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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

The Lindblad dynamics of a Fermi system in a particle dissipative environment

Eliade N. Stefanescu, Paul E. Sterian, Andreea-Rodica P. Sterian

Published Nov 14, 2003• 5 citations
Publisher

Abstract

An essential problem of the quantum information systems is the controllability and observability of the quantum states, generally described by Lindblad's master equation with phenomenological coefficients. However, in its general form, this equation describes a decay of the mean-values, but not necessarily the expected decaying transitions. We propose a quantum master equation with microscopic coefficients where these transitions are correctly described, and investigate the properties of the dissipative coefficients. Being of Lindblad's form, this equation preserves the quantum-mechanical properties of the density matrix during the whole evolution of the system and is in accordance with the entropy principle. On this basis, generalized Bloch-Feynman equations with microscopic coefficients for N-level systems are obtained.

DOI
10.1117/12.537568

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An essential problem of the quantum information systems is the controllability and observability of the quantum states, generally described by Lindblad's master equation with phenomenological coefficients. However, in its general form, this equation describes a decay of the mean-values, but not necessarily the expected decaying transitions. We propose a quantum master equation with microscopic coefficients where these transitions are correctly described, and investigate the properties of the dissipative coefficients. Being of Lindblad's form, this equation preserves the quantum-mechanical properties of the density matrix during the whole evolution of the system and is in accordance with the entropy principle. On this basis, generalized Bloch-Feynman equations with microscopic coefficients for N-level systems are obtained.
In a previous paper, we derived a master equation for fermions, of Lindblad's form, with coefficients depending on microscopic quantities. In this paper, we study the properties of the dissipative coefficients taking into account the explicit expressions of: (a) the matrix elements of the dissipative potential, evaluated from the condition that, essentially, this potential induces transitions among the system eigenstates without significantly modifying these states, (b) the densities of the environment states according to the Thomas–Fermi model, and (c) the occupation probabilities of these states taken as a Fermi–Dirac distribution. The matrix of these coefficients correctly describes the system dynamics: (a) for a normal, Fermi–Dirac distribution of the environment population, the decays dominate the excitation processes; (b) for an inverted (exotic) distribution of this population, specific to a clustering state, the excitation processes are dominant.
We derive a quantum master equation for a system of femions coupled to the blackbody radiation field and to many other excitations of the surrounding particles. In comparison with other master equations for many-level systems, the new master equation depends on microscopic coefficients (as functions of physical constants, matrix elements, densitie of the environment states, and occupation probabilities of these states), and includes two additional terms: (1) a term depending on the selfconsistent field of the collective motion of the system or of other surrounding particles, and (2) a non-Markovian term.
We consider a system of Z fermions coupled to a dissipative environment through a two-body potential. We represent the system in a basis of single-particle, two-particle, … Z-particle excitated states. Using a procedure for averaging the rapid oscillations of the reduced density matrix in the interaction picture, the master equation of the system takes the form of a series expansion of powers of the dissipative potential matrix elements. The term of the second-order describes single-particle transitions, while the higher-order terms correspond to correlated transitions of the system particles. For the second- and the third-order terms, we derive microscopic expressions of the dissipative coefficients. For dissipative systems, when the state collectivity is broken into pieces through quantum diffusion, we use the quantum master equation of the second-order approximation. This equation satisfies basic physical conditions: particle conservation, Fermi–Dirac or Bose–Einstein distributions as asymptotic solutions of the populations, and entropy increase. On this basis, the decay of a Fermi system interacting with a many-mode electromagnetic field is described in terms of microscopic quantities: the matrix elements of the dissipative potential, the densities of the environment states, and the occupation probabilities of these states. A near-dipode–dipode interaction of the system with other neighbouring systems is taken into account. In addition to the coupling of the polarization with the population, included in the usual equations for two-level systems as a non-linear detuning, in equations for N-level systems two new couplings of the polarizations appear: a coupling due to the proximity potential, and a coupling due to the local field corrections, as a renormalization of the Rabi frequencies.
Microscopic master equations have gained traction for the dissipative treatment of molecular spin and solid-state systems for quantum technologies. Single particle approximations are often invoked to treat these systems, which can lead to unphysical evolution when combined with master equation approaches. We present a mathematical constraint on the system-environment parameters to ensure that microscopically-derived Markovian master equations preserve fermionic, NNN-representable statistics when applied to reduced systems. We demonstrate these constraints for the recently derived unified master equation and universal Lindblad equation, along with the Redfield master equation for cases when positivity issues are not present. For operators that break the constraint, we explore the addition of Pauli factors to recover NNN-representability. This work promotes feasible applications of novel microscopic master equations for realistic chemical systems.
We consider a fermionic quantum system exchanging particles with an environment at a fixed temperature and study its reduced evolution by means of a Redfield-I equation with time-dependent (non-Markovian) coefficients. We find that the description can be efficiently reduced to a standard-form Redfield-II equation, however, with a obeying a universal law. At early times, after the system and environment start in a product state, the appears to be very high, yet eventually it settles down towards the true environment value. In this way, we obtain a time-local master equation, offering high accuracy at all times and preserving the crucial properties of the density matrix. It includes non-Markovian relaxation processes beyond the secular approximation and time-averaging methods and can be further applied to various types of Gorini-Kossakowski-Sudarshan-Lindblad equations. We derive the theory from first principles and discuss its application using a simple example of a single quantum dot.