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International Journal of Quantum Information

CALCULATION OF THE 3D INTERACTION GEOMETRY FOR TWO INTERLINKED χ(2) PROCESSES GENERATING ENTANGLED TRIPLETS

Maria Bondani, Alessia Allevi, Alessandra Andreoni

Published Feb 1, 2007• 0 citations
Publisher

Abstract

The geometrical conditions are analytically calculated in which two interlinked second-order nonlinear interactions generating entangled triplets are phase-matched in 3D. The interactions are the spontaneous parametric downconversion of an intense pump and the upconversion of a portion of the downconversion cones by a further pump. The calculation applies to type-I interactions occurring in uniaxial crystals and allows us to forecast positions and frequencies of the entangled triplets experimentally generated. The photon number statistics and the intensity correlations are also measured.

DOI
10.1142/s0219749907002463

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The geometrical conditions are analytically calculated in which two interlinked second-order nonlinear interactions generating entangled triplets are phase-matched in 3D. The interactions are the spontaneous parametric downconversion of an intense pump and the upconversion of a portion of the downconversion cones by a further pump. The calculation applies to type-I interactions occurring in uniaxial crystals and allows us to forecast positions and frequencies of the entangled triplets experimentally generated. The photon number statistics and the intensity correlations are also measured.
An analytical calculation of the interaction geometry of two interlinked second-order nonlinear processes fulfilling phase-matching conditions is presented. The method is developed for type-I uniaxial crystals and gives the positions on a screen beyond the crystal of the entangled triplets generated by the interactions. The analytical results are compared to experiments realized in the macroscopic regime. Preliminary tests to identify the triplets are also performed based on ntensity correlations.
We consider the quantum state of light produced via direct parametric decay of pump photons into photon triples in a medium with cubic nonlinearity. For this state generated in the near-collinear frequency-degenerate regime, the third- and second-order Glauber's correlation functions are calculated and the intensity distribution over frequency and wave vector is found. It is shown that the number of photons generated into a single mode via the three-photon down-conversion is proportional to the width of the frequency-angular intensity distribution for the corresponding two-photon phase matching (spontaneous parametric down-conversion). The intensity of three-photon parametric down-conversion is shown to have an extremely broad frequency spectrum, even for a fixed angle of scattering.
We propose a scheme for generating polarization-entangled photon pairs using a χ((2)) nonlinear photonic crystal, which is designed for enabling two concurrent quasi-phase-matched spontaneous parametric downconversion processes. Beamlike photon pairs produced from each process are collinear but noncollinear with the pump. Moreover, the source we design works in a postselection-free way and applies to both degenerate and nondegenerate cases. Combining possible waveguide technologies, our scheme may provide an integrated polarization entanglement source.
We investigate production of three-photon and four-photon states in cascaded parametric processes of photon splitting and summing in χ (2)nonlinear media, under action of pump field. Generation of photon triplets using simultaneously phase matched three-photon processes: ω0↔ω1+ω2 , ω2↔ω1+ω1 , is considered in dual-grating layered structure that involves nonlinear and linear segments. The production of heralded two-photon entangled states from three-photon states is analyzed for this configuration by using the method of conditional detection of auxiliary photons. Cascaded four-photon downconversion based on simultaneously phase matched three-photon processes: ω0↔ω2 +ω2 , ω2↔ω1+ω1 is arranged for phase-reversed configuration. The effects of correlation between photons in both three-photon and four-photon states is analyzed in the regimes of amplification of corresponding modes at the frequency of three-photon downconversion ω1 = ω0/3 and the frequency of four-photon down-conversion ω1 = ω0/4respectively for both cascaded systems.
The transcendental equations of vector phase matching are transformed into a fourth-order polynomial equation that admits an analytical solution. The real roots of this equation provide the optical axis orientations that are useful for efficient down-conversion in nonlinear uniaxial crystals. The production of entangled photon pairs is discussed in both collinear and non-collinear configurations of the spontaneous parametric down-conversion (SPDC) process. Degenerate and non-degenerate cases are also distinguished. As a practical example, SPDC processes of type-I and type-II are studied for beta-barium borate (BBO) crystals. The predictions are in very good agreement with experimental measurements already reported in the literature and include theoretical results of other authors as particular cases. Some properties that seem to be exclusive to BBO crystals are reported; the experimental verification of the latter would allow a better characterization of these crystals.