presenting a mathematical example in which this approach is exact. ^