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Conference on Lasers and Electro-Optics

Suppression of excited state absorption (ESA) in lasing materials and non-linear optical pulse propagation dynamics in the media subject to ESA

Roman L. Kolesov, Elena Kuznetsova, Olga A. Kocharovskaya

Published Jan 1, 2005• 0 citations
Publisher

Abstract

A method of suppression of excited state absorption (ESA) by means of electromagnetically induced transparency (EIT) is proposed. Optical pulse propagation in the medium subject to ESA is considered and relaxation soliton-type solutions are found.
DOI
10.1109/cleo.2005.202036

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A method of suppression of losses due to excited-state absorption (ESA) in laser crystals is proposed, based on the well-known phenomenon of electromagnetically induced transparency. Typical situations in which ESA prevents lasing are considered. Theoretical analysis shows that by using an additional driving laser field one can inhibit ESA and make lasing possible. On the basis of available spectroscopic information estimates for rare-earth-ion-doped laser materials are presented. They show the feasibility of obtaining optical gain at parity-allowed $4{f}^{n}\ensuremath{\leftrightarrow}4{f}^{n\ensuremath{-}1}5d$ transitions of rare-earth ions in the ultraviolet spectral region after suppression of ESA at an emission wavelength into the conduction band of a host material.
The subject of electromagnetically induced transparency (EIT) is reviewed in this paper. Emphasis is placed on the experimental work reported in this field since 1990. Theoretical work is also covered, although it is not intended to review all the very numerous recent theoretical treatments on this topic. The basic physical ideas behind EIT are elucidated. The relation of EIT to other processes involving laser-induced atomic coherence, such as coherent population trapping, coherent adiabatic population transfer and lasing without inversion, is discussed. Experimental work is described covering the following topics: EIT with pulsed and continuous-wave sources, lasing without inversion, pulse propagation in a laser dressed medium and EIT in nonlinear optical processes. A full set of references and a bibliography are included.
The subject of electromagnetically induced transparency (EIT) is reviewed in this paper. Emphasis is placed on the experimental work reported in this field since 1990. Theoretical work is also covered, although it is not intended to review all the very numerous recent theoretical treatments on this topic. The basic physical ideas behind EIT are elucidated. The relation of EIT to other processes involving laser-induced atomic coherence, such as coherent population trapping, coherent adiabatic population transfer and lasing without inversion, is discussed. Experimental work is described covering the following topics: EIT with pulsed and continuous-wave sources, lasing without inversion, pulse propagation in a laser dressed medium and EIT in nonlinear optical processes. A full set of references and a bibliography are included.
Abstract. The subject of electromagnetically induced transparency (EIT) is reviewed in this paper. Emphasis is placed on the experimental work reported in this ®eld since 1990. Theoretical work is also covered, although it is not intended to review all the very numerous recent theoretical treatments on this topic. The basic physical ideas behind EIT are elucidated. The relation of EIT to other processes involving laser-induced atomic coherence, such as coherent population trapping, coherent adiabatic population transfer and lasing without inversion, is discussed. Experimental work is described covering the following topics: EIT with pulsed and continuous-wave sources, lasing without inversion, pulse propagation in a laser dressed medium and EIT in nonlinear optical processes. A full set of references and a bibliography are included. 1.
Quantum coherence and interference in atomic systems can lead to interesting optical phenomena such as nonabsorbing resonances, lasing without inversion, generating an ultrahigh index of refraction without absorption, propagation of light pulses without losses. In the last-named is given the title transparency. Up to now it is known some types of transparency in multi-level resonant media. One of them is electromagnetically induced transparency (EIT). The phenomenon of EIT in the propagation of laser radiation through an absorbing medium has been recently investigated and explained in terms of quantum coherence and interference for multi-level atomic system. For instance in the (Lambda) -system, if the atomic medium is prepared in a quantum superposition of states, matched pulses, i.e., a pair of optical pulses whose amplitude and phase have a well defined relation, propagate without absorption. The mechanism of coherent population trapping is responsible for EIT in a (Lambda) -system. There is another, well known mechanism for creating transparency in a two-state atom: self-induced transparency, or SIT. Here, a single pulse whose area (the integral of its Rabi frequency over time) is 2(pi) is applied to the medium. Such a pulse causes the atoms to cycle smoothly from the ground to the excited state and then back again. In principle, such a pulse can propagate over long distances. SIT can be generalized to multi-level systems and multiple quasi-monochromatic fields. Generalization of SIT in a (Lambda) -system was obtained in reference 2. In this report we present a new type of transparency (combined transparency). This type describes propagation of laser pulse through a (Lambda) -type medium where the initial atomic state is prepared in the form of spatially varying coherent superposition of low-energetic states (initial coherency gradient). The common envelope behaves as usual 2(pi) hyperbolic secant pulse, but the ratio between the components of frequencies transitions 1> yields 3> and 2> yields 3> changes due to coherent Raman scattering so (phi) equals atan(E1/E2) equals (pi) /2-Gz, where z is the coordinate, G is the constant determined by both the incident pulse parameters and the initial coherence between the atomic states. Our solution demonstrates a direct connection of EIT in adiabatic regime to the SIT effects. This type of a transparency is given the title screw-type transparency, because for the given form of incident pulse (pitch of screw) medium is transparent, if medium's the initial coherence gradient is correspondingly prepared (thread on a engine nut). Besides a transparency, this phenomenon contains a transformation of the incident pulse frequency during the process of the propagation. This property of the phenomena can be result in a complete conversion of the frequency.
Delay bandwidth products (DBPs) and physical pulselengths obtainable in media exhibiting electromagnetically induced transparency (EIT) are analyzed. The study is performed in stationary media as well as for dynamic storing of light pulses in such media. In the latter case, the dispersion inherent in storage and readout of the pulses is analyzed. It is shown that absorption and the group velocity dispersion (GVD) are limiting factors. Analytical expressions for the minimum compressed pulselength and DBP are derived, and these expressions show good agreement with simulations of pulse propagation in EIT media.