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Science

Superradiant Rayleigh Scattering from a Bose-Einstein Condensate

S. Inouye, A. P. Chikkatur, Dan Stamper-Kurn, J. Stenger, David E. Pritchard, Wolfgang Ketterle

Published Jul 23, 1999• 538 citations
Publisher

Abstract

Rayleigh scattering off a Bose-Einstein condensate was studied. Exposing an elongated condensate to a single off-resonant laser beam resulted in the observation of highly directional scattering of light and atoms. This collective light scattering is caused by the coherent center-of-mass motion of the atoms in the condensate. A directional beam of recoiling atoms was built up by matter wave amplification.

DOI
10.1126/science.285.5427.571

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Rayleigh scattering off a Bose-Einstein condensate was studied. Exposing an elongated condensate to a single off-resonant laser beam resulted in the observation of highly directional scattering of light and atoms. This collective light scattering is caused by the coherent center-of-mass motion of the atoms in the condensate. A directional beam of recoiling atoms was built up by matter wave amplification.
The non-equilibrium dynamics of the superradiant scattering of light from a BEC is experimentally investigated by monitoring the time evolution of the population in the condensate. In the experiment, a cigar-shaped Bose-Einstein condensate of /sup 87/Rb atoms is produced and is exposed to a single off-resonant laser pulse directed along the condensate symmetry axis. The superradiant back-scattering of light creates a matter wave pulse moving in the same direction of the laser beam at twice the photon recoil velocity with respect to the original condensate. The efficiency of the process is limited by decoherence between the two atomic spatially overlapped wavepackets. The temporal evolution of the condensate observed in the experiment as well as the results of a simple semiclassical model in which the condensate is described by a density operator for the motional states. The population of the two matter wavepackets as a function of the light pulse duration is reported, together with the experimental points with the analytical formula resulting from the theory of collective atomic recoil laser (CARL).
Equations of a semiclassical model of superradiant Rayleigh scattering of high-intensity short light pulses from a Bose-Einstein condensate of dilute atomic gases are solved numerically taking into account the excitation of atoms by coherent Rayleigh radiation and their recoil in the backward direction. The evolution of the populations of coherent atomic states with a particular momentum is studied, and the pulse shape and the structure of the spectrum of such scattering are found in relation to the laser beam intensity and the recoil kinetic energy of atoms.
We present the results of an experiment on light scattering from an elongated Bose-Einstein condensate (BEC) interacting with a far-off-resonant pump laser. By collective atomic recoil lasing (CARL) a coherent superposition of two atomic wave packets with different momenta is created. Varying the intensity of a weak counterpropagating laser beam we observe the transition from the pure superradiant regime to the Bragg scattering regime, where Rabi oscillations in a two-level system are observed. The process is limited by the decoherence between the two atomic wave packets. In the superradiant regime the experiment gives evidence of a contribution to decoherence which depends on the initial velocity of the condensate. The system is described by the CARL-BEC model, which is a generalization of the Gross-Pitaevskii model to include the self-consistent evolution of the scattered field and a phase-diffusion decoherence process, which accounts for the observed damping.
Due to its coherence properties and high optical depth, a Bose–Einstein condensate [BEC] provides an ideal setting to investigate collective atom-light interactions. Superradiant light scattering [SLS] in a BEC is a fascinating example of such an interaction. It is an analogous process to Dicke superradiance, in which an electronically inverted sample decays collectively, leading to the emission of one or more light pulses in a well-defined direction. Through time-resolved measurements of the superradiant light pulses emitted by an end-pumped BEC, we study the close connection of SLS with Dicke superradiance. A 1D model of the system yields good agreement with the experimental data and shows that the dynamics result from the structures that build up in the light and matter-wave fields along the BEC. This paves the way for exploiting the atom–photon correlations generated by the superradiance.
Recent experiments have demonstrated superradiant Raman scattering from a Bose-Einstein condensate driven by a single off-resonant laser beam. We present a quantum theory describing this phenomenon, showing Raman amplification of matter wave due to collective atomic recoil from 3-level atoms in a $\ensuremath{\Lambda}$-configuration. When atoms are initially in a single lower internal state, a closed two-level system is realized between atoms with different internal states, and entangled atom-photon pairs can be generated. When atoms are initially prepared in both the lower internal states, a fraction of atoms recoiling in the backward direction can be generated.
The superradiant Rayleigh scattering of high-intensity light pulses by the Bose-Einstein condensate of rubidium vapor is studied using the model proposed earlier. It is demonstrated that four states with a certain momentum are occupied under the experimental conditions (two states correspond to the forward recoil and two others correspond to the backward recoil). Condensate pulsations between the zero-momentum state and the above states are detected and studied. The corresponding shape of the coherent Rayleigh pulse is found.